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CuCrP$_2$S$_6$ (CCPS), a type-II multiferroic material, exhibits unique phase transitions involving ferroelectric, antiferroelectric, and antiferromagnetic ordering. In this study, we conduct a comprehensive investigation on the intricate…

The crystallographic and magnetic properties of the cleavable 4d3 transition metal compound a-MoCl3 are reported, with a focus on the behavior above room temperature. Crystals were grown by chemical vapor transport and characterized using…

We present a comprehensive $^{31}$P and $^{65}$Cu nuclear magnetic resonance (NMR) study of the layered van der Waals magnet CuCrP$_2$S$_6$. The compound exhibits a sequence of structural and magnetic phase transitions: a high-temperature…

Strongly Correlated Electrons · Physics 2026-04-06 C. S. Saramgi , L. F. Prager , S. Selter , Y. Shemerliuk , S. Aswartham , B. Büchner , H. -J. Grafe , K. M. Ranjith

The magnetic, dielectric and structural properties of type-I multiferroic KNiPO$_4$ have been investigated by neutron powder diffraction, magnetization, dielectric and high temperature synchrotron-XRD measurements. Below the N\'{e}el…

Strongly Correlated Electrons · Physics 2022-07-15 Alexandre Pages , Jian-Rui Soh , Marjaneh Jafari Fesharaki , Henrik M. Ronnow , Hossein Ahmadvand

We report on optical measurements of the 1D Heisenberg antiferromagnet KCuF3. The crystal-field excitations of the Cu2+ ions have been observed and their temperature dependence can be understood in terms of magnetic and exchange-induced…

Strongly Correlated Electrons · Physics 2009-11-13 J. Deisenhofer , I. Leonov , M. V. Eremin , Ch. Kant , P. Ghigna , F. Mayr , V. V. Iglamov , V. I. Anisimov , D. van der Marell

Unusual magnetic properties of Van der Waals type antiferromagnetic semiconductors make them highly attractive for spintronics and optoelectronics. A link between the magnetic and optical properties of those materials, required for…

Layered magnetic materials potentially hold the key to future applications based on optical control and manipulation of magnetism. NiPS3, a prototype member of this family, is antiferromagnetic below 155 K and exhibits sharp…

We study magneto-transport in heterostructures composed of the van der Waals antiferromagnet CrPS$_{4}$ and the heavy metals Pt and Pd. The transverse resistance (R$_{xy}$) signal reveals the spin-flop transition of CrPS$_{4}$ and a…

Quantum interference gives rise to the asymmetric Fano resonance line shape when the final states of an electronic transition follows within a continuum of states and a discrete state, which has significant applications in optical switching…

Materials Science · Physics 2019-10-14 Pingfan Gu , Qinghai Tan , Yi Wan , Ziling Li , Yuxuan Peng , Jiawei Lai , Junchao Ma , Xiaohan Yao , Kai Yuan , Dong Sun , Bo Peng , Jun Zhang , Yu Ye

The behavior of 2-dimensional (2D) van der Waals (vdW) layered magnetic materials in the 2D limit of the few-layer thickness is an important fundamental issue for the understanding of the magnetic ordering in lower dimensions. The…

Materials Science · Physics 2020-12-02 Soo Yeon Lim , Kangwon Kim , Sungmin Lee , Je-Geun Park , Hyeonsik Cheong

Strong coupling between optical and magnetic excitations could enable contactless, spatially resolved, or ultrafast interrogation and control of magnetism in two-dimensional (2D) materials and devices. The layered 2D A-type antiferromagnet…

Materials Science · Physics 2026-03-27 Jacob T. Baillie , Eden Tzanetopoulos , Rachel T. Smith , Remi Beaulac , Daniel R. Gamelin

The Van der Waals semiconductor metamagnet CrSBr offers an ideal platform for studying the interplay between optical and magnetic properties in the two-dimensional limit. Here, we carried out an exhaustive optical characterization of this…

Type-II multiferroics, where spin interactions induce a ferroelectric polarization, are interesting for new device functionalities due to large magnetoelectric coupling. We report on a new type of multiferroicity in the quadruple-perovskite…

The crystalline and optical anisotropy of low-symmetry two-dimensional (2D) materials can enable strong dichroic responses, enhancing polarization contrast for photonic and optoelectronic devices. Here, we unveil pronounced optical and…

Mesoscale and Nanoscale Physics · Physics 2026-05-18 Cédric A. Cordero-Silis , Daniel Vaquero , Teresa López-Carrasco , Harshan Madeshwaran , Marcos H. D. Guimarães

The ternary van der Waals material NbIrTe$_4$ is a Type-II Weyl semimetal. We use a tunable circularly polarized mid-infrared laser to investigate the existence of band-to-band excitations using transient reflectivity in an exfoliated…

Materials Science · Physics 2022-01-03 Seyyedesadaf Pournia , Giriraj Jnawali , Samuel Linser , Howard E. Jackson , Leigh M. Smith

Changes in the spin configuration of atomically-thin, magnetic van-der-Waals multilayers can cause drastic modifications in their opto-electronic properties. Conversely, the opto-electronic response of these systems provides information…

Mesoscale and Nanoscale Physics · Physics 2020-05-28 Zhe Wang , Marco Gibertini , Dumitru Dumcenco , Takashi Taniguchi , Kenji Watanabe , Enrico Giannini , Alberto F. Morpurgo

BaMF4 (M=Fe, Co, Ni and Mn) family are typical multiferroic materials, having antiferromagnetism at around liquid nitrogen temperature. In this work, polycrystalline BaFeF4 has been prepared by solid state reaction. The slight deficiency of…

Hexagonal YMnO$_3$ is well known for the co-occurrence of ferroelectricity and antiferromagnetism at low temperatures. Using temperature-dependent spectroscopic ellipsometry at an $a$-plane oriented single crystal, we show how the…

Materials Science · Physics 2015-03-16 Steffen Richter , Stefan G. Ebbinghaus , Marius Grundmann , Rüdiger Schmidt-Grund

The van der Waals antiferromagnet CrSBr exhibits coupling of vibrational, electronic, and magnetic degrees of freedom, giving rise to distinctive quasi-particle interactions. We investigate these interactions across a wide temperature range…

Layered magnetic materials are becoming a major platform for future spin-based applications. Particularly the air-stable van der Waals compound CrSBr is attracting considerable interest due to its prominent magneto-transport and…

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