We report the results of low-temperature magnetization and specific heat measurements of Sr3CoTa2O9 powder, in which Co2+ ions with effective spin-1/2 form a uniform triangular lattice in the ab plane. It was found that Sr3CoTa2O9 undergoes successive antiferromagnetic transitions at TN1=0.97K and TN2=0.79K at zero magnetic field. As the magnetic field increases, both TN1 and TN2 decrease monotonically. The obtained magnetic field vs temperature phase diagram together with a sharp magnetization anomaly at a saturation field of μ0Hs=2.3T indicates that Sr3CoTa2O9 is described as a spin-1/2 three-dimensional triangular-lattice antiferromagnet with a weak easy-axis anisotropy. We discuss the characteristics of the magnetic phase diagram, which approximates the phase diagram for the magnetic field perpendicular to the c axis.
@article{arxiv.2304.14693,
title = {Magnetic phase diagram in three-dimensional triangular-lattice antiferromagnet Sr$_3$CoTa$_2$O$_9$ with small easy-axis anisotropy},
author = {Iori Nishizawa and Nobuyuki Kurita and Hidekazu Tanaka and Takayuki Goto},
journal= {arXiv preprint arXiv:2304.14693},
year = {2023}
}
Comments
12 pages, 11 figures, accepted for publication in Phys. Rev. B