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The phase diagram of Ca$_{2-x}$Sr$_x$RuO$_4$ has been studied by neutron diffraction on powder and single-crystalline samples. The experiments reveal antiferromagnetic order and structural distortions characterized by tilts and rotations of…

Superconductivity · Physics 2009-10-31 O. Friedt , M. Braden , G. Andre , P. Adelmann , S. Nakatsuji , Y. Maeno

We report a detailed examination the magnetic structure of anhydrous cupric chloride CuCl2 carried out by powder neutron diffraction, magnetic susceptibility and specific heat measurements on polycrystalline and single crystal samples as…

Strongly Correlated Electrons · Physics 2009-04-21 M. G. Banks , R. K. Kremer , C. Hoch , A. Simon , B. Ouladdiaf , J. -M. Broto , H. Rakoto , C. Lee , M. -H. Whangbo

We have studied the crystal structure and magnetic properties of the organic radical cation salt, BBDTA-InCl4. This material formed a one-dimensional coordination polymer, whose structure was characteristic of inorganic spin-Peierls…

Materials Science · Physics 2007-05-23 Wataru Fujita , Ryusuke Kondo , Seiichi Kagoshima , Kunio Awaga

Electron microscopy techniques are instrumental in the characterization of energy storage materials, with atomic resolution images providing the detailed structural features that are needed to understand their properties. Atomically…

Materials Science · Physics 2026-04-21 Ninon Scherz , Shashwat Anand , Colin Ophus , Tucker Holstun , Mary Scott , Tara P. Mishra , Gerbrand Ceder

The high-pressure synthesized quasi-one-dimensional compounds NaMn$_2$O$_4$ and Li$_{0.92}$Mn$_2$O$_4$ are both antiferromagnetic insulators, and here their atomic and magnetic structures were investigated using neutron powder diffraction.…

The term sample dependence describes the troublesome tendency of nominally equivalent samples to exhibit different physical properties. High entropy oxides (HEOs) are a class of materials where sample dependence has the potential to be…

The calculation of magnetic anisotropy constants is performed beyond the point charge model for a continuous charge density distribution of screening conduction electrons. An important role of the non-uniform electron density, in…

Condensed Matter · Physics 2009-10-31 V. Yu. Irkhin , Yu. P. Irkhin

Local configurational disorder can have a dominating role in the formation of macroscopic functional responses in strongly correlated materials. Here, we use entropy-stabilization synthesis to create single crystal epitaxial ABO3 perovskite…

We have employed first-principles electronic structure calculations to examine the hypothetical (but plausible) oxide spinel, LiCr2O4 with the d^{2.5} electronic configuration. The cell (cubic) and internal (oxygen position) structural…

Materials Science · Physics 2009-11-10 Markus Lauer , Roser Valenti , H. C. Kandpal , Ram Seshadri , .

The impurity paramagnetic ion, $Cu^{2+}$ substitutes $Al$ in the $SrLaAlO_4$ single crystal lattice, this results in a $CuO_6$ elongated octahedron, the resulting measured g-factors shows four-fold axes variation condition. The aggregate…

Quantum Physics · Physics 2024-03-26 M. A. Hosain , J. -M. Le Floch , J. Krupka , M. E. Tobar

The A-site spinel material, CoAl2O4, is a physical realization of the frustrated diamond-lattice antiferromagnet, a model in which is predicted to contain unique incommensurate or `spin-spiral liquid' ground states. Our previous…

The magnetic properties of metal-organic complexes are strongly influenced by conformational changes in the ligand. The flexibility of Fe-tetra-pyridyl-porphyrin molecules leads to different adsorption configurations on a Au(111) surface.…

Mesoscale and Nanoscale Physics · Physics 2018-11-06 Daniela Rolf , Christian Lotze , Constantin Czekelius , Benjamin W. Heinrich , Katharina J. Franke

We have investigated the structural, magnetic, thermodynamic, and dielectric properties of polycrystalline CoCr$_2$O$_4$, an insulating spinel exhibiting both ferrimagnetic and spiral magnetic structures. Below $T_c$ = 94 K the sample…

Materials Science · Physics 2007-05-23 G. Lawes , B. Melot , K. Page , C. Ederer , M. A. Hayward , Th. Proffen , R. Seshadri

We report the magnetic properties of $A$-site spinel compound MnSc$_2$Se$_4$. The macroscopic magnetic measurements uncovers successive magnetic transitions at $T_{\rm{N1}}$= 2.04 K, followed by two further transitions at $T_{\rm{N2}}$=1.8…

Strongly Correlated Electrons · Physics 2022-06-01 K. Guratinder , V. Tsurkan , L. Prodan , L. Keller , J. P. Embs , F. Juranyi , M. Medarde , Ch. Rüegg , O. Zaharko

Spin-frustrated systems are one avenue for inducing macroscopic quantum states in materials. However, experimental realization of this goal has been difficult because of the lack of simple materials and, if available, the separation of the…

Strongly Correlated Electrons · Physics 2010-04-07 S. Chu , T. M. McQueen , R. Chisnell , D. E. Freedman , P. Müller , Y. S. Lee , D. G. Nocera

Stabilization of unusual spin-orbit driven magnetic orderings are achieved for chains of Mn atoms deposited on a W(110) substrate. First-principles electronic structure calculations show that the ground state spin configuration is…

The complex metal oxides Mn2ASbO6 (A=In, Sc) with a corundum-related structure A3BO6 have been prepared as polycrystalline powders by a solid state reaction route. The crystal structure and magnetic properties have been investigated using a…

Materials Science · Physics 2011-11-21 S. A. Ivanov , P. Nordblad , R. Mathieu , R. Tellgren , E. Politova , G. André

Neutron diffraction measurement on the spin glass double perovskite Sr$_2$FeCoO$_6$ reveals site disorder as well as Co$^{3+}$ intermediate spin state. In addition, multiple valence states of Fe and Co are confirmed through M\"{o}ssbauer…

Strongly Correlated Electrons · Physics 2015-06-05 R. Pradheesh , Harikrishnan S. Nair , V. Sankaranarayanan , K. Sethupat

KCrF3 represents another prototypical orbital-ordered perovskite, where Cr2+ possesses the same electronic configuration of 3d4 as that of strongly Jahn-Teller distorted Mn3+ in many CMR manganites. The crystal and magnetic structures of…

Strongly Correlated Electrons · Physics 2013-09-30 Y. Xiao , Y. Su , H. -F. Li , C. M. N. Kumar , R. Mittal , J. Persson , A. Senyshyn , K. Gross , Th. Brueckel

The S=1/2 Heisenberg spin chain compound SrCuO2 doped with different amounts of nickel (Ni), palladium (Pd), zinc (Zn) and cobalt (Co) has been studied by means of Cu nuclear magnetic resonance (NMR). Replacing only a few of the S=1/2 Cu…