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High fidelity entanglement of an on-chip array of spin qubits poses many challenges. Spin-orbit coupling (SOC) can ease some of these challenges by enabling long-ranged entanglement via electric dipole-dipole interactions, microwave…

Mesoscale and Nanoscale Physics · Physics 2017-01-06 J. Salfi , J. A. Mol , Dimitrie Culcer , S. Rogge

We derive the spin-atomic vibration interaction $V_{\rm SA}$ and the spin-flip Hamiltonian $V_{\rm SF}$ of a single atomic spin in a crystal field. We here apply the perturbation theory to a model with the spin-orbit interaction and the…

Mesoscale and Nanoscale Physics · Physics 2010-11-11 Satoshi Kokado , Kikuo Harigaya , Akimasa Sakuma

Coherent tripartite interactions among degrees of freedom of completely different nature are instrumental for quantum information and simulation technologies, but they are generally difficult to realize and remain largely unexplored. Here,…

Quantum Physics · Physics 2023-03-01 Xin-Lei Hei , Peng-Bo Li , Xue-Feng Pan , Franco Nori

Recent radio frequency scanning tunneling spectroscopy (rf-STS) experiments have demonstrated nuclear and electron spin excitations up to $\pm12\hbar$ in a single molecular spin quantum dot (qudot). Despite the profound experimental…

Single-molecule memory device based on a single-molecule magnet (SMM) is one of the ultimate goals of semiconductor nanofabrication technologies. Here, we study how to manipulate and readout the SMM's two spin-state of stored information…

Mesoscale and Nanoscale Physics · Physics 2021-12-28 Hai-Bin Xue , Jiu-Qing Liang , Wu-Ming Liu

A single atom is the prototypical quantum system, and a natural candidate for a quantum bit - the elementary unit of a quantum computer. Atoms have been successfully used to store and process quantum information in electromagnetic traps, as…

Mesoscale and Nanoscale Physics · Physics 2013-05-21 Jarryd J. Pla , Kuan Y. Tan , Juan P. Dehollain , Wee H. Lim , John J. L. Morton , David N. Jamieson , Andrew S. Dzurak , Andrea Morello

Single-molecule magnets (SMMs) with chemically tailorable properties are potential building blocks for quantum computing, high-density magnetic memory, and spintronics.1 2 3,4 These applications require isolated or few molecules on…

We consider the Kondo tunneling induced by multiphonon emission/absorption processes in magnetic molecular complexes with low-energy singlet-triplet spin gap and show that the number of assisting phonons may be changed by varying the Zeeman…

Strongly Correlated Electrons · Physics 2009-11-13 K. Kikoin , M. N. Kiselev

Spin wave modes confined in a ferromagnetic film by the spatially inhomogeneous magnetic field generated by a scanned micromagnetic tip of a ferromagnetic resonance force microscope (FMRFM) enable microscopic imaging of the internal fields…

The spin dynamics in [TbPc$_{2}$]$^{0}$ and [DyPc$_{2}$]$^{0}$ single molecule magnets have been investigated by means of muon and nuclear spin-lattice relaxation rate measurements. The correlation time for the spin fluctuations was found…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 F. Branzoli , M. Filibian , P. Carretta , S. Klytaskaya , M. Ruben

Spin-electronic devices are poised to become part of mainstream microelectronic technology .Downsizing them, however, faces the intrinsic difficulty that as ferromagnets become smaller, it becomes more difficult to stabilize their magnetic…

Molecular spin clusters are mesoscopic systems whose structural and physical features can be tailored at the synthetic level. Besides, their quantum behavior is directly accessible in laboratory and their magnetic properties can be…

Mesoscale and Nanoscale Physics · Physics 2015-05-18 F. Troiani , V. Bellini , A. Candini , G. Lorusso , M. Affronte

Magnetic metal-organic frameworks (MMOFs), where magnetic metal nodes are connected into a crystal structure by organic linkers, have a potential to host exotic magnetic states. We present a study of bulk magnetic properties of four…

The simulation of nuclear magnetic resonance (NMR) experiments is a notoriously difficult task, if many spins participate in the dynamics. The recently established dynamic mean-field theory for high-temperature spin systems (spinDMFT)…

Chemical Physics · Physics 2026-02-04 Timo Gräßer , Götz S. Uhrig

We present measurements and a theoretical model for the interplay of spin dependent interactions and external magnetic fields in atomic spinor condensates. We highlight general features like quadratic Zeeman dephasing and its influence on…

Other Condensed Matter · Physics 2009-11-11 J. Kronjäger , C. Becker , M. Brinkmann , R. Walser , P. Navez , K. Bongs , K. Sengstock

Magnetophononics, the modulation of magnetic interactions by driven infrared-active lattice excitations, is emerging as a key mechanism for the ultrafast dynamical control of both semiclassical and quantum spin systems by coherent light. We…

Strongly Correlated Electrons · Physics 2023-05-17 M. Yarmohammadi , M. Krebs , G. S. Uhrig , B. Normand

We theoretically investigate spin-dependent carrier dynamics due to the electron-phonon interaction after ultrafast optical excitation in ferromagnetic metals. We calculate the electron-phonon matrix elements including the spin-orbit…

Materials Science · Physics 2015-05-30 Sven Essert , Hans Christian Schneider

We developed a general framework for hybrid quantum-classical computing of molecular and periodic embedding approaches based on an orbital space separation of the fragment and environment degrees of freedom. We demonstrate its potential by…

Chemical Physics · Physics 2024-12-23 Stefano Battaglia , Max Rossmannek , Vladimir V. Rybkin , Ivano Tavernelli , Jürg Hutter

We study the reduced dynamics of a spin (qubit) coupled to a spin-boson environment in the case of pure dephasing. We derive formal exact expressions which can be cast in terms of exact integro-differential master equations. We present…

Statistical Mechanics · Physics 2009-11-10 E. Paladino , M. Sassetti , G. Falci

We investigate the validity conditions of the single mode approximation (SMA) in spinor-1 atomic condensate when effects due to residual magnetic fields are negligible. For atomic interactions of the ferromagnetic type, the SMA is shown to…

Superconductivity · Physics 2009-11-07 S. Yi , O. E. Mustecaplioglu , C. P. Sun , L. You
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