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Using density functional theory and LDA+U method, we investigate magnetic and electronic structure of Y$_{2}$Ir$_{2}$O$_{7}$ and rare-earth based pyrochlore iridates. Our study reveals that the ground state is a non-collinear magnetic…

Materials Science · Physics 2010-03-18 Xiangang Wan , Jinming Dong , Sergey Y. Savrasov

The electrical resistivity, magnetic susceptibility, and heat capacity of sintered samples of Ca2Ir2O7, in which pentavalent Ir atoms with 5d4 electron configuration form a pyrochlore structure, have been studied. The obtained experimental…

Strongly Correlated Electrons · Physics 2022-11-18 Yuki Nakayama , Yoshihiko Okamoto , Daigorou Hirai , Koshi Takenaka

Semimetallic osmium pyrochlore oxide Cd2Os2O7 undergoes a magnetic transition to an all-in-all-out (AIAO)-type order at 227 K, followed by a crossover to an AIAO insulator at around 210 K. Here, we studied the isostructural and…

Strongly Correlated Electrons · Physics 2022-02-09 Kota Kataoka , Daigorou Hirai , Akihiro Koda , Ryosuke Kadono , Takashi Honda , Zenji Hiroi

The pyrochlore Eu$_2$Ir$_2$O$_7$ has recently attracted significant attention as a candidate Weyl semimetal. The previous reports on this compound unanimously show a thermally induced metal to insulator (MI) transition, concomitant with…

Strongly Correlated Electrons · Physics 2018-06-27 Prachi Telang , Kshiti Mishra , A. K. Sood , Surjeet Singh

We report low-temperature susceptibility and magnetisation data for the cubic pyrochlore Er2Ti2O7. By performing the measurements on single crystals we are able to establish the degree of magnetic anisotropy present in this compound and to…

Strongly Correlated Electrons · Physics 2013-10-08 O. A. Petrenko , M. R. Lees , G. Balakrishnan

Neutron powder diffraction and inelastic measurements were performed examining the 5d pyrochlore Y$_2$Ir$_2$O$_7$. Temperature dependent measurements were performed between 3.4 K and 290 K, spanning the magnetic transition at 155 K. No sign…

Strongly Correlated Electrons · Physics 2014-05-30 M. C. Shapiro , S. C. Riggs , M. B. Stone , C. R. de la Cruz , S. Chi , A. A. Podlesnyak , I. R. Fisher

The possible existence of topological insulators in cubic pyrochlore iridates A$_{2}$Ir$_{2}$O$_{7}$ (A = Y or rare-earth elements) is investigated by taking into account the strong spin-orbit coupling and trigonal crystal field effect. It…

Strongly Correlated Electrons · Physics 2015-03-14 Bohm-Jung Yang , Yong Baek Kim

Several rare earth magnetic pyrochlore materials are well modeled by a spin-1/2 quantum Hamiltonian with anisotropic exchange parameters Js. For the Er2Ti2O7 material, the Js were recently determined from high-field inelastic neutron…

Strongly Correlated Electrons · Physics 2014-04-11 J. Oitmaa , R. R. P. Singh , A. G. R. Day , B. V. Bagheri , M. J. P. Gingras

The very low temperature properties of two pyrochlore compounds, Yb2Ti2O7 and Gd2Sn2O7, were investigated using an ensemble of microscopic and bulk techniques. In both compounds, a first order transition is evidenced, as well as spin…

We present results from muon spin relaxation/rotation, magnetization, neutron scattering and transport measurements on polycrystalline samples of the pyrochlore iridates Y2Ir2O7 (Y-227) and Yb2Ir2O7 (Yb-227). Well-defined spontaneous…

Strongly Correlated Electrons · Physics 2012-08-08 S. M. Disseler , Chetan Dhital , A. Amato , S. R. Giblin , Clarina de la Cruz , Stephen D. Wilson , M. J. Graf

We have studied the effect of pressure on the pyrochlore iridate Eu$_2$Ir$_2$O$_7$, which at ambient pressure has a thermally driven insulator to metal transition at $T_{MI}\sim120$\,K. As a function of pressure the insulating gap closes,…

Strongly Correlated Electrons · Physics 2012-05-16 F. F. Tafti , J. J. Ishikawa , A. McCollam , S. Nakatsuji , S. R. Julian

The crystal lattice of Sr$_2$IrO$_4$ is investigated with synchrotron X-ray powder diffraction under hydrostatic pressures up to $P=43$ GPa and temperatures down to $20$ K. The tetragonal unit cell is maintained over the whole investigated…

Strongly Correlated Electrons · Physics 2020-02-26 K. Samanta , R. Tartaglia , U. F. Kaneko , N. M. Souza-Neto , E. Granado

Using 170-Yb and 155-Gd Mossbauer measurements down to 0.03K, we have examined the semiconducting pyrochlore Yb2Mo2O7 where the Mo intra-sublattice interaction is anti-ferromagnetic and the metallic pyrochlore Gd2Mo2O7 where this…

Condensed Matter · Physics 2009-11-10 J. A. Hodges , P. Bonville , A. Forget , J. P. Sanchez , P. Vulliet , M. Rams , K. Krolas

We report on the evolution of the thermal metal-insulator transition in polycrystalline samples of Nd$_2$Ir$_2$O$_7$ upon hole-doping via substitution of Ca$^{2+}$ for Nd$^{3+}$. Ca substitution mediates a filling-controlled Mott-like…

Non-Fermi liquid behavior in some fermionic systems have attracted significant interest in last few decades. Certain pyrochlore iridates with stronger spin-orbit coupling strength have recently been added to the list. Here, we provide…

Strongly Correlated Electrons · Physics 2022-01-03 Md Salman Khan , Ilaria Carlomagno , Carlo Meneghini , P. K. Biswas , Fabrice Bert , Subham Majumdar , Sugata Ray

The frustrated pyrochlore iridate Pr$_2$Ir$_2$O$_7$ was proposed as a metallic quantum spin liquid located at a zero-field quantum critical point. Here we present the ultralow-temperature thermal conductivity measurements on the…

Strongly Correlated Electrons · Physics 2022-08-23 J. M. Ni , Y. Y. Huang , E. J. Cheng , Y. J. Yu , B. L. Pan , Q. Li , L. M. Xu , Z. M. Tian , S. Y. Li

R2In (R = rare earth) intermetallics exhibit unusual magnetic and magnetocaloric properties, driven by subtle electronic effects, lattice distortions, and spin-lattice coupling. Most of these binary compounds adopt the hexagonal Ni2In-type…

Materials Science · Physics 2025-12-18 Anis Biswas , Ajay Kumar , Prashant Singh , Yaroslav Mudryk

We have synthesized two iron-pnictide/chalcogenide materials, CuFeTe2 and Fe2As, which share crystallographic features with known iron-based superconductors, and carried out high-pressure electrical resistivity measurements on these…

We report neutron diffraction measurements of the magnetic structures in two pyrochlore iridates, Yb2Ir2O7 and Lu2Ir2O7. Both samples exhibit the all-in-all-out magnetic structure on the Ir4+ sites below TN~ 150,K, with a low temperature…

Magnetic-rare-earth pyrochlore iridates exhibit a rich variety of unconventional phases, driven by the complex interactions within and between the rare-earth and the iridium sublattices. In this study, we investigate the peculiar magnetic…

Strongly Correlated Electrons · Physics 2026-01-05 Y. Alexanian , E. Lhotel , J. Robert , S. Petit , E. Lefrançois , P. Lejay , A. Hadj-Azzem , F. Damay , J. Ollivier , B. Fåk , R. Ballou , S. De Brion , V. Simonet