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A consistent theory of electron energy-loss spectroscopy (EELS) includes two indispensable elements: (i) electronic response of the target system and (ii) quantum kinematics of probing electrons. While for the bulk materials and their…

Mesoscale and Nanoscale Physics · Physics 2017-12-12 Vladimir U. Nazarov , Vyacheslav M. Silkin , Eugene E. Krasovskii

In this work we perform electron energy-loss spectroscopy (EELS) of freestanding graphene with high energy and momentum resolution to disentangle the quasielastic scattering from the excitation gap of Dirac electrons close to the optical…

This work demonstrates electron energy loss spectroscopy of 2D materials in a 1-30 keV electron microscope, observing 100-times stronger electron-matter coupling relative to 125 keV microscopes. We observe that the universal curve relating…

Instrumentation and Detectors · Physics 2025-12-23 John W. Simonaitis , Joseph A. Alongi , Benjamin Slayton , William P. Putnam , Karl K. Berggren , Phillip D. Keathley

Recently, we have reported theoretical studies (J. Chem. Phys. 129, 054703, 2008 and J. Chem. Phys. 130, 086101, 2009) on the rate of energy transfer from an electronically excited molecule to graphene. It was found that graphene is a very…

Mesoscale and Nanoscale Physics · Physics 2011-04-18 R S Swathi , K L Sebastian

Strong nanoscale light-matter interaction is often accompanied by ultra-confined photonic modes and large momentum polaritons existing far beyond the light cone. A direct probe of such phenomena is difficult due to the momentum mismatch of…

The electric drift current bias was recently introduced as a new paradigm to break the Lorentz reciprocity in graphene. Here, we study the impact of the nonreciprocal response in the energy extracted from a beam of swift charges travelling…

Applied Physics · Physics 2019-12-10 Filipa R. Prudêncio , Mário G. Silveirinha

The unique optical properties of graphene, with broadband absorption and ultrafast response, make it a critical component of optoelectronic and spintronic devices. Using time-resolved momentum microscopy with high data rate and high dynamic…

We report angle-resolved electron transmission measurements through freestanding graphene sheets in the energy range of 18 to 30 eV above the Fermi level. The measurements are carried out in a low-energy electron point source microscope,…

Mesoscale and Nanoscale Physics · Physics 2016-08-19 Flavio Wicki , Jean-Nicolas Longchamp , Tatiana Latychevskaia , Conrad Escher , Hans-Werner Fink

The ab initio theory of electronic excitations in atomically thin [quasi-two-dimensional (Q2D)] crystals presents extra challenges in comparison to both the bulk and purely 2D cases. We argue that the conventionally used energy-loss…

Mesoscale and Nanoscale Physics · Physics 2015-07-16 Vladimir U. Nazarov

Analytic expressions for the absorption coefficient (AC) of a weak electromagnetic wave (EMW) in 2D Graphene under influence of strong laser radiation are calculated using the quantum kinetic equation (QKE) in the case of electron-optical…

Mesoscale and Nanoscale Physics · Physics 2024-12-24 Anh-Tuan Tran , Nguyen Dinh Nama , Nguyen Thi Thanh Nhan , Nguyen Quang Bau

The E12-14-012 experiment, performed in Jefferson Lab Hall A, has measured the (e,e'p) cross section in parallel kinematics using a natural titanium target. Here, we report the full results of the analysis of the data set corresponding to…

The finite momentum transfer ($\boldsymbol{q}$) longitudinal optical response $\sigma^L(\boldsymbol{q},\omega)$ of graphene has a peak at an energy $\omega=\hbar v_F q$. This corresponds directly to a quasiparticle peak in the spectral…

Mesoscale and Nanoscale Physics · Physics 2013-01-11 J. P. Carbotte , J. P. F. LeBlanc , Phillip E. C. Ashby

Van der Waals heterostructures made from atomically thin transition metal dichalcogenides (TMD) and graphene have emerged as a building block for optoelectronic devices. Such systems are also uniquely poised to investigate interfacial…

We develop a theory of momentum-resolved electron energy-loss spectra in the scanning transmission microscope (STEM-EELS) that captures the effects of coupled phonon and magnon excitations within a unified formalism, and apply it to…

We study quasi-particle transmission through an $n $-$p$ junction in a graphene irradiated by an electromagnetic field (EF). In the absence of EF the electronic spectrum of undoped graphene is gapless, and one may expect the perfect…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 M. V. Fistul , K. B. Efetov

Spectroscopies utilizing free electron beams as probes offer detailed information on the reciprocal-space excitations of 2D materials such as graphene and transition metal dichalcogenide monolayers. Yet, despite the attention paid to such…

Materials Science · Physics 2024-02-08 Andrew W. Rossi , Marc R. Bourgeois , Caleb Walton , David J. Masiello

The dynamic charge susceptibility, $\chi(q,\omega)$, is a fundamental observable of all materials, in one, two, and three dimensions, quantifying the collective charge modes, the ability of a material to screen charge, as well as its…

Strongly Correlated Electrons · Physics 2024-04-09 Peter Abbamonte , Jörg Fink

The near-field interaction between fluorescent emitters and graphene exhibits rich physics associated with local dipole-induced electromagnetic fields that are strongly enhanced due to the unique properties of graphene. Here, we measure…

Mesoscale and Nanoscale Physics · Physics 2013-07-08 L. Gaudreau , K. J. Tielrooij , G. E. D. K. Prawiroatmodjo , J. Osmond , F. J. Garcia de Abajo , F. H. L. Koppens

We present an accurate measurement and a quantitative analysis of electron-beam induced displacements of carbon atoms in single-layer graphene. We directly measure the atomic displacement ("knock-on") cross section by counting the lost…

We study the temperature-dependent corrections to the conductance due to electron-electron (e-e) interactions in clean two-dimensional conductors, such as lightly doped graphene or other Dirac matter. We use semiclassical Boltzmann kinetic…

Mesoscale and Nanoscale Physics · Physics 2018-08-01 A. Uzair , K. Sabeeh , Markus Mueller
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