Related papers: Spin/Phonon Dynamics in Single Molecular Magnets: …
Molecular vibrations are increasingly seen as a key factor for spin dynamics in single-ion magnets and molecular spin qubits. Herein we show how an inexpensive combination of molecular dynamics calculations and a crystal field analysis can…
Magnetic-field gradients are important for single-site addressability and electric-dipole spin resonance of spin qubits in semiconductor devices. We show that these advantages are offset by a potential reduction in coherence time due to the…
The quantum dot spin chain system is vital for quantum simulation and studying collective electron behaviors, necessitating an understanding of its mechanisms and control protocols. Chapter 1 introduces key concepts, focusing on the…
We study the spin mixing dynamics of ultracold spin-1 atoms in a weak non-uniform magnetic field with field gradient $G$, which can flip the spin from +1 to -1 so that the magnetization $m=\rho_{+}-\rho_{-}$ is not any more a constant. The…
Multi-configurational wave-function theory (MC-WFT) that combines complete active space self-consistent field (CASSCF) approach with subsequent state interaction (SI) treatment of spin-orbit coupling (SOC), abbreviated as CASSCF-SO, plays…
We describe and analyze a tight-binding model of single molecule magnets (SMMs) that captures both the spin and spatial aspects of the SMM electronic structure. The model generalizes extended Huckel theory to include the effects of spin…
Understanding the spin dephasing mechanism is of fundamental importance in all potential applications of the spin qubit. Here we demonstrate a spin dephasing mechanism in semiconductor quantum dot due to the $1/f$ charge noise. The…
Understanding the spin dynamics in antiferromagnetic (AFM) thin films is fundamental for designing novel devices based on AFM magnon transport. Here, we study the magnon dynamics in thin films of AFM $S=5/2$ $\alpha$-Fe$_2$O$_3$ by…
We show that in the presence of ferromagnetic electronic reservoirs and spin-dependent tunnel couplings, molecular vibrations in nonmagnetic single molecular transistors induce an effective intramolecular exchange magnetic field. It…
A new family of supramolecular, antiferromagnetically exchange-coupled dimers of single-molecule magnets (SMMs) has recently been reported [W. Wernsdorfer, N. Aliaga-Alcalde, D.N. Hendrickson, and G. Christou, Nature 416, 406 (2002)]. Each…
It has been shown elsewhere that two spatially separated atoms can jointly absorb one photon, whose frequency is equal to the sum of the transition frequencies of the two atoms. We describe this process in the presence of an ensemble of…
We measure magnetization changes in a single crystal of the single-molecule magnet Fe8 when exposed to intense, short (<20 $\mu$s) pulses of microwave radiation resonant with the m = 10 to 9 transition. We find that radiation induces a…
In the "flopping-mode" regime of electron spin resonance, a single electron confined in a double quantum dot is electrically driven in the presence of a magnetic field gradient. The increased dipole moment of the charge in the flopping mode…
Numerical modelling of coherent spin relaxation in nanomagnets, formed by magnetic molecules of high spins, is accomplished. Such a coherent spin dynamics can be realized in the presence of a resonant electric circuit coupled to the magnet.…
A general polarizable embedded (PE) quantum mechanics/molecular mechanics scheme for periodic systems is presented, describing mutual polarization of the two subsystems. The QM system, described with density functional theory (DFT), is…
An emerging paradigm in modern electronics is that of CMOS + $\sf X$ requiring the integration of standard CMOS technology with novel materials and technologies denoted by $\sf X$. In this context, a crucial challenge is to develop accurate…
Solid-state spin systems hold great promise for quantum information processing and the construction of quantum networks. However, the considerable inhomogeneity of spins in solids poses a significant challenge to the scaling of solid-state…
Magnetic switching of a single molecular magnet (SMM) due to spin-polarized current flowing between ferromagnetic metallic electrodes is investigated theoretically. Magnetic moments of the electrodes are assumed to be collinear and parallel…
Entanglement in a many-particle system can enable measurement sensitivities beyond that achievable by only classical correlations. For an ensemble of spins, all-to-all interactions are known to reshape the quantum projection noise, leading…
The realisation of quantum computers based on molecular electronic spins requires the design of qubits with very long coherence times, T2. Dephasing can proceed over several different microscopic pathways, active at the same time and in…