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By combining band gap engineering with the self-organized growth of quantum dots, we present a scheme of adjusting the mid-infrared absorption properties to desired energy transitions in quantum dot based photodetectors. Embedding the self…

Other Condensed Matter · Physics 2013-05-29 F. F. Schrey , L. Rebohle , T. Mueller , G. Strasser , K. Unterrainer , D. P. Nguyen , N. Regnault , R. Ferreira , G. Bastard

Ultra-precision machining of metals, the breaking of nanowires under tensile stress and fracture of nanoscale materials are examples of technologically important processes which are both extremely difficult and costly to investigate…

Materials Science · Physics 2007-05-23 Maciej Bobrowski , Jacek Dziedzic , Jaroslaw Rybicki

Routine investigations of plasmonic phenomena at the quantum level present a formidable computational challenge due to the large system sizes and ultrafast timescales involved. This Feature Article highlights the use of density functional…

Mesoscale and Nanoscale Physics · Physics 2025-06-19 Nikhil S. Chellam , Subhajyoti Chaudhuri , Abhisek Ghosal , Sajal K. Giri , George C. Schatz

First-principles calculations were performed to investigate the electronic structure of two-dimensional (2-D) Ge, Sn, and Pb without and with the presence of an external electric field in combination with spin-orbit coupling. Tight-binding…

We analyze and present applications of a recently proposed empirical tight-binding scheme for investigating the effects of alloy disorder on various electronic and optical properties of semiconductor alloys, such as the band gap variation,…

Materials Science · Physics 2024-01-31 Anh-Luan Phan , Alessandro Pecchia , Alessia Di Vito , Matthias Auf der Maur

Dilute nitride bismide GaNBiAs is a potential semiconductor alloy for near- and mid-infrared applications, particularly in 1.55 $\mu$m optical communication systems. Incorporating dilute amounts of Bismuth (Bi) into GaAs reduces the…

Mesoscale and Nanoscale Physics · Physics 2017-06-22 W. J. Fan , Sumanta Bose , D. H Zhang

\textit{Ab initio} pseudo-atomic orbital (PAO) Hamiltonians express the electronic structure of a solid in a compact, localized basis that spans the same Hilbert space as a conventional Slater--Koster tight-binding model, thereby providing…

Materials Science · Physics 2026-04-17 Marco Buongiorno Nardelli

Bridging the gap between first principles methods and empirical schemes, the density functional based tight-binding method (DFTB) has become a versatile tool in predictive atomistic simulations over the past years. One of the major…

Materials Science · Physics 2015-04-02 Vitalij Lutsker , Balint Aradi , Thomas A. Niehaus

We propose to adapt the confined pseudo-atomic orbitals underpinning the precalculated Slater-Koster (SK) interaction tables in Density Functional Tight Binding (DFTB) to local atomic environments. We demonstrate significant improvement in…

Tuning the bandgap in ternary III-V semiconductors via modification of the composition or the strain in the material is a major approach for the design of optoelectronic materials. Experimental approaches screening a large range of possible…

Materials Science · Physics 2023-07-10 Badal Mondal , Marcel Kröner , Thilo Hepp , Kerstin Volz , Ralf Tonner-Zech

We develop a probabilistic machine learning model and use it to screen for new hybrid organic-inorganic perovskites (HOIPs) with targeted electronic band gap. The data set used for this work is highly diverse, containing multiple atomic…

Materials Science · Physics 2021-12-08 Vu Ngoc Tuoc , Nga T. T. Nguyen , Vinit Sharma , Tran Doan Huan

The interaction between electrons and lattice vibrations determines key physical properties of materials, including their electrical and heat transport, excited electron dynamics, phase transitions, and superconductivity. We present a new…

Materials Science · Physics 2018-07-04 Luis A. Agapito , Marco Bernardi

We suggest a technique for the observation of a predicted supersolid phase in extended Bose-Hubbard models which are potentially realizable in cold atom optical lattice systems. In particular, we discuss important subtleties arising from…

Other Condensed Matter · Physics 2009-11-11 V. W. Scarola , E. Demler , S. Das Sarma

We have performed Linearized Augmented Plane Wave (LAPW) calculations for five crystal structures (alpha, dhcp, sc, fcc, bcc) of Boron which we then fitted to a non-orthogonal tight-binding model following the Naval Research Laboratory…

Materials Science · Physics 2016-06-29 Joseph W. McGrady , Dimitrios A. Papaconstantopoulos , Michael J. Mehl

A general-purpose Density Functional Tight Binding method, the GFN-xTB model is gaining increased popularity in accurate simulations that are out of scope for conventional ab initio formalisms. We show that in its original GFN1-xTB…

Chemical Physics · Physics 2021-12-14 Leonid Komissarov , Toon Verstraelen

The electronic structure of the molecular compound (TTM-TTP)I_3, which exhibits a peculiar intra-molecular charge ordering, has been studied using multi-configuration ab initio calculations. First we derive an effective Hubbard-type model…

We propose a new method of calculating electronically excited states that combines a density functional theory (DFT) based ground state calculation with a linear response treatment that employs approximations used in the time-dependent…

Chemical Physics · Physics 2016-05-11 Robert Rüger , Erik van Lenthe , Thomas Heine , Lucas Visscher

Rapid design and development of the emergent ultra-wide bandgap semiconductors Ga$_2$O$_3$ and Al$_2$O$_3$ requires a compact model of their electronic structures, accurate over the broad energy range accessed in future high-field,…

Mesoscale and Nanoscale Physics · Physics 2022-11-01 Yifan , Zhang , Mengren , Liu , Guru Khalsa , Debdeep Jena

We introduce a machine learning method in which energy solutions from the Schrodinger equation are predicted using symmetry adapted atomic orbitals features and a graph neural-network architecture. \textsc{OrbNet} is shown to outperform…

We predict and examine various topological states on a two-dimensional (2D) triangular kagome lattice (TKL) using the tight-binding (TB) models and theory of topological quantum chemistry (TQC). Firstly, on the basis of TQC, we diagnose…

Mesoscale and Nanoscale Physics · Physics 2023-09-25 Yun-Feng Chen , Dao-Xin Yao