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The interplay between spin-orbit coupling, anisotropic magnetic interaction, frustration-induced quantum fluctuations and spin correlations can lead to novel quantum states with exotic excitations in rare-earth-based quantum magnets.…

Strongly Correlated Electrons · Physics 2023-08-31 J. Khatua , Q. P. Ding , M. S. Ramachandra Rao , K. Y. Choi , A. Zorko , Y. Furukawa , P. Khuntia

We report the results of ac and dc magnetization (M) and heat-capacity (C) measurements on the solid solution, Sr$_3$Cu$_{1-x}$Zn$_x$IrO$_6$. While the Zn end member is known to form in a rhombohedral pseudo one-dimensional K$_4$CdCl$_6$…

Strongly Correlated Electrons · Physics 2009-11-07 Asad Niazi , E. V. Sampathkumaran , P. L. Paulose , D. Eckert , A. Handstein , K. -H. Müller

We have synthesized single crystals of Na_2IrO_3 and studied their structure, transport, magnetic, and thermal properties using powder x-ray diffraction (PXRD), electrical resistivity, isothermal magnetization M versus magnetic field H,…

Strongly Correlated Electrons · Physics 2010-06-03 Yogesh Singh , P. Gegenwart

Spin-phonon coupling originated from spin-lattice correlation depends upon different exchange interactions in transition metal oxides containing 3d magnetic ions. Spin-lattice coupling can influence the coupling mechanism in magnetoelectric…

Strongly Correlated Electrons · Physics 2021-09-09 P. Pal , Shalini Badola , P. K. Biswas , Ranjana R. Das , Surajit Saha , S. D. Kaushik , P. N. Vishwakarma , A. K. Singh

We report proximate quantum spin liquid behavior in K$_2$Co$_2$(SO$_4$)$_3$ with the magnetic Co$^{2+}$ ions embedded on a highly frustrated three-dimensional double trillium lattice. Single-crystal and high-resolution synchrotron powder…

We report the results of low-temperature magnetization and specific heat measurements of Sr$_3$CoTa$_2$O$_9$ powder, in which Co$^{2+}$ ions with effective spin-1/2 form a uniform triangular lattice in the $ab$ plane. It was found that…

Strongly Correlated Electrons · Physics 2023-05-24 Iori Nishizawa , Nobuyuki Kurita , Hidekazu Tanaka , Takayuki Goto

The spin dynamics of the ferromagnetic Kondo lattice CeRuPO is investigated by Electron Spin Resonance (ESR) at microwave frequencies of 1, 9.4, and 34~GHz. The measured resonance can be ascribed to a rarely observed bulk Ce3+ resonance in…

Strongly Correlated Electrons · Physics 2010-10-13 T. Förster , J. Sichelschmidt , C. Krellner , C. Geibel , F. Steglich

In this paper we present the microscopic origin of the ferromagnetism of Fe0.25TaS2 and its finite-temperature magnetic properties. We first obtain the band structures of Fe0.25TaS2 by the first-principles calculations and find that both…

Materials Science · Physics 2022-03-10 Jin-Hua Wang , Ya-Min Quan , Da-Yong Liu , Liang-Jian Zou

The crystallographic, magnetic, and transport properties of the van der Waals bonded, layered compound CrTe3 have been investigated on single crystal and polycrystalline materials. The crystal structure contains layers made up of lozenge…

Strongly Correlated Electrons · Physics 2017-04-19 Michael A. McGuire , V. Ovidiu Garlea , Santosh KC , Valentino R. Cooper , Jiaqiang Yan , Huibo Cao , Brian C. Sales

Dimerized magnets forming alternating Heisenberg chains exhibit quantum coherence and entanglement and thus can find potential applications in quantum information and computation. However, magnetic systems typically undergo thermal…

The complex magnetism and transport properties of tetragonal Ce$_3$Cu$_4$As$_4$O$_2$ were examined through neutron scattering and physical properties measurements on polycrystalline samples. The lamellar structure consists of alternating…

Strongly Correlated Electrons · Physics 2016-09-07 Jiakui K. Wang , Shan Wu , Yiming Qiu , Jose A. Rodriguez-Rivera , Qingzhen Huang , C. Broholm , E. Morosan

The two-dimensional triangular-lattice antiferromagnet (TLAF) is a textbook example of frustrated magnetic systems. Despite its simplicity, the TLAF model exhibits a highly rich and complex magnetic phase diagram, featuring numerous…

The layered compound Fe3GaTe2 is attracting attention due to its high Curie temperature, low dimensionality, and the presence of topological spin textures above room temperature, making Fe$_3$GaTe$_2$ a good candidate for applications in…

We present the temperature dependence of the uniform susceptibility of spin-half quantum antiferromagnets on spatially anisotropic triangular-lattices, using high temperature series expansions. We consider a model with two exchange…

Strongly Correlated Electrons · Physics 2009-11-10 Weihong Zheng , Rajiv R. P. Singh , Ross H. McKenzie , Radu Coldea

The spin-orbit assisted Mott insulator $\alpha$-RuCl3 is proximate to the coveted quantum spin liquid (QSL) predicted by the Kitaev model. In the search for the pure Kitaev QSL, reducing the dimensionality of this frustrated magnet by…

We report here the observation of robust thermoremanent magnetization (TRM) in Fe-intercalated TaS$_2$ single crystal Fe$_{x}$TaS$_2$, which develops upon cooling under a moderate magnetic field of 500 Oe or higher. The thermoremanence is…

Geometrically frustrated magnetic systems, such as those based on the Shastry-Sutherland lattice (SSL), offer a rich playground for exploring unconventional magnetic states. The delicate balance between competing interactions in these…

Precision measurements of the magnetization and ac susceptibility of Cu$_2$0SeO$_3$ are reported for magnetic fields along different crystallographic directions, focussing on the border between the conical and the field-polarized state for…

Strongly Correlated Electrons · Physics 2021-04-01 M. Halder , A. Chacon , A. Bauer , W. Simeth , S. Mühlbauer , H. Berger , L. Heinen , M. Garst , A. Rosch , C. Pfleiderer

The discovery of new magnetic ground states in geometrically frustrated lattices remains a central challenge in materials science. Here, we report the synthesis, structural characterization, and frustrated magnetic properties of…

Strongly Correlated Electrons · Physics 2026-01-15 Matt Boswell , Mingyu Xu , Haozhe Wang , Mouyang Cheng , N. Li , X. F. Sun , Haidong Zhou , Huibo Cao , Mingda Li , Weiwei Xie

Kitaev-type interactions between neighbouring magnetic moments emerge in the honeycomb material ${\alpha}$-RuCl3. It is debated however whether these Kitaev interactions are ferromagnetic or antiferromagnetic. With electron energy loss…

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