English

Magnetic phase diagram in three-dimensional triangular-lattice antiferromagnet Sr$_3$CoTa$_2$O$_9$ with small easy-axis anisotropy

Strongly Correlated Electrons 2023-05-24 v1

Abstract

We report the results of low-temperature magnetization and specific heat measurements of Sr3_3CoTa2_2O9_9 powder, in which Co2+^{2+} ions with effective spin-1/2 form a uniform triangular lattice in the abab plane. It was found that Sr3_3CoTa2_2O9_9 undergoes successive antiferromagnetic transitions at TN1=0.97 KT_{\rm N1}\,{=}\,0.97~{\rm K} and TN2=0.79 KT_{\rm N2}\,{=}\,0.79~{\rm K} at zero magnetic field. As the magnetic field increases, both TN1T_{\rm N1} and TN2T_{\rm N2} decrease monotonically. The obtained magnetic field vs temperature phase diagram together with a sharp magnetization anomaly at a saturation field of μ0Hs=2.3 T{\mu_0}H_{\rm s}\,{=}\,2.3~{\rm T} indicates that Sr3_3CoTa2_2O9_9 is described as a spin-1/2 three-dimensional triangular-lattice antiferromagnet with a weak easy-axis anisotropy. We discuss the characteristics of the magnetic phase diagram, which approximates the phase diagram for the magnetic field perpendicular to the cc axis.

Keywords

Cite

@article{arxiv.2304.14693,
  title  = {Magnetic phase diagram in three-dimensional triangular-lattice antiferromagnet Sr$_3$CoTa$_2$O$_9$ with small easy-axis anisotropy},
  author = {Iori Nishizawa and Nobuyuki Kurita and Hidekazu Tanaka and Takayuki Goto},
  journal= {arXiv preprint arXiv:2304.14693},
  year   = {2023}
}

Comments

12 pages, 11 figures, accepted for publication in Phys. Rev. B