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We show that time ordering underlying time-dependent quantum dynamics is a physical observable accessible by attosecond streaking. We demonstrate the extraction of time ordering for the prototypical case of time-resolved two-photon double…

Atomic Physics · Physics 2015-03-06 Renate Pazourek , Stefan Nagele , Joachim Burgdörfer

A photoelectron forced to pass through two atomic energy levels before receding from the residual ion shows interference fringes in its angular distribution as manifestation of a two-slit-type interference experiment in wave-vector space.…

Quantum Physics · Physics 2019-07-16 Jonas Wätzel , Andrew James Murray , Jamal Berakdar

Several recent attoclock experiments have investigated the fundamental question of a quantum mechanically induced time delay in tunneling ionization via extremely precise photoelectron momentum spectroscopy. The interpretations of those…

We predict a significant delay of two-electron photoemission from the helium atom after absorption of an attosecond XUV pulse. We establish this delay by solving the time dependent Schr\"odinger equation and by subsequent tracing the…

Atomic Physics · Physics 2026-03-03 A. S. Kheifets , I. A. Ivanov , Igor. Bray

We study orientation and two-center interference effects in attosecond time-resolved photoionization of the H$_2$ molecule. Time resolution of XUV ionization of H$_2$ is gained through the phase retrieval capability of attosecond angular…

Atomic Physics · Physics 2026-03-03 Vladislav V. Serov , Anatoli S. Kheifets

Photoionization of matter is one of the fastest electronic processes in nature. Experimental measurements of photoionization dynamics have become possible through attosecond metrology. However, all experiments reported to date contain a…

Quantum Physics · Physics 2025-02-11 Meng Han , Jia-Bao Ji , Leung Chung Sum , Kiyoshi Ueda , Hans Jakob Wörner

It is shown that it is feasible to use ultrashort time delay between two XUV femtosecond pulses in order to control two photon resonant ionization. The proposal is demonstrated on the spectrum of Helium, in terms of nonperturbative…

Atomic Physics · Physics 2019-08-22 Theodoros Mercouris , Yannis Komninos , Cleanthes A. Nicolaides

We investigated experimentally and theoretically angular momentum alignment-to-orientation conversion created by the joint interaction of laser radiation and an external magnetic field with atomic rubidium at room temperature. In particular…

Atomic Physics · Physics 2020-11-11 A. Mozers , L. Busaite , D. Osite , M. Auzinsh

It is proved that when the retarded effect (or multiple moment effect) of radiation fields is taken into account, the high order stimulated radiation and stimulated absorption probabilities of light are not the same so that time reversal…

General Physics · Physics 2008-04-10 Mei Xiaochun

We present transient absorption spectra of an extreme ultraviolet attosecond pulse train in helium dressed by an 800 nm laser field with intensity ranging from $2\times10^{12}$ W/cm$^2$ to $2\times10^{14}$ W/cm$^2$. The energy range probed…

A new semiclassical approach to ionization by an oscillating field is presented. For a delta-function atom, an asymptotic analysis is performed with respect to a quantity h, defined as the ratio of photon energy to ponderomotive energy.…

Quantum Physics · Physics 2009-10-30 Klaus Ergenzinger

The photoelectric effect, explained by Einstein in 1905, is often regarded as a one-electron phenomenon. However, in multi-electron systems, the interaction of the escaping electron with other electrons, referred to as electron correlation,…

Ji \etal [New J. Phys. {\bf 26}, 093014 (2024)] established a direct link between the photoionization cross section and the attosecond time delay near Cooper minima (CM) in the valence shells of noble-gas atoms. This link is based on the…

Atomic Physics · Physics 2026-03-03 Adam J. C. Singor , Dmitry V. Fursa , Igor Bray , Anatoli S. Kheifets

Non-resonant light interacting with diatomics via the polarizability anisotropy couples different rotational states and may lead to strong hybridization of the motion. The modification of shape resonances and low-energy scattering states…

The evolution of electron wavepackets determines the course of many physical and chemical phenomena and attosecond spectroscopy aims to measure and control such dynamics in real-time. Here, we investigate radial electron wavepacket motion…

Atomic Physics · Physics 2015-09-04 Niranjan Shivaram , Xiao-Min Tong , Henry Timmers , Arvinder Sandhu

In conventional \textit{ab initio} methodologies, phonons are calculated by solving equations of motion involving static interatomic force constants and atomic masses. The Born-Oppenheimer approximation, where all electronic degrees of…

Materials Science · Physics 2024-03-15 Shang Ren , John Bonini , Massimiliano Stengel , Cyrus E. Dreyer , David Vanderbilt

The use of finite harmonic oscillator spaces in many-body calculations introduces both infrared (IR) and ultraviolet (UV) errors. The IR effects are well approximated by imposing a hard-wall boundary condition at a properly identified…

Nuclear Theory · Physics 2014-12-30 S. König , S. K. Bogner , R. J. Furnstahl , S. N. More , T. Papenbrock

A formalism for describing relativistic ponderomotive effects, which occur in the dynamics of an electron driven by a focused relativisticaly intense optical envelope, is established on the basis of a rigorous asymptotic expansion of the…

Plasma Physics · Physics 2019-11-19 O. B. Shiryaev

Measuring and controlling the ionization dynamics by intense laser fields has recently led to important breakthroughs, from the investigation of tunneling time delays to attosecond molecular imaging by electron holography. In these…

We use R-Matrix with Time-dependence (RMT) theory, with spin-orbit effects included, to study krypton irradiated by two time-delayed XUV ultrashort pulses. The first pulse excites the atom to 4s$^{2}$4p$^{5}$5s. The second pulse then…