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Higher order parameters in the hard disk fluid are computed to investigate the number, the life time and size of transient crystal nuclei in the pre-freezing phase. The methodology introduces further neighbor shells bond orientational order…

Statistical Mechanics · Physics 2012-11-22 Masaharu Isobe , Berni J. Alder

The crystalline solids with lack of orientational ordering of anisotropic particles serve the purpose of studying the disordered systems with many fundamental applications in contemporary research. Despite the orientational disorder,…

Soft Condensed Matter · Physics 2024-11-01 Sumitava Kundu , Kaustav Chakraborty , Avisek Das

Granular crystallisation is an important phenomenon whereby ordered packing structures form in granular matter under vibration. However, compared with the well-developed principles of crystallisation at the atomic scale, crystallisation in…

Disordered Systems and Neural Networks · Physics 2018-05-22 Weijing Dai , Joerg Reimann , Dorian Hanaor , Claudio Ferrero , Yixiang Gan

By molecular-dynamics simulations, we have studied the devitrification (or crystallization) of aged hard-sphere glasses. First, we find that the dynamics of the particles are intermittent: Quiescent periods, when the particles simply…

Soft Condensed Matter · Physics 2014-04-03 Eduardo Sanz , Chantal Valeriani , Emanuela Zaccarelli , Wilson C K Poon , Michael E Cates , Peter N Pusey

We present a method for simulating fluid vesicles with in-plane orientational ordering. The method involves computation of local curvature tensor and parallel transport of the orientational field on a randomly triangulated surface. It is…

Biological Physics · Physics 2015-05-18 N. Ramakrishnan , P. B. Sunil Kumar , John H. Ipsen

Advancements in the synthesis of faceted nanoparticles and colloids have spurred interest in the phase behavior of polyhedral shapes. Regular tetrahedra have attracted particular attention because they prefer local symmetries that are…

Soft Condensed Matter · Physics 2011-11-24 Amir Haji-Akbari , Michael Engel , Sharon C. Glotzer

Since the 1920s, packing arguments have been used to rationalize crystal structures in systems ranging from atomic mixtures to colloidal crystals. Packing arguments have recently been applied to complex nanoparticle structures, where they…

Soft Condensed Matter · Physics 2018-05-09 Rose Cersonsky , Greg van Anders , Paul M. Dodd , Sharon C. Glotzer

I report on the experimental confirmation that critical percolation statistics underlie the ordering kinetics of twisted nematic phases in the Allen-Cahn universality class. Soon after the ordering starts from a homogeneous disordered phase…

Statistical Mechanics · Physics 2024-01-17 Renan A. L. Almeida

We investigate the atomistic mechanism of homogeneous nucleation during solidification in molybdenum employing transition path sampling. The mechanism is characterized by the formation of a pre-structured region of high bond-orientational…

Materials Science · Physics 2020-10-16 Sarath Menon , Grisell Díaz Leines , Ralf Drautz , Jutta Rogal

Orientational and positional ordering properties of liquid crystal monolayers are examined by means of Fundamental-Measure Density Functional Theory. Particles forming the monolayer are modeled as hard parallelepipeds of square section of…

Soft Condensed Matter · Physics 2015-06-19 Yuri Martinez-Raton , Szabolcs Varga y Enrique Velasco

We study here how phase transitions are induced in colloidal suspensions by a point-like heat source, an optically trapped metal oxide particle absorbing light. We find that thermophoresis increases the number density of colloids around the…

Soft Condensed Matter · Physics 2019-11-26 Nicolas Bruot , Hajime Tanaka

We present a numerical study on geometric percolation in liquid dispersions of hard slender colloidal particles subjected to an external orienting field. In the formulation and liquid-state processing of nanocomposite materials, the…

Soft Condensed Matter · Physics 2020-02-26 Shari P. Finner , Ilian Pihlajamaa , Paul van der Schoot

The intricate interplay between colloidal particle shape and precisely engineered interaction potentials has paved the way for the discovery of unprecedented crystal structures in both two and three dimensions. Here, we make use of…

Soft Condensed Matter · Physics 2023-11-27 Fabrizio Camerin , Susana Marín-Aguilar , Marjolein Dijkstra

Via mechanisms not accessible at equilibrium, self-propelled particles can form phases with positional order, such as crystals, and with orientational order, such as polar flocks. However, the interplay between these two types of order…

Soft Condensed Matter · Physics 2025-08-13 Till Welker , Ricard Alert

Non-aligning self-propelled particles with purely repulsive excluded volume interactions undergo athermal motility-induced phase separation into a dilute gas and a dense cluster phase. Here, we use enhanced sampling computational methods…

Soft Condensed Matter · Physics 2016-10-05 Gabriel S. Redner , Caleb G. Wagner , Aparna Baskaran , Michael F. Hagan

Nucleation processes are at the heart of a large number of phenomena, from cloud formation to protein crystallization. A recently emerging area where nucleation is highly relevant is the initiation of filamentous protein self-assembly, a…

Soft Condensed Matter · Physics 2017-01-05 Anđela Šarić , Thomas C. T. Michaels , Alessio Zaccone , Tuomas P. J. Knowles , Daan Frenkel

The phase field theory of crystal nucleation described in [L. Granasy, T. Borzsonyi, T. Pusztai, Phys. Rev. Lett. 88, 206105 (2002)] is applied for nucleation in hard--sphere liquids. The exact thermodynamics from molecular dynamics is…

Statistical Mechanics · Physics 2009-11-10 Laszlo Granasy , Tamas Pusztai , Zoltan Jurek , Massimo Conti , Bjorn Kvamme

Monte Carlo simulations of crystal nuclei coexisting with the fluid phase in thermal equilibrium in finite volumes are presented and analyzed, for fluid densities from dense melts to the vapor. Generalizing the lever-rule for two-phase…

Statistical Mechanics · Physics 2017-11-01 Peter Koß , Antonia Statt , Peter Virnau , Kurt Binder

Dynamical density functional simulations reveal structural aspects of crystal nucleation in undercooled liquids: the first appearing solid is amorphous, which promotes the nucleation of bcc crystals, but suppresses the appearance of the fcc…

Materials Science · Physics 2015-05-30 Gyula I. Tóth , Tamás Pusztai , György Tegze , Gergely Tóth , László Gránásy

Monte Carlo simulation, experiment and continuum theory are used to examine the anchoring exhibited by a nematic liquid crystal at a patterned substrate comprising a periodic array of rectangles that, respectively, promote vertical and…

Soft Condensed Matter · Physics 2013-08-09 Candy Anquetil-Deck , Douglas J. Cleaver , Jonathan P. Bramble , Timothy J. Atherton