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We elucidate light-induced orbital and spin current through nonlinear response theory, which generalizes the well-known bulk photovoltaic effect in centrosymmetric broken materials from charge to the spin and orbital degrees of freedom. We…

Materials Science · Physics 2021-08-30 Xingchi Mu , Jian Zhou

We investigate the dependence of the photogalvanic response of a multi-Weyl semimetal on its topological charge, tilt, and chemical potential. We derive analytical expressions for the shift and injection conductivities for tilted charge-$n$…

Mesoscale and Nanoscale Physics · Physics 2024-01-17 Arpit Raj , Swati Chaudhary , Gregory A. Fiete

We study the Fermi surface contribution to the nonlinear DC photocurrent at quadratic order in a spatially uniform optical field in the ultra-clean limit. In addition to shift and injection current, we find that polarized light incident on…

Materials Science · Physics 2021-12-07 Lingyuan Gao , Zachariah Addison , E. J. Mele , Andrew M. Rappe

Bulk photovoltaic (BPV) effect, a second order nonlinear process that generates static current under light irradiation, requires centrosymmetric broken systems as its application platform. In order to realize measurable BPV photocurrent in…

Materials Science · Physics 2023-01-05 Xingchi Mu , Qianqian Xue , Yan Sun , Jian Zhou

A bicircular light (BCL) consists of left and right circularly polarized lights with different frequencies, and draws a rose-like pattern with a rotational symmetry determined by the ratio of the two frequencies. Here we show that an…

Mesoscale and Nanoscale Physics · Physics 2023-09-13 Yuya Ikeda , Sota Kitamura , Takahiro Morimoto

We theoretically discover possible dc-current induction and high-harmonic generation from photodriven chiral fermions in B20-type semimetals irradiated with circularly polarized light as nonlinear optical responses with several…

Materials Science · Physics 2025-06-24 Yuya Ominato , Masahito Mochizuki

Ferroelectric anomalous photovoltaic (APV) effect, as a fascinating physical conceptual phenomenon, holds significant potentials for new optoelectronic device applications. However, due to the knowledge lacking on the origin and underlying…

Materials Science · Physics 2025-09-04 Linjie Wei , Fu Li , Yi Liu , Hongbin Zhang , Junhua Luo , Zhihua Sun

Symmetry plays a central role in conventional and topological phases of matter, making the ability to optically drive symmetry change a critical step in developing future technologies that rely on such control. Topological materials, like…

The bulk photovoltaic effect is a photocurrent generation from alternating electric field, which is a promising candidate for future efficient solar cell technology. It is the second-order optical current, which is the injection current or…

Mesoscale and Nanoscale Physics · Physics 2025-05-22 Motohiko Ezawa

The photogalvanic effect (PGE) occurring in noncentrosymmetric materials enables the generation of a dc photocurrent at zero bias with a high polarization sensitivity, which makes it very attractive in photodetection. However, the magnitude…

Applied Physics · Physics 2021-06-28 Liyu Qian , Juan Zhao , Yiqun Xie

Weyl semimetals are crystals in which electron bands cross at isolated points in momentum space. Associated with each crossing point (or Weyl node) is an integer topological invariant known as the Berry monopole charge. The discovery of new…

Mesoscale and Nanoscale Physics · Physics 2020-07-28 Dylan Rees , Kaustuv Manna , Baozhu Lu , Takahiro Morimoto , Horst Borrmann , Claudia Felser , J. E. Moore , Darius H. Torchinsky , J. Orenstein

We employ first-principles calculations to investigate the ferroelectric properties and the bulk photovoltaic effect (BPVE) of antimony sulfur iodide (SbSI). The BPVE enables direct sunlight-to-electricity conversion in homogeneous…

Materials Science · Physics 2025-06-13 Giuseppe Cuono , Subhadeep Bandyopadhyay , Andrea Droghetti , Silvia Picozzi

Valleytronics that uses the inequivalent electronic states at the band extrema in semiconductors have been considered to play a vital role in the future information read/write technology. In the current work, we theoretically show that…

Materials Science · Physics 2023-06-07 Qianqian Xue , Xingchi Mu , Yan Sun , Jian Zhou

The circular photogalvanic effect (CPGE) is the photocurrent generated in an optically active material in response to an applied ac electric field, and it changes sign depending on the chirality of the incident circularly polarized light.…

Strongly Correlated Electrons · Physics 2020-06-03 Ipsita Mandal

Periodically driven systems provide tunable platforms to realize interesting Floquet topological phases and phase transitions. In electronic systems with Weyl dispersions, the band crossings are topologically protected even in the presence…

Mesoscale and Nanoscale Physics · Physics 2016-09-14 Ching-Kit Chan , Yun-Tak Oh , Jung Hoon Han , Patrick A. Lee

Bulk photovoltaic effect, which arises from crystal symmetry-driven charge carrier separation, is an intriguing physical phenomenon that has attracted extensive interest in photovoltaic application due to its junction-free photovoltaic and…

Materials Science · Physics 2023-08-22 Xiaojuan Chen , Kang Xu , Tingxiao Qin , Yubin Wang , Yuzhong Chen , Haiyun Liu , Qihua Xiong

In future solar cell technologies, the thermodynamic Shockley-Queisser limit for solar-to-current conversion in traditional p-n junctions could potentially be overcome with a bulk photovoltaic effect by creating an inversion broken symmetry…

We investigate the shift current bulk photovoltaic response of materials close to a band inversion topological phase transition. We find that the bulk photocurrent reverses direction across the band inversion transition, and that its…

Mesoscale and Nanoscale Physics · Physics 2016-09-08 Liang Z. Tan , Andrew M. Rappe

Anomalous local photocurrent generation via second-order nonlinear and thermoelectric responses is a signature of many topological semimetals. The emergence of these photocurrents is inherently linked to symmetry breaking and anisotropy of…

Q. Ma et al.[1] recently reported a strong photocurrent associated with charge neutrality in graphene devices with non-uniform geometries, which they interpreted as an intrinsic photoresponse enhanced by the momentum non-relaxing nature of…

Mesoscale and Nanoscale Physics · Physics 2020-02-26 Michael S. Fuhrer , Nikhil V. Medhekar