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In this paper we present a computer simulation study of ionic conductivity in solid polymeric electrolytes. The multiphase nature of the material is taken into account. The polymer is represented by a regular lattice whose sites represent…

Condensed Matter · Physics 2007-05-23 Aninda Jiban Bhattacharyya , T. R. Middya , S. Tarafdar

Dielectrophoresis (DEP), the motion of polarizable particles in non-uniform electric fields, has become an important tool for the transport, separation, and characterization of microparticles in biomedical and nanoelectronics research. In…

Soft Condensed Matter · Physics 2009-11-11 E. Salonen , E. Terama , I. Vattulainen , M. Karttunen

An immobile charged species provides a charged medium for transport of charge carriers that is exploited in many applications, such as permselective membranes, doped semiconductors, biological ion channels, as well as porous media and…

Chemical Physics · Physics 2019-10-09 Juhyun Song , Edwin Khoo , Martin Z. Bazant

We report measurements on the dynamics of the Debye layer at a gold electrode in several electrolytes. In the experiments, the Debye layer transmits a damped voltage wave along the electrode, which we use to probe the dynamics. We compare…

Mesoscale and Nanoscale Physics · Physics 2023-10-10 Thanh-Tri Châu , Giovanni Zocchi

Lithium chloride LiCl is widely used as a prototype system to study the strongly dissociated 1-1 electrolyte solution. Here, we combined experimental measurements and classical molecular dynamics simulations to study the ion conduction in…

Soft Condensed Matter · Physics 2019-05-14 Are Yllö , Chao Zhang

Multiparticle collision dynamics (MPCD) is a relatively new algorithm of fluid flow simulations that has been applied mostly to flows around simple objects. One might ask how it behaves in more complex flows. Therefore, we extend MPCD to…

Computational Physics · Physics 2016-10-31 Maciej Matyka

Electrostatic interactions in polymeric systems are responsible for a wide range of liquid-liquid phase transitions that are of importance for biology and materials science. Such transitions are referred to as complex coacervation, and…

Soft Condensed Matter · Physics 2023-09-29 Boyuan Yu , Heyi Liang , Paul F. Nealey , Matthew Tirrell , Artem M. Rumyantsev , Juan J. de Pablo

Using molecular dynamics simulations we study the thermodynamic behavior of a single-component covalent material described by the recently proposed Environment-Dependent Interatomic Potential (EDIP). The parameterization of EDIP for silicon…

Materials Science · Physics 2009-11-07 P. Keblinski , M. Z. Bazant , R. K. Dash , M. M. Treacy

A kinetic model of the electron transfer at the electrode / electrolyte solution interface is developed, implemented in a Monte Carlo framework, and applied to simulate this process in idealised systems consisting of the primitive model of…

Solid state batteries have emerged as a potential next-generation energy storage device due to safety and energy density advantages. Development of electrolyte is one of the most important topics in solid state batteries. Electrochemical…

Materials Science · Physics 2021-10-04 Changyu Deng , Wei Lu

Polymer electrolytes are intensely investigated for use as solid electrolytes in next generation lithium-ion and lithium-metal batteries. However, little is known about the structural and dynamical properties of polymer electrolytes close…

Soft Condensed Matter · Physics 2021-12-02 Andreas Thum , Diddo Diddens , Andreas Heuer

The electrical impedance response of Gelatin based solid polymer electrolyte to gamma irradiation is investigated by impedance spectroscopy. An analysis based on Poisson-Nernst-Plank model, incorporating fractional time derivatives is…

Materials Science · Physics 2015-03-25 Tania Basu , Abhra Giri , Sujata Tarafdar , Shantanu Das

Polyelectrolyte gels are a very attractive class of actuation materials with remarkable electronic and mechanical properties with a great similarity to biological contractile tissues. They consist of a polymer network with ionizable groups…

Materials Science · Physics 2015-09-16 Thomas Wallmersperger , Falk K. Wittel , Michele D'Ottavio , Bernd Kröplin

Many key industrial processes, from electricity production, conversion and storage to electrocatalysis or electrochemistry in general, rely on physical mechanisms occurring at the interface between a metallic electrode and an electrolyte…

Computational Physics · Physics 2021-09-03 Laura Scalfi , Mathieu Salanne , Benjamin Rotenberg

We investigate theoretically the phase diagram of an insoluble charged surfactant monolayer in contact with a semi-dilute polyelectrolyte solution (of opposite charge). The polyelectrolytes are assumed to have long-range and attractive…

Soft Condensed Matter · Physics 2012-07-19 Adi Shafir , David Andelman

Polymeric ionic liquids are emerging polyelectrolyte materials for modern electrochemical applications. In this paper, we propose a self-consistent field theory of the polymeric ionic liquid on a charged conductive electrode. Taking into…

Soft Condensed Matter · Physics 2022-02-02 Yury A. Budkov , Nikolai N. Kalikin , Andrei L. Kolesnikov

This tutorial review focuses on the basic theoretical backgrounds, their working principles, and implementation of impedance spectroscopy in both electroceramics and electrochemical research and technological applications. Various…

Applied Physics · Physics 2024-06-26 Subrata Karmakar

Recent experimental observations of anisotropic conductivity in stretched polymer electrolytes films of the polyethylene oxide family are discussed. The main experimental observations, enhancement of the ionic diffusion and conductivity in…

Soft Condensed Matter · Physics 2007-05-23 Oliver Duerr , Wolfgang Dieterich , Philipp Maas , Abraham Nitzan

Study of various interesting features related to the nonlinear electrical response in composite materials through a model bond percolative system.

Condensed Matter · Physics 2007-05-23 Abhijit Kar Gupta , Asok K. Sen

Electropolymerization is a bottom-up materials engineering process of micro and nano-scale that utilizes electrical signals to deposit conducting dendrites' morphologies by a redox reaction in the liquid phase. It resembles synaptogenesis…

Disordered Systems and Neural Networks · Physics 2021-07-08 Ankush Kumar , Kamila Janzakova , Yannick Coffinier , Sébastien Pecqueur , Fabien Alibart