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We develop a generic method in Liouville space to describe the dissipative dynamics of coherent interacting quantum dots with adiabatic time dependence beyond linear response. We show how the adiabatic response can be related to effective…

Mesoscale and Nanoscale Physics · Physics 2012-07-25 Oleksiy Kashuba , Herbert Schoeller , Janine Splettstoesser

Quantum adiabatic algorithm is of vital importance in quantum computation field. It offers us an alternative approach to manipulate the system instead of quantum gate model. Recently, an interesting work arXiv:1805.10549 indicated that we…

Quantum Physics · Physics 2019-01-23 Jingwei Wen , Xiangyu Kong , Shijie Wei , Bixue Wang , Tao Xin , Guilu Long

Autoionizing resonances that arise from the interaction of a bound single-excitation with the continuum can be accurately captured with the presently used approximations in time-dependent density functional theory (TDDFT), but those arising…

Materials Science · Physics 2019-03-27 August J. Krueger , Neepa T. Maitra

We consider quantum field theoretic systems subject to a time-dependent perturbation, and discuss the question of defining a time dependent particle number not just at asymptotic early and late times, but also during the perturbation.…

High Energy Physics - Theory · Physics 2016-09-14 Robert Dabrowski , Gerald V. Dunne

Time-dependent density-functional theory (TDDFT) is deemed to be a formally rigorous way of dealing with the time-evolution of a many-electron system at the level of electron densities rather than the underlying wavefunctions, which in turn…

Chemical Physics · Physics 2024-11-26 Jochen Schirmer

Within a Lagrangian formalism we derive the time-dependent Gutzwiller approximation for general multi-band Hubbard models. Our approach explicitly incorporates the coupling between time-dependent variational parameters and a time-dependent…

Strongly Correlated Electrons · Physics 2015-06-15 J. Bünemann , M. Capone , J. Lorenzana , G. Seibold

Most applications of time-dependent density-functional theory (TDDFT) use the adiabatic local-density approximation (ALDA) for the dynamical exchange-correlation potential Vxc(r,t). An exact (i.e., nonadiabatic) extension of the…

Mesoscale and Nanoscale Physics · Physics 2015-06-25 C. A. Ullrich

The adiabatic theorem states that an initial eigenstate of a slowly varying Hamiltonian remains close to an instantaneous eigenstate of the Hamiltonian at a later time. We show that a perfunctory application of this statement is problematic…

Quantum Physics · Physics 2009-11-10 Karl-Peter Marzlin , Barry C. Sanders

Several misprints and small mistakes were in the initial version. They have been corrected. Following the recent experimental realization of synthetic gauge magnetic forces, Jean Dalibard adressed the question whether the adiabatic ansatz…

Analysis of PDEs · Mathematics 2012-01-24 Amandine Aftalion , Francis Nier

An explicit expression for the quadratic density-response function of a many-electron system is obtained in the framework of the time-dependent density-functional theory, in terms of the linear and quadratic density-response functions of…

Materials Science · Physics 2009-11-10 V. U. Nazarov , J. M. Pitarke , C. S. Kim , Y. Takada

We propose a nonadiabatic time-dependent spin-density functional theory (TDSDFT) approach for studying the single-electron excited states and the ultrafast response of systems with strong electron correlations. The correlations are…

Strongly Correlated Electrons · Physics 2013-11-27 Volodymyr Turkowski , Talat S. Rahman

Most present applications of time-dependent density functional theory use adiabatic functionals, i.e. the effective potential at time t is determined solely by the density at the same time. This paper discusses a method that aims to go…

Strongly Correlated Electrons · Physics 2009-11-10 Yair Kurzweil , Roi Baer

Adiabatic passage employs a slowly varying time-dependent Hamiltonian to control the evolution of a quantum system along the Hamiltonian eigenstates. For processes of finite duration, the exact time evolving state may deviate from the…

Quantum Physics · Physics 2021-06-18 Albert Benseny , Klaus Mølmer

The charge-density response of extended materials is usually dominated by the collective oscillation of electrons, the plasmons. Beyond this feature, however, intriguing many-body effects are observed. They cannot be described by one of the…

Materials Science · Physics 2018-12-20 Martin Panholzer , Matteo Gatti , Lucia Reining

In the conventional quantum mechanics (i.e., hermitian QM) the adia- batic theorem for systems subjected to time periodic fields holds only for bound systems and not for open ones (where ionization and dissociation take place) [D. W. Hone,…

Atomic Physics · Physics 2009-11-11 Avner Fleischer , Nimrod Moiseyev

Adiabatic approximations in time-dependent density functional theory (TDDFT) will in general yield unphysical time-dependent shifts in the resonance positions of a system driven far from its ground-state. This spurious time-dependence is…

Chemical Physics · Physics 2016-08-24 Kai Luo , Johanna I. Fuks , Neepa T. Maitra

The time-evolution operator for an explicitly time-dependent Hamiltonian is expressed as the product of a sequence of unitary operators. These are obtained by successive time-dependent unitary transformations of the Hilbert space followed…

Quantum Physics · Physics 2009-10-30 Ali Mostafazadeh

We make use of the time-dependent density functional theory to derive a new formally exact expression for the dc resistivity of metals with impurities. This expression takes fully into account the dynamics of electron-electron interactions.…

Strongly Correlated Electrons · Physics 2014-07-04 V. U. Nazarov , G. Vignale , Y. -C. Chang

Approximate exchange-correlation functionals built by modeling in a non-linear way the adiabatic connection (AC) integrand of density functional theory have many attractive features, being virtually parameters-free and satisfying different…

Chemical Physics · Physics 2018-05-25 S. Vuckovic , P. Gori-Giorgi , F. Della Sala , E. Fabiano

A general quantum adiabatic theorem with and without the time-dependent orthogonalization is proven, which can be applied to understand the origin of activation energies in chemical reactions. Further proofs are also developed for the…

Strongly Correlated Electrons · Physics 2011-11-03 Andrew Das Arulsamy