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A comprehensive study of the structural properties of the heavily investigated rare-earth A2Ir2O7 series under extreme conditions is presented. The series is covered by studying iridates with A = Pr, Sm, Dy-Lu. Temperature- and…

We report the low temperature properties of a new series of pyrochlore iridates R2Ir2O7 (R = rare-earth elements). We found that the compounds with R = Pr, Sm, Nd, and Eu exhibit metallic conductivity, whereas those with smaller rare-earth…

Strongly Correlated Electrons · Physics 2009-11-07 D. Yanagishima , Y. Maeno

Rare-earth pyrochlore iridates host two interlocking magnetic sublattices of corner-sharing tetrahedra and can harbour a unique combination of frustrated moments, exotic excitations and highly correlated electrons. They are also the first…

Reliable and profound studies of actual magnetic domain structure in rare-earth A2Ir2O7 pyrochlore iridates are frequently limited by insufficient sample quality or lack of single crystals. We report the magnetic properties of the…

Pyrochlore iridates A2Ir2O7 (A = rare earth elements, Y or Bi) hold great promise for realizing novel electronic and magnetic states owing to the interplay of spin-orbit coupling, electron correlation and geometrical frustration. A…

Strongly Correlated Electrons · Physics 2017-10-04 W. C. Yang , W. K. Zhu , H. D. Zhou , L. Ling , E. S. Choi , M. Lee , Y. Losovyj , Chi-Ken Lu , S. X. Zhang

The interplay of spin-orbit interactions and electronic correlations dominates the physical properties of pyrochlore iridates, R2Ir2O7 (R = Y, rare earth element), which are typically magnetic insulators. We report an…

Strongly Correlated Electrons · Physics 2015-06-03 T. F. Qi , O. B. Korneta , Xiangang Wan , L. E. DeLong , P. Schlottmann , G. Cao

The magnetic behavior of polycrystalline samples of Er$_2$Ir$_2$O$_7$ and Tb$_2$Ir$_2$O$_7$ pyrochlores is studied by magnetization measurements and neutron diffraction. Both compounds undergo a magnetic transition at 140 and 130 K…

Strongly Correlated Electrons · Physics 2015-07-30 E. Lefrançois , V. Simonet , R. Ballou , E. Lhotel , A. Hadj-Azzem , S. Kodjikian , P. Lejay , P. Manuel , D. Khalyavin , L. C. Chapon

We address the concomitant metal-insulator transition (MIT) and antiferromagnetic ordering in the novel pyrochlore iridate Eu2Ir2O7 by combining x-ray absorption spectroscopy, x-ray and neutron diffractions and density functional theory…

Metal-insulator transitions in pyrochlore iridates (A2Ir2O7) are believed to occur due to subtle interplay of spin-orbit coupling, geometric frustration, and electron interactions. In particular, the nature of magnetic ordering of iridium…

Strongly Correlated Electrons · Physics 2014-07-29 Eric Kin-Ho Lee , Subhro Bhattacharjee , Yong Baek Kim

Muon spin rotation and relaxation experiments in the pyrochlore iridate Eu2Ir2O7 yield a well-defined muon spin precession frequency below the metal-insulator/antiferromagnetic transition temperature TM = 120 K, indicative of long-range…

Strongly Correlated Electrons · Physics 2015-03-19 Songrui Zhao. J. M. Mackie , D. E. MacLaughlin , O. O. Bernal , J. J. Ishikawa , Y. Ohta , S. Nakatsuji

Tuning of spin-orbit coupling and electron correlation effects in pyrochlore iridates is considered for many interesting phenomena. We have investigated the temperature evolution of structural, magnetic and electronic properties in doped…

Strongly Correlated Electrons · Physics 2019-05-07 Harish Kumar , A. K. Pramanik

The $f$-$d$ magnetic exchange interaction is considered to be a key ingredient for many exotic topological phases in pyrochlore iridates. Here, we have investigated the evolution of structural, magnetic and electronic properties in doped…

Strongly Correlated Electrons · Physics 2020-02-07 Harish Kumar , K. C. Kharkwal , Kranti Kumar , K. Asokan , A. Banerjee , A. K. Pramanik

Our single crystal study of the magneto-thermal and transport properties of the pyrochlore iridate Eu2Ir2O7 reveals a continuous phase transition from a paramagnetic metal to an antiferromagnetic insulator for a sample with stoichiometry…

Strongly Correlated Electrons · Physics 2015-06-04 Jun J. Ishikawa , Eoin C. T. O'Farrell , Satoru Nakatsuji

The pyrochlore iridates, A$_2$Ir$_2$O$_7$, show a wide variety of structural, electronic, and magnetic properties controlled by the interplay of different exchange interactions, which can be tuned by external pressure. In this work, we…

Materials Science · Physics 2024-05-14 M Rosalin , K. A. Irshad , Boby Joseph , Prachi Telang , Surjeet Singh , D. V. S. Muthu , A. K. Sood , .

Fully relativistic first-principles electronic structure calculations based on a noncollinear local spin density approximation (LSDA) are performed for pyrochlore iridates Y$_2$Ir$_2$O$_7$ and Pr$_2$Ir$_2$O$_7$. The all-in, all-out…

Strongly Correlated Electrons · Physics 2015-06-22 Fumiyuki Ishii , Yo Pierre Mizuta , Takehiro Kato , Taisuke Ozaki , Hongming Weng , Shigeki Onoda

Building a full understanding of the complex magnetism in the rare-earth pyrochlore iridates, A2Ir2O7, is an ongoing issue in condensed matter physics. The possibility of two interpenetrating and interacting frustrated magnetic pyrochlore…

Strongly Correlated Electrons · Physics 2021-01-01 Ross H. Colman , Kristina Vlaskova , Adam Berlie , Milan Klicpera

Transition metal oxides of the $4d$ and $5d$ block have recently become the targets of materials discovery, largely due to their strong spin-orbit coupling that can generate exotic magnetic and electronic states. Here we report the high…

The interplay between spin-orbit coupling (SOC) and electron correlation ($U$) is considered for many exotic phenomena in iridium oxides. We have investigated the evolution of structural, magnetic and electronic properties in pyrochlore…

Strongly Correlated Electrons · Physics 2017-03-08 Harish Kumar , R. S. Dhaka , A. K. Pramanik

We report a combined muon spin relaxation/rotation, bulk magnetization, neutron scattering, and transport study of the electronic properties of the pyrochlore iridate Nd2Ir2O7. We observe the onset of strongly hysteretic behavior in the…

The synergy of strong spin-orbit coupling and electron-electron interactions gives rise to unconventional topological states, such as topological Mott insulator, Weyl semimetal, and quantum spin liquid. In this study, we have grown single…

Strongly Correlated Electrons · Physics 2024-07-18 Harish Kumar , M. Köpf , P. Telang , N. Bura , A. Jesche , P. Gegenwart , C. A. Kuntscher
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