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We present a conceptually simple method for treating electron-phonon scattering and phonon limited mobilities. By combining Green's function based transport calculations and molecular dynamics (MD), we obtain a temperature dependent…

Mesoscale and Nanoscale Physics · Physics 2017-06-28 Troels Markussen , Mattias Palsgaard , Daniele Stradi , Tue Gunst , Mads Brandbyge , Kurt Stokbro

The past decade has seen the emergence of ab initio computational methods for calculating phonon-limited carrier mobilities in semiconductors with predictive accuracy. More realistic calculations ought to take into account additional…

Materials Science · Physics 2023-04-12 Joshua Leveillee , Xiao Zhang , Emmanouil Kioupakis , Feliciano Giustino

The nonlocal electron-phonon couplings in organic semiconductors responsible for the fluctuation of intermolecular transfer integrals has been the center of interest recently. Several irreconcilable scenarios coexist for the description of…

Materials Science · Physics 2021-08-04 Weitang Li , Jiajun Ren , Zhigang Shuai

This work is devoted to the \textit{ab initio} calculation of transport and optical properties of aluminum. The calculation is based on the quantum molecular dynamics simulation, density functional theory and the Kubo-Greenwood formula.…

Computational Physics · Physics 2013-10-16 D. V. Knyazev , P. R. Levashov

We probe the accuracy limit of {\it ab initio} calculations of carrier mobilities in semiconductors, within the framework of the Boltzmann transport equation. By focusing on the paradigmatic case of silicon, we show that fully predictive…

Materials Science · Physics 2018-03-28 Samuel Ponce , Elena R. Margine , Feliciano Giustino

The coherent quantum effect becomes increasingly important in the heat dissipation bottleneck of semiconductor nanoelectronics with the characteristic size shrinking down to few nano-meters scale nowadays. However, the quantum mechanical…

Mesoscale and Nanoscale Physics · Physics 2020-11-18 Yangyu Guo , Marc Bescond , Zhongwei Zhang , Mathieu Luisier , Masahiro Nomura , Sebastian Volz

We propose a feasible and effective approach to study quantum thermal transport through anharmonic systems. The main idea is to obtain an {\it effective} harmonic Hamiltonian for the anharmonic system by applying the self-consistent phonon…

Statistical Mechanics · Physics 2016-10-19 Dahai He , Juzar Thingna , Jian-Sheng Wang , Baowen Li

While the vast majority of calculations reported on molecular conductance have been based on the static non-equilibrium Green's function formalism combined with density functional theory, in recent years a few time-depedent approaches to…

We present a novel theory of charge-carrier mobilities in organic molecular crystals of high purity. Our approach is based on Holstein's original concept of small-polaron bands but generalized with respect to the inclusion of nonlocal…

Soft Condensed Matter · Physics 2007-05-23 K. Hannewald , P. A. Bobbert

The spinless Falicov-Kimball model exhibits outside the particle-hole symmetric point different stable nonhomogeneous charge orderings. These include the well known charge stripes and a variety of orderings with phase separated domains,…

Strongly Correlated Electrons · Physics 2020-05-07 Rudolf Smorka , Martin Žonda , Michael Thoss

$\beta-Ga_2O_3$ is a promising material candidate for next-generation high power devices even as its low thermal conductivity ($\kappa$) limits utilization due to an inability to sufficiently dissipate heat. Despite its importance, a…

Materials Science · Physics 2024-10-16 Abdulaziz Alkandari , Zherui Han , Ziqi Guo , Thomas Beechem , Xiulin Ruan

We present an ab initio calculation of the DC conductivity of amorphous silicon and hydrogenated amorphous silicon. The Kubo-Greenwood formula is used to obtain the DC conductivity, by thermal averaging over extended dynamical simulation.…

Materials Science · Physics 2009-11-13 T. A. Abtew , M. Zhang , D. A. Drabold

In this work, we use a combination of first-principles calculations under the density functional theory framework and heat transport simulations using the atomistic Green's function (AGF) method to quantitatively predict the contribution of…

Mesoscale and Nanoscale Physics · Physics 2017-03-01 Sridhar Sadasivam , Ning Ye , James Charles , Kai Miao , Joseph P. Feser , Tillmann Kubis , Timothy S. Fisher

Lead halide perovskite semiconductors are soft, polar, materials. The strong driving force for polaron formation (the dielectric electron-phonon coupling) is balanced by the light band effective-masses, leading to a strongly-interacting…

Materials Science · Physics 2017-11-15 Jarvist Moore Frost

We study dynamic nonequilibrium electron charging phenomena in ballistic molecular devices at room temperature that compromise their response to bias and whose nature is evidently distinguishable from static Schottky-type potential…

Mesoscale and Nanoscale Physics · Physics 2008-05-13 Ioannis Deretzis , Antonino La Magna

We review recent results on electronic and thermal transport in two different quasi one-dimensional systems: Silicon nanowires (SiNW) and atomic gold chains. For SiNW's we compute the ballistic electronic and thermal transport properties on…

Mesoscale and Nanoscale Physics · Physics 2015-05-18 A. P. Jauho , M. Engelund , T. Markussen , M. Brandbyge

Thermal properties in the metal/graphene (Gr) systems are analyzed by using an atomistic phonon transport model based on Landauer formalism and first-principles calculations. The specific structures under investigation include chemisorbed…

Mesoscale and Nanoscale Physics · Physics 2015-06-15 R. Mao , B. D. Kong , C. Gong , S. Xu , T. Jayasekera , K. Cho , K. W. Kim

We present a first-principles approach to compute the transport properties of 2D materials in an accurate and automated framework. We use density-functional perturbation theory in the appropriate bidimensional setup with open-boundary…

Materials Science · Physics 2018-12-05 Thibault Sohier , Davide Campi , Nicola Marzari , Marco Gibertini

We study the finite-temperature transport of electrons coupled to anharmonic local phonons. Our focus is on the high-temperature incoherent regime, where controlled calculations are possible both for weak and strong electron--phonon…

Strongly Correlated Electrons · Physics 2021-10-22 Attila Szabó , S. A. Parameswaran , Sarang Gopalakrishnan

Unusual magnetotransport behaviors, such as temperature-dependent negative magnetoresistance (MR) and bowtie-shaped MR, have puzzled us for a long time. Although several mechanisms have been proposed to explain these phenomena, the absence…

Materials Science · Physics 2025-09-23 Zhihao Liu , Shengnan Zhang , Zhong Fang , Hongming Weng , Quansheng Wu
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