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The success of non-linear optics relies largely on pulse-to-pulse consistency. In contrast, covariance based techniques used in photoionization electron spectroscopy and mass spectrometry have shown that wealth of information can be…
Accurate calculations of the fine and hyperfine splitting of the 2P state in Li and Be$^+$ isotopes using the explicitly correlated Hylleraas basis set are presented. Theoretical predictions including the mixing of $P_{1/2}$ and $P_{3/2}$…
We demonstrate a high-stability laser offset-frequency locking technique based on a balanced filter discriminator. The beat note between two 852 nm external-cavity diode lasers is down-converted in two parallel arms using local-oscillator…
Split-pulse x-ray photon correlation spectroscopy has been proposed as one of the unique capabilities made possible with the x-ray free electron lasers. It enables characterization of atomic scale structural dynamics that dictates the…
We propose to use local electromagnetic noise spectroscopy as a versatile and noninvasive tool to study Wigner crystal phases of strongly-interacting two-dimensional electronic systems. In-plane imaging of the local noise is predicted to…
A new method for high-sensitivity subwavelength spectromicroscopy is proposed based on the usage of a spaser (near-field laser) in the form of a scanning probe microscope tip. The high spatial resolution is defined by the tip's curvature,…
We present an experimental technique for realizing a specific absorption spectral pattern in a rare-earth-doped crystal at cryogenic temperatures. This pattern is subsequently probed on two spectral channels simultaneously, thereby…
Methods are studied to compute the boosting effects produced by the observer motion that modifies and transfers to higher l the isotropic monopole frequency spectrum of the cosmic background. Explicit analytical solutions for spherical…
Noise measurement is a powerful tool to investigate many phenomena from laser characterization to quantum behavior of light. In this paper, we report on intensity noise measurements obtained when a laser beam is transmitted through a large…
We demonstrate a technique for precisely measuring hyperfine intervals in alkali atoms. The atoms form a three-level $\Lambda$ system in the presence of a strong control laser and a weak probe laser. The dressed states created by the…
Ultrafast lasers ($< 500$ fs) have enabled laser-matter interactions at intensities exceeding $10^{18} \rm{Wcm}^{-2}$ with only millijoules of laser energy. However, as pulse durations become shorter, larger spectral bandwidths are…
Today, wide-open, high-resolution Doppler frequency shift (DFS) estimation is essential for radar, microwave/millimeter-wave, and communication systems. Using photonics technology, an effective approach is proposed and experimentally…
Large-amplitude molecular motions which occur during isomerization can cause significant changes in electronic structure. These variations in electronic properties can be used to identify vibrationally-excited eigenstates which are…
Attosecond metrology sensitive to sub-optical-cycle electronic and structural dynamics is opening up new avenues for ultrafast spectroscopy of condensed matter. Using intense lightwaves to precisely control the extremely fast carrier…
We report a measurement of the hyperfine-structure constants of the $^{85}$Rb 4$D_{3/2}$ state using a two-photon 5$S_{1/2}\rightarrow$4$D_{3/2}$ transition. The hyperfine transitions are probed by measuring the transmission of the…
The resolution limits of classical spectroscopy can be surpassed by quantum-inspired methods leveraging the information contained in the phase of the complex electromagnetic field. Their counterpart in spatial imaging has been widely…
Broadband precision spectroscopy is indispensable for providing high fidelity molecular parameters for spectroscopic databases. We have recently shown that mechanical Fourier transform spectrometers based on optical frequency combs can…
We discuss layout and performance of a high-resolution Stimulated Raman Loss spectrometer that has been newly developed for accurate studies of spectral lineshapes and line center frequencies of hydrogen isotopologues and in general of…
Time-Of-Flight (TOF) methods are very effective to detect particles accelerated in laser-plasma interactions, but they shows significant limitations when used in experiments with high energy and intensity lasers, where both high-energy ions…
Rapid progress in cooling and trapping of molecules has enabled first experiments on high resolution spectroscopy of trapped diatomic molecules, promising unprecedented precision. Extending this work to polyatomic molecules provides unique…