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The development of compact and bright XUV and soft X-ray sources based on high-order harmonic generation is boosting advances towards understanding the behavior of matter with extreme temporal and spatial resolutions. Here, we report…

We describe a new method for imaging ultrafast dynamics in condensed matter using inelastic x-ray scattering (IXS). We use the concepts of causality and irreversibility to construct a general solution to the inverse scattering problem (or…

Other Condensed Matter · Physics 2009-06-12 P. Abbamonte , G. C. L. Wong , D. Cahill , J. P. Reed , R. H. Coridan , N. W. Schmidt , G. H. Lai , Y. I. Joe , D. Casa

We use femtosecond x-ray diffraction to study the structural response of charge and orbitally ordered Pr$_{1-x}$Ca$_x$MnO$_3$ thin films across a phase transition induced by 800 nm laser pulses. By investigating the dynamics of both…

We report on the development of an ultrafast Transmission Electron Microscope based on a laser-driven cold-field emission source. We first describe the instrument before reporting on numerical simulations of the laser-driven electron…

Optics · Physics 2019-11-27 G. M. Caruso , F. Houdellier , S. Weber , M. Kociak , A. Arbouet

We report the design and performance of a time-resolved electron diffraction apparatus capable of producing intense bunches with simultaneously single digit micron probe size, long coherence length, and $200$ fs rms time resolution. We…

We have explored the light induced dynamics in superfluid helium nanodroplets with wide-angle scattering in a pump-probe measurement scheme. The droplets are doped with xenon atoms to facilitate the ignition of a nanoplasma through…

Thick diffractive optical elements offer a promising way to achieve focusing or imaging at a resolution approaching 1 nm for X-ray wavelengths shorter than about 0.1 nm. Efficient focusing requires that these are fabricated with structures…

Optics · Physics 2020-12-02 Henry N. Chapman , Saša Bajt

Laser-driven proton sources have long been developed with an eye on their potential for medical application to radiation therapy. These sources are compact, versatile, and show peculiar characteristics such as extreme instantaneous dose…

Novel optical elements containing semitransparent wavelike films embedded into the bulk of transparent material, which form a reflection image without transmitted light distortion, are studied. The dynamic theory of light diffraction by a…

Optics · Physics 2018-05-23 Anatoly M. Smolovich , Valery Chernov

Ultrashort and ultracold electron bunches created by near-threshold femtosecond photoionization of a laser-cooled gas hold great promise for single-shot ultrafast diffraction experiments. In previous publications the transverse beam quality…

Atomic Physics · Physics 2018-01-17 J. G. H. Franssen , J. M. Kromwijk , E. J. D. Vredenbregt , O. J. Luiten

Coherent x-ray diffractive imaging is extended to high resolution strain analysis in crystalline nanostructured devices. The application potential is demonstrated by determining the strain distribution in (Ga,Mn)As/GaAs nanowires. By…

The observation of non-perturbative harmonic emission in solids from ultrashort laser pulses [1] sparked a wave of studies [2,3] as a probe of charge carrier dynamics in solids under strong fields and a route to extreme ultraviolet (XUV)…

Water-window X-rays are crucial in medical and biological applications, enabling natural contrast imaging of biological cells in their near-native states without external staining. However, water-window X-ray sources whose output photon…

The availability of ultrafast pulses of coherent hard x-rays from the Linac Coherent Light Source opens new opportunities for studies of atomic-scale dynamics in amorphous materials. Here we show that single ultrafast coherent x-ray pulses…

Grazing incidence fast atom diffraction has mainly been investigated with helium atoms, considered as the best possible choice for surface analysis. This article presents experimental diffraction profiles recorded with neon projectile,…

Chemical Physics · Physics 2023-10-24 Maxime Debiossac , Peng Pan , Philippe Roncin

We report the implementation of energy dispersive X-ray spectroscopy for layered semiconductors in the form of atomically thin transition metal dichalcogenides. The technique is based on a scanning electron microscope equipped with a…

Mesoscale and Nanoscale Physics · Physics 2022-11-17 Anna Rupp , Jonas Göser , Zhijie Li , Philipp Altpeter , Ismail Bilgin , Alexander Högele

Here we experimentally map the dynamics of electron plasma waves in laser solid interaction. We do time resolved measurements of second harmonic and hard X-ray generation from interaction of intense ($10^{16} W cm^{-2}$, 100 fs, 800nm)…

Plasma Physics · Physics 2007-05-23 Arvinder S. Sandhu , G. Ravindra Kumar , S. Sengupta , A. Das , P. K. Kaw

Delivering sub-micrometer particles to an intense x-ray focus is a crucial aspect of single-particle diffractive-imaging experiments at x-ray free-electron lasers. Enabling direct visualization of sub-micrometer aerosol particle streams…

Solid-state high-harmonic spectroscopy allows the study of strongly driven ultrafast electron dynamics. Microscopically, high harmonics are generated by strong-laser-field acceleration of electron-hole pairs through the lattice. At finite…

Interfering deep ultraviolet (DUV) lasers can induce substantial density modulations in an ozone-doped gas flow via photochemical reactions, creating volume diffraction gratings. These transient optics are immune to target debris and…