English
Related papers

Related papers: Time-dependent convergent close coupling method fo…

200 papers

Double ionization of diatomic molecules by short linearly polarized laser pulses is analyzed. We consider the final stage of the ionization process, that is the decay of a highly excited two electron molecule, which is formed after…

Atomic Physics · Physics 2016-09-08 Jakub S. Prauzner-Bechcicki , Krzysztof Sacha , Bruno Eckhardt , Jakub Zakrzewski

We present an embedding approach to treat local electron correlation effects in periodic environments. In a single, consistent framework, our plane-wave based scheme embeds a local high-level correlation calculation (here Coupled Cluster…

Chemical Physics · Physics 2021-01-07 Tobias Schäfer , Florian Libisch , Georg Kresse , Andreas Grüneis

The process of ionization of a hydrogen atom by a short infrared laser pulse is studied in the regime of very large pulse intensity, in the dipole approximation. Let $A$ denote the integral of the electric field of the pulse over time at…

Mathematical Physics · Physics 2015-05-18 Juerg Froehlich , Alessandro Pizzo , Benjamin Schlein

Two-color laser fields offer significantly enhanced control over electron excitation dynamics under ultrashort intense laser pulses compared to monochromatic fields. However, their strong nonlinearity necessitates computationally expensive…

Optics · Physics 2025-07-03 Mizuki Tani , Kenichi L. Ishikawa , Tomohito Otobe

We investigate the time-evolution of quantum entanglement between an electron, liberated by a strong few-cycle laser pulse, and its parent ion-core. Since the standard procedure is numerically prohibitive in this case, we propose a novel…

Quantum Physics · Physics 2017-10-18 Szilárd Majorosi , Mihály G. Benedict , Attila Czirják

In parallel with the evolution of femtosecond and attosecond laser as well as free-electron laser technology, a variety of theoretical methods have been developed to describe the behavior of atoms, molecules, clusters, and solids under the…

Atomic Physics · Physics 2015-11-12 Kenichi L. Ishikawa , Takeshi Sato

We review different computational methods for the calculation of photoelectron spectra and angular distributions of atoms and molecules when excited by laser pulses using time-dependent density-functional theory (TDDFT) that are suitable…

Chemical Physics · Physics 2017-03-28 Philipp Wopperer , Umberto De Giovannini , Angel Rubio

Strong field photoemission and electron recollision provide a viable route to extract electronic and nuclear dynamics from molecular targets with attosecond temporal resolution. However, since an {\em ab-initio} treatment of even the…

Atomic Physics · Physics 2016-11-02 N. Suárez , A. Chacón , M. F. Ciappina , B. Wolter , J. Biegert , M. Lewenstein

Few-cycle pulses of intense 800 nm light are used to probe ionization and dissociation of carbon disulfide in the intensity and temporal regime where rescattering is expected to dominate the laser-molecule interaction. The wavepacket of the…

Real-time coupled cluster (CC) methods have several advantages over their frequency-domain counterparts, namely, response and equation of motion CC theories. Broadband spectra, strong fields, and pulse manipulation allow for the simulation…

Chemical Physics · Physics 2023-08-04 Benjamin G. Peyton , Zhe Wang , T. Daniel Crawford

We explore and develop the mathematics of the two multi-level ions. In particular, we describe some new features of quantum entanglement in two three-level trapped ions confined in a one-dimensional harmonic potential, allowing the…

Quantum Physics · Physics 2009-11-13 Mahmoud Abdel-Aty , Ting Yu

We revisit a recently proposed scheme [M.F. Ciappina et al 2019 Phys. Rev. A 99 043405] for accurate measurement of electromagnetic radiation intensities in a focus of high-power laser beams. The method is based on the observation of…

Atomic Physics · Physics 2020-02-19 M. F. Ciappina , S. V. Popruzhenko

Ionization is critical in the formation and evolution of plasma dynamics; collisional ionization, in particular, is an often overlooked source of electrons when dealing with laser-plasma interactions. Ionization plays a crucial role in…

Plasma Physics · Physics 2026-03-19 Stephen DiIorio , Ricardo Fonseca , Frank Tsung , Benjamin J. Winjum , Alec G. R. Thomas

An efficient numerical algorithm for the laser driven multi-level ionization of high-atomic-number gases is proposed and implemented in an electromagnetic particle-in-cell code SPACE. The algorithm is based on analytical solutions to the…

Plasma Physics · Physics 2022-02-23 Aiqi Cheng , Roman Samulyak

External electric fields are highly attractive for dynamical manipulation of excitons in two-dimensional materials. Here, we theoretically study the ionization of excitons in monolayer transition metal dichalcogenides (TMDs) by intense…

Materials Science · Physics 2022-01-05 Høgni C. Kamban , Thomas G. Pedersen

Ionization rates and Stark shifts of H$_2$, CO, O$_2$, H$_2$O, and CH$_4$ in static electric fields have been computed with coupled-cluster methods in a basis set of atom-centered Gaussian functions with complex-scaled exponent.…

Chemical Physics · Physics 2018-06-13 Thomas-C. Jagau

The Jaynes-Cummings (JC) model stands as a fully quantized, fundamental framework for exploring light-matter interactions, a timely reflection on a century of quantum theory. The time-dependent Jaynes-Cummings (TDJC) model introduces…

We have developed a new time propagation method, time-dependent adaptive sampling configuration interaction (TD-ASCI), to describe the dynamics of a strongly correlated system. We employ the short iterative Lanczos (SIL) method as the…

Chemical Physics · Physics 2025-06-23 Avijit Shee , Zhen Huang , Martin Head-Gordon , K. Birgitta Whaley

A theoretical comparison of the electronic excitation and ionisation behaviour of molecular hydrogen oriented either parallel or perpendicular to a linear polarised laser pulse is performed. The investigation is based on a non-perturbative…

Quantum Physics · Physics 2009-11-13 Yulian V. Vanne , Alejandro Saenz

Critical coagulation concentration (CCC) is a key parameter of particle dispersions, since it provides the threshold limit of electrolyte concentrations, above which the dispersions are destabilized due to rapid particle aggregation. A…

Soft Condensed Matter · Physics 2020-06-08 Marco Galli , Szilard Saringer , Istvan Szilagyi , Gregor Trefalt