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The generation of high harmonics in laser-irradiated light homonuclear diatomics (H2+, N2 and O2) compared to that in atomic counterparts (of nearly identical binding energy) is studied within the velocity gauge version of conventional…

Atomic Physics · Physics 2009-11-11 Vladimir I. Usachenko , Pavel E. Pyak , Shih-I Chu

High harmonic generation (HHG) is an established means of producing coherent, short wavelength, ultrafast pulses from a compact set-up. Table-top high-harmonic sources are increasingly being used to image physical and biological systems…

In analogy with equilibrium phase transitions, we address the problem of the instability to symmetry-breaking perturbations of systems undergoing a laser transition. The symmetry in question is the $U(1)$ invariance with respect to a phase…

Mesoscale and Nanoscale Physics · Physics 2019-03-26 P. Gartner

We make a systematic study of high-order harmonic generation (HHG) in a He$^+$-like model ion when the initial states are prepared as a coherent superposition of the ground state and an excited state. It is found that, according to the…

Atomic Physics · Physics 2009-11-11 Bingbing Wang , Taiwang Cheng , Xiaofeng Li , Panming Fu , Shigang Chen , Jie Liu

We study numerically the Bloch electron wave-packet dynamics in periodic potentials to simulate laser-solid interactions. We introduce a quasi-classical model in the \emph{k} space combined with the energy band structure to understand the…

Optics · Physics 2017-01-05 Tao-Yuan Du , Xue-Bin Bian

The high-order harmonic generation (HHG), if phase matched, opens a unique way to produce coherent ultrafast extreme-UV (XUV) or soft x-ray light sources. Here we describe a robust and tunable method for scaling and narrowing the bandwidth…

Optics · Physics 2017-10-03 L. Mashhadi , G. Shayeganrad

High-order harmonic generation (HHG) is combined with resonant x-ray excitation of a core electron into the transient valence vacancy that is created in the course of the HHG process. To describe this setting, I develop a…

Atomic Physics · Physics 2015-10-15 Christian Buth

In our earlier work on harmonic generation with complex light [Nature Communications 15, 6878 (2024)], we demonstrated how the harmonic spectrum of a complex laser beam in a nonlinear medium can be obtained through the judicious application…

Optics · Physics 2025-11-17 Raoul Trines , Holger Schmitz , Martin King , Paul McKenna , Robert Bingham

High-harmonic generation (HHG) in solids has rapidly emerged as a promising platform for creating compact attosecond sources and probing ultrafast electron dynamics. Resonant metasurfaces are essential for enhancement of the otherwise small…

High-harmonic generation (HHG) of a two-level-system driven by an intense monochromatic phase-locked laser is studied in terms of complex spectral analysis with the Floquet method. In contrast to the phenomenological approaches, this…

Quantum Physics · Physics 2021-02-03 Hidemasa Yamane , Ken-ichi Noba , Tomio Petrosky , Satoshi Tanaka

High-harmonic generation (HHG) in solids has been touted as a way to probe ultrafast dynamics and crystal symmetries in condensed matter systems. Here, we investigate the polarization properties of high-order harmonics generated in…

Light generation through optical harmonics plays a pivotal role in photonics, driving innovations in coherent light sources, biological imaging, and spectroscopy. Traditional methods for tuning optical harmonics, including electrostatic…

Optics · Physics 2025-04-01 George Trivizas , Matthew D. Feinstein , Euclides Almeida

We present a comprehensive theoretical investigation of high-order harmonic generation in H$_2^+$ molecular ions within a quantum optical framework. Our study focuses on characterizing various quantum optical and quantum information…

This study presents an investigation of second harmonic generation (SHG) resulting from interaction of radially polarized laser beam propagating in homogeneous, unmagnetized plasma. Lorentz force and continuity equations have been used to…

Plasma Physics · Physics 2025-09-30 Shivani Aggarwal , Saumya Singh , Dinkar Mishra , Bhupesh Kumar , Pallavi Jha

We investigate high-order harmonic generation in inhomogeneous media for reduced dimensionality models. We perform a phase-space analysis, in which we identify specific features caused by the field inhomogeneity. We compute high-order…

Atomic Physics · Physics 2016-05-25 C. Zagoya , M. Bonner , H. Chomet , E. Slade , C. Figueira de Morisson Faria

The interaction of intense mid-infrared laser fields with atoms and molecules leads to a range of new opportunities, from the production of bright, coherent radiation in the soft x-ray range to imaging molecular structures and dynamics with…

High-order frequency mixing in graphene using a two-color radiation field consisting of the fundamental and the second harmonic fields of an ultrashort linearly polarized laser pulse is studied. It is shown that the harmonics originated…

Mesoscale and Nanoscale Physics · Physics 2022-05-25 Hamlet K. Avetissian , Garnik F. Mkrtchian , Andreas Knorr

Topological materials are of interest to both fundamental science and advanced technologies, because topological states are robust with respect to perturbations and dissipation. Experimental detection of topological invariants is thus in…

We generate high-order harmonics at high pulse repetition rates using a turnkey laser. High-order harmonics at 400 kHz are observed when argon is used as target gas. In neon we achieve generation of photons with energies exceeding 90 eV…

Using Time-Dependent Density Functional Theory (TDDFT) nonlinear nonperturbative response of the molecular system is studied for photoisomerization reaction. The 1,3-cyclohexadiene photoisomerization is probed by the high-harmonic…

Chemical Physics · Physics 2024-08-06 Lauren Bauerle , Agnieszka Jaron
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