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In this work, the effects of finite size on the determination of the three-phase coexistence temperature ($T_3$) of carbon dioxide (CO$_2$) hydrate have been studied by molecular dynamic simulations and using the direct coexistence…

Soft Condensed Matter · Physics 2024-08-06 J. Algaba , S. Blazquez , E. Feria , J. M. Míguez , M. M. Conde , F. J. Blas

In this work, the effect of the range of the dispersive interactions in the determination of the three-phase coexistence line of the CO$_2$ and CH$_4$ hydrates has been studied. In particular, the temperature ($T_3$) at which solid hydrate,…

Soft Condensed Matter · Physics 2024-08-06 J. Algaba , S. Blazquez , J. M. Míguez , M. M. Conde , F. J. Blas

Molecular dynamics simulations have been performed to determine the three-phase coexistence temperature for a methane hydrate system in equilibrium with a NaCl solution and a methane gas phase. The direct coexistence technique is used…

Chemical Physics · Physics 2024-01-29 S. Blazquez , C. Vega , M. M. Conde

Molecular dynamics simulations are performed for a supercooled simple liquid with changing the system size from N=108 to $10^4$ to examine possible finite-size effects. Although almost no systematic deviation is detected in the static pair…

Soft Condensed Matter · Physics 2007-05-23 Kang Kim , Ryoichi Yamamoto

Methane clathrate hydrates, particularly those with an sI structure, are significant due to their potential as energy resources and their impact on gas pipelines. In this study, a two-dimensional (2D) lattice-gas model is employed to…

Disordered Systems and Neural Networks · Physics 2025-02-10 Julian Juan , Maria E. Pronsato , Antonio J. Ramirez-Pastor , Pablo Longone

We investigate the three-phase coexistence line of ethane (C$_2$H$_6$) hydrate through molecular dynamics simulations using the direct coexistence approach. In this framework, C$_2$H$_6$ sI hydrate, aqueous, and pure guest phases are…

Soft Condensed Matter · Physics 2025-11-12 Paula Gómez-Álvarez , Miguel J. Torrejón , Jesús Algaba , Felipe J. Blas

We study zero-range processes which are known to exhibit a condensation transition, where above a critical density a non-zero fraction of all particles accumulates on a single lattice site. This phenomenon has been a subject of recent…

Statistical Mechanics · Physics 2015-03-14 Paul Chleboun , Stefan Grosskinsky

We present the first analytic study of finite-size effects on critical diffusion above and below T_c of three-dimensional Ising-like systems whose order parameter is coupled to a conserved density. We also calculate the finite-size…

Statistical Mechanics · Physics 2009-10-31 Wolfgang Koch , Volker Dohm

We present a comprehensive theoretical study of finite size effects in the relaxation dynamics of glass-forming liquids. Our analysis is motivated by recent theoretical progress regarding the understanding of relevant correlation length…

Statistical Mechanics · Physics 2012-09-12 Ludovic Berthier , Giulio Biroli , Daniele Coslovich , Walter Kob , Cristina Toninelli

Water shows intriguing thermodynamic and dynamic anomalies in the supercooled liquid state. One possible explanation of the origin of these anomalies lies in the existence of a metastable liquid-liquid phase transition (LLPT) between two…

Statistical Mechanics · Physics 2016-05-04 Rakesh S. Singh , John W. Biddle , Pablo G. Debenedetti , Mikhail A. Anisimov

Gas hydrates are crystalline compounds formed when water molecules encapsulate guest gas molecules under high pressure and low temperatures. They have gained significant interest due to their potential as alternative energy resources and…

Chemical Physics · Physics 2025-11-14 Ramkhelavan Kanaujiya , Atanu K. Metya , Rajnish Kumar , Tarak K Patra

The effects of a finite temperature on the equilibrium structures of hydrocarbon molecules are computationally explored as a function of size and relative chemical composition in hydrogen and carbon. Using parallel tempering Monte Carlo…

Chemical Physics · Physics 2022-10-14 Ariel Francis Perez-Mellor , Pascal Parneix , Florent Calvo , Cyril Falvo

Recently gigantic peaks in thermodynamic response functions have been observed at finite temperature for one-dimensional models with short-range coupling, closely resembling a second-order phase transition. Thus, we will analyze the finite…

Statistical Mechanics · Physics 2021-02-24 Onofre Rojas

In this work, the univariant two-phase coexistence line of the hydrate of tetrahydrofuran (THF) is determined from 100 to 1000 bar by molecular dynamics simulations. The study is carried out by putting in contact a THF hydrate phase with a…

Soft Condensed Matter · Physics 2024-05-09 Jesús Algaba , Cristóbal Romero-Guzmán , Miguel J. Torrejón , F. J. Blas

The thermodynamical cluster model is known to present a first-order liquid-gas phase transition in the idealized case of an uncharged, infinitely extended medium. However, in most practical applications of this model, the system is finite…

Nuclear Theory · Physics 2016-04-13 S. Mallik , F. Gulminelli , G. Chaudhuri

We investigate by means of Monte Carlo simulations the fully connected p-state Potts model for different system sizes in order to see how the static and dynamic properties of a finite model compare with the, exactly known, behavior of the…

Statistical Mechanics · Physics 2009-11-07 Claudio Brangian , Walter Kob , Kurt Binder

We present a finite-size scaling analysis of the droplet condensation-evaporation transition of a lattice gas (in two and three dimensions) and a Lennard-Jones gas (in three dimensions) at fixed density. Parallel multicanonical simulations…

Soft Condensed Matter · Physics 2015-08-04 Johannes Zierenberg , Wolfhard Janke

The effects of (in)homogeneity and size on the phase diagram of Lennard-Jones fluids are investigated. It is shown that standard multifragmentation scenarios (finite equilibrated systems with conserved center of mass position and momentum)…

Nuclear Theory · Physics 2009-11-10 Al. H. Raduta , Ad. R. Raduta

Finite-size effects in systems with diverging characteristic lengthscale have been addressed via state-of-the-art Monte Carlo and molecular dynamics simulations of various models exhibiting solid-solid, liquid-liquid and vapor-liquid…

Statistical Mechanics · Physics 2018-03-09 Subir K. Das , Sutapa Roy , Suman Majumder , Shaista Ahmad

The isothermal compressibility (i.e., the asymptotic number variance) of equilibrium liquid water as a function of temperature is minimal near ambient conditions. This anomalous non-monotonic temperature dependence is due to a balance…

Statistical Mechanics · Physics 2024-05-06 Michael A. Klatt , Jaeuk Kim , Thomas E. Gartner , Salvatore Torquato
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