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Laser spectroscopic studies on minute samples of exotic radioactive nuclei require very efficient experimental techniques. In addition, high resolving powers are required to allow extraction of nu- clear structure information. Here we…
Molecules containing short-lived isotopes, namely radioactive molecules, are among the most promising candidates for probing new physics beyond the Standard Model, although their production and spectroscopic measurements remain technically…
Two-dimensional (2D) spectroscopy combines high temporal and spectral resolution, allowing the observation of ultrafast energy transfer and the separation of homogeneous and inhomogeneous broadening. Typically, 2D spectroscopy is dominated…
We have measured hyperfine structure in the first-excited $P$ state ($D$ lines) of all the naturally-occurring alkali atoms. We use high-resolution laser spectroscopy to resolve hyperfine transitions, and measure intervals by locking the…
Spectral analysis is one of the most powerful technologies for studying and understanding matter. As the devices for spectral analysis, spectrometers are widely used in material detection, isotope analysis, trace gas detection, and the…
Hyperfine-structures of highly charged ions (HCIs) are favourable spectroscopic targets for exploring fundamental physics as well as nuclear properties. Recent proposals of HCI atomic clocks highlight their importance, especially for…
We have constructed a collinear laser spectroscopy (CLS) system installed at the Beijing Radioactive Ion-beam Facility (BRIF), aiming to investigate the nuclear properties of unstable nuclei. The first on-line commissioning experiment of…
Femtosecond interferometry combined with acousto-optical phase modulation is an effective approach to implement various types of coherent nonlinear and multidimensional spectroscopy schemes. The high sensitivity of this method has recently…
Transition frequencies and fine-structure splittings of the $2\,{}^3\!S_1 \rightarrow 2\,{}^3\!P_{\!J}$ transitions in helium-like $^{12}\mathrm{C}^{4+}$ were measured by collinear laser spectroscopy on a 1-ppb level. Accuracy is increased…
Ultrafast lasers have become one of the most powerful tools in coherent nonlinear optical spectroscopy. Short pulses enable direct observation of fast molecular dynamics, whereas broad spectral bandwidth offers ways of controlling nonlinear…
Hyperfine structure $A$ and $B$ factors of the atomic $5s\,5p\,\; ^3\rm{P}_2 \rightarrow 5s\,6s\,\; ^3\rm{S}_1$ transition are determined from collinear laser spectroscopy data of $^{107-123}$Cd and $^{111m-123m}$Cd. Nuclear magnetic…
An approach to determine the kinetic beam energy at the $10^{-5}$ level is presented, which corresponds to an improvement by more than one order of magnitude compared to conventional methods. Particularly, collinear fluorescence and…
In proton therapy, depth scanning of the irradiated object is performed by changing the Output Energy (OE) of the accelerated beam. In pulsed linear accelerators, adjustment of the OE is usually by changing the amplitude and/or phase of the…
Long-lived isotopes of plutonium were studied using two complementary techniques, high-resolution resonance ionisation spectroscopy (HR-RIS) and collinear laser spectroscopy (CLS). Isotope shifts have been measured on the $5f^67s^2\ ^7F_0…
Recent and upcoming stabilized spectrographs are pushing the frontier for Doppler spectroscopy to detect and characterize low-mass planets. Specifications for these instruments are so impressive that intrinsic stellar variability is…
Nonlinear spectroscopy employs a series of laser pulses to interrogate dynamics in large interacting many-body systems, and has become a highly successful method for experiments in chemical physics. Current quantum optical experiments…
Laser frequency combs (LFCs) are an important component of Doppler radial velocity (RV) spectroscopy that pushes fractional precision to the $10^{-10}$ level, as required to identify and characterize Earth-like exoplanets. However, large…
Skimmed supersonic beams provide intense, cold, collision-free samples of atoms and molecules are one of the most widely used tools in atomic and molecular laser spectroscopy. High-resolution optical spectra are typically recorded in a…
We explore the radial velocity performance benefits of coupling starlight to a fast-scanning interferometer and a fast-readout spectrometer with zero readout noise. By rapidly scanning an interferometer we can decouple wavelength…
The local interaction of charges and light in organic solids is the basis of distinct and fundamental effects. We here observe, at the single molecule scale, how a focused laser beam can locally shift by hundreds-time their natural…