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We introduce a novel computational approach for the investigation of complex correlated electron materials which makes it possible to evaluate interatomic forces and thereby determine atomic displacements and structural transformations…

Strongly Correlated Electrons · Physics 2014-04-24 I. Leonov , V. I. Anisimov , D. Vollhardt

Quantum transport in disordered systems is studied using a polaron-based master equation. The polaron approach is capable of bridging the results from the coherent band-like transport regime governed by the Redfield equation to incoherent…

Mesoscale and Nanoscale Physics · Physics 2016-05-11 Chee Kong Lee , Jeremy Moix , Jianshu Cao

In this paper, we review and substantially develop the recently proposed "Microscopic Response Method", which has been devised to compute transport coefficients and especially associated temperature dependence in complex materials. The…

Statistical Mechanics · Physics 2023-07-19 MingLiang Zhang , D. A. Drabold

In polar semiconductors and oxides, the long-range nature of the electron-phonon (\textit{e}-ph) interaction is a bottleneck to compute charge transport from first principles. Here, we develop an efficient ab initio scheme to compute and…

Materials Science · Physics 2016-12-07 Jin-Jian Zhou , Marco Bernardi

A first-principles approach based on Density Functional Theory and Non-Equilibrium Green's functions is used to study the molecular transport system consisting of benzenedithiolate connected with monoatomic gold and platinum electrodes.…

Mesoscale and Nanoscale Physics · Physics 2017-10-10 M. Rumetshofer , G. Dorn , L. Boeri , E. Arrigoni , W. von der Linden

Chromium antimonide has emerged as a key material platform for studying altermagnetism because of its simple binary composition, high N\'eel temperature, and semimetallic electronic structure. Here, we investigate electrical and thermal…

We prove that a diagrammatic evaluation of the Kubo formula for the electronic transport conductivity due the exchange of bosonic excitations, in the usual conserving ladder approximation, yields a result consistent with the Boltzmann…

Statistical Mechanics · Physics 2015-05-13 D. Belitz , T. R. Kirkpatrick

We analyze the quantum transport properties of MAPbI3 within a tight-binding model. Charge carriers are strongly scattered by the Fr\"ohlich interaction with longitudinal optical phonon modes. This limits their mobilities at room…

Ab initio Green-Kubo (aiGK) simulations of heat transport in solids allow for assessing lattice thermal conductivity in anharmonic or complex materials from first principles. In this work, we present a detailed account of their practical…

Materials Science · Physics 2023-06-14 Florian Knoop , Matthias Scheffler , Christian Carbogno

In this review, we survey the current progress in computing transport properties in semimetals which harbour non-Fermi liquid phases. We first discuss the widely-used Kubo formalism, which can be applied to the effective theory describing…

Strongly Correlated Electrons · Physics 2024-08-28 Ipsita Mandal , Hermann Freire

We present a computational method to quantitatively describe the linear-response conductance of nanoscale devices in the Kondo regime. This method relies on a projection scheme to extract an Anderson impurity model from the results of…

Mesoscale and Nanoscale Physics · Physics 2017-04-05 Andrea Droghetti , Ivan Rungger

We present a method to analyze the results of first-principles based calculations of electronic currents including inelastic electron-phonon effects. This method allows us to determine the electronic and vibrational symmeties in play, and…

Mesoscale and Nanoscale Physics · Physics 2008-06-11 Magnus Paulsson , Thomas Frederiksen , Hiromu Ueba , Nicolas Lorente , Mads Brandbyge

We propose a non-perturbative $ab$ $initio$ approach to calculate the electrical conductivity of a liquid metal. Our approach is based on the Kubo formula and the theory of electron-phonon coupling (EPC), and unlike the conventional…

Materials Science · Physics 2022-04-26 Xiao-Wei Zhang , Haoran Chen , En-Ge Wang , Junren Shi , Xin-Zheng Li

BaSnO$_3$ (BSO) is a promising transparent conducting oxide (TCO) with reported room-temperature (RT) Hall mobility exceeding 320 cm$^{2}$V$^{-1}$s$^{-1}$. Among perovskite oxides, it has the highest RT mobility, about 30 times higher than…

We investigate the structural, electronic, vibrational, power and transport properties of the $\beta$ allotrope of Ga$_2$O$_3$ from first-principles. We find phonon frequencies and elastic constants that reproduce the correct band ordering,…

Materials Science · Physics 2020-07-29 Samuel Poncé , Feliciano Giustino

The parameter-free computation of charge transport properties of semiconductors is now routine owing to advances in the ab-initio description of the electron-phonon interaction. Many studies focus on the low-field regime in which the…

Materials Science · Physics 2023-01-18 David Catherall , Austin Minnich

Transport of charge carriers in mechanically soft semiconductors is mainly limited by their interaction with slow intermolecular phonons. Carrier motion exhibits a crossover from superdiffusive to subdiffusive, producing a distinct…

Strongly Correlated Electrons · Physics 2025-07-08 Veljko Janković

In this article we present a novel semi-analytical approach to calculate first-order electron-vibration coupling constants within the framework of density functional theory. It combines analytical expressions for the first-order derivative…

Mesoscale and Nanoscale Physics · Physics 2013-11-12 Marius Bürkle , Janne K. Viljas , Thomas J. Hellmuth , Elke Scheer , Florian Weigend , Gerd Schön , Fabian Pauly

An efficient computational methodology is used to explore charge transport properties in chemically-modified (and randomly disordered) graphene-based materials. The Hamiltonians of various complex forms of graphene are constructed using…

Mesoscale and Nanoscale Physics · Physics 2011-12-16 Nicolas Leconte , Aurélien Lherbier , François Varchon , Pablo Ordejon , Stephan Roche , Jean-Christophe Charlier

Predicting the electrical properties of organic molecular crystals (OMCs) is challenging due to their complex crystal structures and electron-phonon (e-ph) interactions. Charge transport in OMCs is conventionally categorized into two…

Materials Science · Physics 2022-04-22 Benjamin K. Chang , Jin-Jian Zhou , Nien-En Lee , Marco Bernardi