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Dual-comb spectroscopy enables broadband analysis of key molecules with unparalleled frequency resolution and exceptional signal-to-noise ratios across various spectral regions. However, fully harnessing its potential for broadband…

Experiments and theoretical modeling yielded significant progress towards understanding of Kerr-effect induced optical frequency comb generation in microresonators. However, the simultaneous interaction of hundreds or thousands of optical…

High resolution and fast detection of molecular vibrational absorption is important for organic synthesis, pharmaceutical process and environmental monitoring, and is enabled by mid-infrared (mid-IR) laser frequency combs via dual-comb…

Frequency combs, spectra of evenly-spaced narrow phase-coherent laser lines, have revolutionized precision measurements. On-chip frequency comb generators hold much promise for fully-integrated instruments of time and frequency metrology.…

Mid-infrared microscopy is an important tool for biological analyses, allowing a direct probe of molecular bonds in their low energy landscape. In addition to the label-free extraction of spectroscopic information, the application of…

Rapid and large scanning of a dissipative Kerr-microresonator soliton comb with the characterization of all comb modes along with the separation of the comb modes is imperative for the emerging applications of the frequency-scanned soliton…

Dual-comb spectroscopy is emerging as one of the most appealing applications of mid-infrared frequency combs for high-resolution molecular spectroscopy, as it leverages on the unique coherence properties of frequency combs combined with the…

We demonstrate the advantages of THz frequency combs for high-resolution spectroscopy. This benefits from wide spectral coverage and the exact knowledge of the frequency position of each comb component. Heterodyne detection combined with a…

Instrumentation and Detectors · Physics 2024-12-03 Francis Hindle , Alexandra Khabbaz , Anthony Roucou , Jean-Francois Lampin , Gaël Mouret

Ultrabroadband electro-optic sampling with few-cycle optical pulses is known to be an extremely sensitive technique to detect electric field amplitudes. By combining this method with dual-comb spectroscopy and with a new class of ultrafast…

A fully stabilized mid-infrared optical frequency comb spanning from 2.9 to 3.4 um is described. The comb is based on half-harmonic generation in a femtosecond optical parametric oscillator, which transfers the high phase coherence of a…

Optics · Physics 2017-04-05 Markku Vainio , Juho Karhu

Frequency combs are powerful tools for many applications and high performances are achieved by stabilizing these lasers. For operation in the mid-infrared, quantum cascade lasers (QCL) are ideal candidates as they present numerous…

Two techniques that employ equally spaced trains of optical pulses to map an optical high frequency into a low frequency modulation of the signal that can be detected in real time are compared. The development of phase-stable optical…

Quantum Physics · Physics 2017-08-22 Kochise Bennett , Jeremy Rouxel , Shaul Mukamel

Chip-scale semiconductor laser frequency combs offer remarkable prospects for compact and power-efficient optical sensors. For the laser to be suitable for typical comb applications, its degree of coherence must first be assessed from a…

Dual-comb spectroscopy is a powerful technique for real-time, broadband optical sampling of molecular spectra which requires no moving components. Recent developments with microresonator-based platforms have enabled frequency combs at the…

Mid-infrared (mid-IR) spectroscopy offers unparalleled sensitivity for the detection of trace gases, solids and liquids, which is based on the existence of strong telltale vibrational bands in this part of the spectrum. It was shown more…

Optics · Physics 2016-08-29 Viktor O. Smolski , Honglei Yang , Jia Xu , Konstantin L. Vodopyanov

A 12.5 GHz-spaced optical frequency comb locked to a Global Positioning disciplined oscillator for near-IR spectrograph calibration is presented. The comb is generated via filtering a 250 MHz-spaced comb. Subsequency nonlinear broadening of…

Optics · Physics 2015-05-18 F. Quinlan , G. Ycas , S. Osterman , S. Diddams

We measure phase-dependent Kerr soliton squeezing and anti-squeezing in the time-domain dualcomb interferograms generated using two independent frequency comb lasers. The signal appears as non-stationary quantum noise that varies with the…

The noise dynamics of an Optical Frequency Comb (OFC) based on a mode-locked Ti-Sapphire laser is analyzed in terms of noise modes. A spectrally resolved multipixel homodyne detection enables the simultaneous measurement of the amplitude…

Instrumentation and Detectors · Physics 2021-08-04 Matthieu Ansquer , Valérian Thiel , Syamsundar De , Bérengère Argence , Gregory Gredat , Fabien Bretenaker , Nicolas Treps

We present quasi-real-time dual-comb spectroscopy (DCS) using two Yb:fiber combs with ~750 MHz repetition rates. A computational coherent averaging technique is employed to correct timing and phase fluctuations of the measured dual-comb…

To meet the challenges of high-resolution molecular spectroscopy, increasingly sophisticated spectroscopic techniques were developed. For a long time FTIR and laser-based spectroscopies were used for these studies. The recent development of…