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We present three schemes to go beyond the electric-dipole approximation in X-ray absorption spectroscopy calculations within a four-component relativistic framework. The first is based on the full semi-classical light-matter interaction…

Chemical Physics · Physics 2021-07-02 Nanna Holmgaard List , Timothé Romain Léo Melin , Martin van Horn , Trond Saue

The non-resonant two-photon ionization of hydrogen-like ions is studied in second-order perturbation theory, based on the Dirac equation. To carry out the summation over the complete Coulomb spectrum, a Green function approach has been…

Atomic Physics · Physics 2009-11-10 Peter Koval , Stephan Fritzsche , Andrey Surzhykov

Two-photon detachment from the F-minus negative ion is investigated within the lowest order of perturbation theory. We show that in accordance with the adiabatic theory a proper asymptotic behaviour of the 2p bound state wave function is…

Atomic Physics · Physics 2007-05-23 G. F. Gribakin , V. K. Ivanov , A. V. Korol , M. Yu. Kuchiev

We address nonsequential double ionization induced by strong, linearly polarized laser fields of only a few cycles, considering a physical mechanism in which the second electron is dislodged by the inelastic collision of the first electron…

Atomic Physics · Physics 2009-11-10 C. Figueira de Morisson Faria , X. Liu , A. Sanpera , M. Lewenstein

The Lorentz-Abraham-Dirac (LAD) equation has proved valuable in describing the motion of radiating electric charges but suffers from runaway, pre-acceleration and other ambiguities. The usual scheme is problematic because of locality, which…

Classical Physics · Physics 2016-11-24 Sofiane Faci , Mario Novello

Angular dependence of photoemission time delay for the valence $np_{3/2}$ and $np_{1/2}$ subshells of Ar, Kr and Xe is studied in the dipole relativistic random phase approximation. Strong angular anisotropy of the time delay is reproduced…

Atomic Physics · Physics 2026-03-03 A. S. Kheifets , Ankur Mandal , P. C. Deshmukh , V. K. Dolmatov , S. T. Manson

Attosecond streaking of atomic photoemission holds the promise to provide unprecedented information on the release time of the photoelectron. We show that attosecond streaking phase shifts indeed contain timing (or spectral phase)…

Parity mixing in photoionization, i.e. when emitted electrons have different parities but the same energy, causes interference observable only in angle-resolved measurements. The interference typically manifests as a symmetry violation in…

Atomic Physics · Physics 2026-04-20 Maria M. Popova , Sergei N. Yudin , Alexei N. Grum-Grzhimailo , Elena V. Gryzlova

Attosecond pulses can ionize atoms in a coherent process. Since the emerging fragments are entangled, however, each preserves only a fraction of the initial coherence, thus limiting the chance of guiding the ion subsequent evolution. In…

Atomic Physics · Physics 2021-06-30 Saad Mehmood , Eva Lindroth , Luca Argenti

Phase and time delays of atomic above-threshold ionization were recently experimentally explored in an $\omega -2\omega$ setting [Zipp et al, Optica 1, 361 (2014)]. The phases of wavepackets ejected from argon by a strong $2\omega$ pulse…

Atomic Physics · Physics 2022-11-23 Diego G. Arbó , Sebastián D. López , Joachim Burgdörfer

The present review addresses the technical advances and the theoretical developments to realize and rationalize attosecond-science experiments that reveal a new dynamical time scale ($10^{-15}$-$10^{-18}$ s), with a particular emphasis on…

Chemical Physics · Physics 2020-02-07 Denitsa Baykusheva , Hans Jakob Wörner

We study ionization of aligned H$_2^+$ in strong elliptically-polarized laser fields numerically and analytically. The calculated offset angle in photoelectron momentum distribution is several degrees larger for the molecule than a model…

Atomic Physics · Physics 2023-01-03 J. Y. Che , Y. G. Peng , F. B. Zhang , X. J. Xie , G. G. Xin , Y. J. Chen

The relativistic theory of above-threshold ionization (ATI) of hydrogen-like atoms in ultrastrong radiation fields, taking into account the photoelectron induced rescattering in the continuum spectrum is developed. It is shown that the…

Quantum Physics · Physics 2007-05-23 H. K. Avetissian , A. G. Markossian , G. F. Mkrtchian

The force exerted on a material by an incident beam of light is dependent upon the material's velocity in the laboratory frame of reference. This velocity dependence is known to be diffcult to measure, as it is proportional to the incident…

Optics · Physics 2012-05-28 S. A. R. Horsley , M. Artoni , G. C. La Rocca

In this tutorial we summarize the physics and mathematics behind refractive electromagnetic wave bending and delay. Refractive bending and delay through the Earth's atmosphere at both radio/millimetric and optical/IR wavelengths are…

Instrumentation and Methods for Astrophysics · Physics 2015-06-23 Jeffrey G. Mangum , Patrick Wallace

We argue that the asymmetry between diverging and converging electromagnetic waves is just one of many asymmetries in observed phenomena that can be explained by a past hypothesis and statistical postulate (together assigning probabilities…

History and Philosophy of Physics · Physics 2023-04-21 Mario Hubert , Charles T. Sebens

We theoretically study time-resolved photoemission in atoms as probed by attosecond streaking. We review recent advances in the study of the photoelectric effect in the time domain and show that the experimentally accessible time shifts can…

Atomic Physics · Physics 2015-03-06 Stefan Nagele , Renate Pazourek , Michael Wais , Georg Wachter , Joachim Burgdörfer

Photoelectron angular distributions of the two-photon ionization of neutral atoms are theoretically investigated. Numerical calculations of two-photon ionization cross sections and asymmetry parameters are carried out within the…

Atomic Physics · Physics 2020-10-22 J. Hofbrucker , L. Eiri , A. V. Volotka , S. Fritzsche

Shape resonances in photoionization of atoms and molecules arise from a particular geometry of the ionic potential which traps the receding photoelectron in a quasi-bound state in a particular partial wave. This mechanism allows us to…

Atomic Physics · Physics 2026-03-03 Anatoli S. Kheifets , Stephen Catsamas

Shake-up is a fundamental phenomenon in photoionisation of many-electron systems whereby the ionisation of one electron is accompanied by the simultaneous excitation of another. As a single-photon two-electron excitation, it is the most…