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Related papers: Displacive Jahn--Teller transition in NaNiO$_2$

200 papers

The Jahn-Teller effect is a fascinating and ubiquitous phenomenon in modern quantum physics and chemistry. We propose a class of oxides with melilite structure Ba$_2$TGe$_2$O$_7$ (T=V,Ni) where Jahn-Teller distortions are the main…

Materials Science · Physics 2015-08-03 Paolo Barone , Kunihiko Yamauchi , Silvia Picozzi

The atomic pair distribution function (PDF) of stoichiometric LaMnO_3 has been measured. This has been fit with a structural model to extract the local Jahn-Teller distortion for an ideal Mn(3+)O_6 octahedron. These results are compared to…

Materials Science · Physics 2009-10-31 Th. Proffen , R. G. DiFrancesco , S. J. L. Billinge , E. L. Brosha , G. H. Kwei

Charge-state transitions of a single Cu-phthalocyanine molecule adsorbed on an insulating layer of NaCl on Cu(111) are probed by means of alternate charging scanning tunneling microscopy. Real-space imaging of the electronic transitions…

High-pressure optical-absorption measurements performed in CuWO4 up to 20 GPa provide experimental evidence of the persistence of the Jahn-Teller (JT) distortion in the whole pressure range both in the low-pressure triclinic and in the…

Materials Science · Physics 2012-04-20 J. Ruiz-Fuertes , A. Segura , F. Rodriguez , D. Errandonea , M. N. Sanz-Ortiz

We report a comprehensive study of dc susceptibility, specific heat, neutron diffraction, and inelastic neutron scattering measurements on polycrystalline Ba3(Cr1-xVx)2O8 samples, where x=0, 0.06, 0.15, and 0.53. A Jahn-Teller structure…

Materials Science · Physics 2013-05-02 Tao Hong , L. Y. Zhu , X. Ke , V. O. Garlea , Y. Qiu , Y. Nambu , H. Yoshizawa , M. Zhu , G. E. Granroth , A. T. Savici , Zheng Gai , H. D. Zhou

It is demonstrated that under common conditions a molecular solid subject to Jahn-Teller interactions supports stable Q-ball-like non-topological solitons. Such solitons represent a localized lump of excess electric charge in periodic…

Materials Science · Physics 2007-05-23 Dennis P. Clougherty

A C$_3$-symmetric crystal-field potential in the Fe(II)Fe(III) bimetallic oxalates splits the L=2 Fe(II) multiplet into two doublets and a singlet. In compounds that exhibit magnetic compensation, one of the doublets was predicted to lie…

Other Condensed Matter · Physics 2009-11-13 Randy S. Fishman , Satoshi Okamoto , Fernando A. Reboredo

The local and intermediate structure of stoichiometric LaMnO$_3$ has been studied in the pseudocubic and rhombohedral phases at high temperatures (300 to 1150 K). Neutron powder diffraction data were collected and a combined Rietveld and…

Strongly Correlated Electrons · Physics 2009-11-10 Xiangyun Qiu , Th. Proffen , J. F. Mitchell , S. J. L. Billinge

In LiNiO$_2$ Ni$^{3+}$ ion has $d^7$ configuration in cubic crystal field with one electron on double degenerate $e_g$ orbitals, and such ion is considered to be Jahn-Teller (JT) active. However despite the fact, that this compound is an…

Strongly Correlated Electrons · Physics 2019-01-09 Dm. M. Korotin , D. Novoselov , V. I. Anisimov

We observe two consecutive transitions in La1-xCaxMnO3, x=0.19: ferromagnetic ordering at Tc = 177 K and Jahn-Teller orbital ordering at T_JT = 150 K. The presence of a ferromagnetic insulating state below T_JT shows that the metallic phase…

Strongly Correlated Electrons · Physics 2007-05-23 Bas B. van Aken , Auke Meetsma , Thomas T. M. Palstra

We have studied the temperature dependence of crystal and magnetic structures of the Jahn-Teller distorted transition metal difluorides CrF$_2$ and CuF$_2$ by neutron powder diffraction in the temperature range 2-280 K. The lattice…

Strongly Correlated Electrons · Physics 2012-07-03 Tapan Chatterji , Thomas C. Hansen

The electronic structure and magnetism in the sodium nickelate NaNiO_2 in the low-temperature phase is studied from density-functional calculations using the linear muffin-tin orbitals method. An antiferromagnetic solution with a magnetic…

Strongly Correlated Electrons · Physics 2009-11-10 H. Meskine , S. Satpathy

A synchrotron x-ray diffraction study of the crystallographic structure of PrO2 in the Jahn-Teller distorted phase is reported. The distortion of the oxygen sublattice, which was previously ambiguous, is shown to be a chiral structure in…

Strongly Correlated Electrons · Physics 2009-11-13 C. H. Webster , L. M. Helme , A. T. Boothroyd , D. F. McMorrow , S. B. Wilkins , C. Detlefs , B. Detlefs , R. I. Bewley , M. J. McKelvy

We studied in detail the structural relaxation and Jahn-Teller distortion in LaMnO3 (001) surface of the orthorhombic phase by means of classical atomistic simulation. It is found that MnO2-terminated surface is more energetically favorable…

Materials Science · Physics 2009-04-24 F. L. Tang , M. Huang , W. J. Lu , W. Y. Yu

The nature of the cooperative Jahn-Teller (JT) transition accompanied by orbital order-disorder in Nd1-xCaxMnO3 has been studied by high temperature (300 - 1200K) synchrotron and laboratory X-ray powder diffraction in the low doping region…

Materials Science · Physics 2009-11-13 C. V. Colin , A. J. C. Buurma , M. v. Zimmermann , T. T. M. Palstra

Distortions of the oxygen sublattice couple to $e_g$ orbitals of Mn$^{3+}$ and drive a cooperative Jahn-Teller (orbital ordering) transition in LaMnO$_3$. A simple model for this transition is studied. Without further adjustment, the model…

Strongly Correlated Electrons · Physics 2009-10-31 Philip B. Allen , Vasili Perebeinos

The Jahn-Teller effect in the charge-ordered (CO) state for La1-xCaxMnO3 (0.5<x<0.87) was studied by measuring the low-temperature powder x-ray diffraction, internal friction, and shear modulus. We find that the electron-lattice interaction…

Strongly Correlated Electrons · Physics 2009-11-07 R. K. Zheng , R. X. Huang , A. N. Tang , G. Li , X. G. Li , J. N. Wei , J. P. Shui , Z. Yao

Exotic quantum phases, arising from a complex interplay of charge, spin, lattice and orbital degrees of freedom, are of immense interest to a wide research community. A well-known example of such an entangled behavior is the Jahn-Teller…

Using high resolution X-Ray diffraction (XRD) on high purity powders, we resolved the structure and $ab$ symmetry of the intriguing compound \svo$ $ from room temperature down to 20 K to an unprecedented level of accuracy. Upon cooling,…

Strongly Correlated Electrons · Physics 2016-03-31 J. Teyssier , E. Giannini , A. Stucky , R. Cerný , M. V. Eremin , D. van der Marel

The crystal and magnetic structure of LaTiO3 ~ has been studied by x-ray and neutron diffraction techniques using nearly stoichiometric samples. We find a strong structural anomaly near the antiferromagnetic ordering, T$_N$=146 K. In…

Strongly Correlated Electrons · Physics 2009-11-10 M. Cwik , T. Lorenz , J. Baier , R. Mueller , G. Andre , F. Bouree , F. Lichtenberg , A. Freimuth , E. Mueller-Hartmann , M. Braden