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We report synthesis of polycrystalline samples of the recently discovered spin liquid material Ca$_{10}$Cr$_7$O$_{28}$ and present measurements of the ambient and high pressure magnetic susceptibility $\chi$ versus temperature $T$,…

Strongly Correlated Electrons · Physics 2017-07-20 Ashiwini Balodhi , Yogesh Singh

The search for novel phases of matter is a central theme of modern physics, with some of the most intriguing examples provided by the spin liquids found in magnets with competing, or "frustrated" interactions. Ca$_{10}$Cr$_7$O$_{28}$, a…

Strongly Correlated Electrons · Physics 2025-04-11 Rico Pohle , Han Yan , Nic Shannon

Spiral spin liquids are unique classical spin liquids that occur in many frustrated spin systems, but do not comprise a new phase of matter. Owing to extensive classical ground-state degeneracy, the spins in a spiral spin liquid thermally…

Strongly Correlated Electrons · Physics 2021-06-01 Xu-Ping Yao , Jian Qiao Liu , Chun-Jiong Huang , Xiaoqun Wang , Gang Chen

Quantum spin liquids are long-range entangled states of matter with emergent gauge fields and fractionalized excitations. While candidate materials, such as the Kitaev honeycomb ruthenate $\alpha$-RuCl$_3$, show magnetic order at low…

Strongly Correlated Electrons · Physics 2019-07-16 I. Rousochatzakis , S. Kourtis , J. Knolle , R. Moessner , N. B. Perkins

Spin noise spectroscopy is emerging as a powerful technique for studying the dynamics of various spin systems also beyond their thermal equilibrium and linear response. Here, we study spin fluctuations of room-temperature neutral atoms in a…

Atomic Physics · Physics 2021-07-21 V. Guarrera , R. Gartman , G. Bevilacqua , W. Chalupczak

A spin liquid is a new state of matter with topological order where the spin moments continue to fluctuate coherently down to the lowest temperatures rather than develop static long-range magnetic order as found in conventional magnets. For…

Ca$_{10}$Cr$_7$O$_{28}$ is a novel spin-$1/2$ magnet exhibiting spin liquid behaviour which sets it apart from any previously studied model or material. However, understanding Ca$_{10}$Cr$_7$O$_{28}$ presents a significant challenge,…

Strongly Correlated Electrons · Physics 2021-07-28 Rico Pohle , Han Yan , Nic Shannon

We present new experimental low-temperature heat capacity and detailed dynamical spin-structure factor data for the quantum spin liquid candidate material Ca$_{10}$Cr$_7$O$_{28}$. The measured heat capacity shows an almost perfect linear…

Most materials freeze when cooled to sufficiently low temperature. We find that magnetic dipoles randomly distributed in a solid matrix condense into a spin liquid with spectral properties on cooling that are the diametric opposite of those…

Condensed Matter · Physics 2009-11-10 S. Ghosh , R. Parthasarathy , T. F. Rosenbaum , G. Aeppli

We identify the low energy effective Hamiltonian that is expected to describe the low temperature properties of the frustrated magnet $\mathrm{Ca}_{10}\mathrm{Cr}_{7}\mathrm{O}_{28}$. Motivated by the fact that this effective Hamiltonian…

Strongly Correlated Electrons · Physics 2018-03-07 Sounak Biswas , Kedar Damle

We report gapless quantum spin liquid behavior in the layered triangular Sr$_{3}$CuSb$_{2}$O$_{9}$ (SCSO) system. X-ray diffraction shows superlattice reflections associated with atomic site ordering into triangular Cu planes well-separated…

While the spin dynamics of La$_{0.7}$Ca$_{0.3}$MnO$_3$ in the ferromagnetic phase are known to be unconventional, previous measurements have yielded contradictory results regarding the damping of spin wave excitations. Neutron spectroscopy…

Strongly Correlated Electrons · Physics 2017-09-18 Joel S. Helton , Susumu K. Jones , Daniel Parshall , Matthew B. Stone , Dmitry A. Shulyatev , Jeffrey W. Lynn

The existence of a quantum spin liquid (QSL) in which quantum fluctuations of spins are sufficiently strong to preclude spin ordering down to zero temperature was originally proposed theoretically more than 40 years ago, but its…

Quantum spin liquids are highly entangled ground states of quantum systems with emergent gauge structure, fractionalized spinon excitations, and other unusual properties. While these features clearly distinguish quantum spin liquids from…

Strongly Correlated Electrons · Physics 2013-06-18 Lucile Savary , Leon Balents

Experimental identification of quantum spin liquids remains a challenge, as the pristine nature is to be seen in asymptotically low temperatures. We here theoretically show that the precursor of quantum spin liquids appears in the spin…

Strongly Correlated Electrons · Physics 2016-10-12 Junki Yoshitake , Joji Nasu , Yukitoshi Motome

Magnetization noise measurements on the spin ice Dy${}_2$Ti${}_2$O${}_7$ have revealed a remarkable `pink noise' power spectrum $S(f,T)$ below 4 K, including evidence of magnetic monopole excitations diffusing in a fractal landscape.…

Strongly Correlated Electrons · Physics 2026-05-06 D. Billington , E. Riordan , C. Cafolla-Ward , J. Wilson , E. Lhotel , C. Paulsen , D. Prabhakaran , S. T. Bramwell , F. Flicker , S. R. Giblin

Neutron scattering experiments on a polycrystalline sample of the frustrated pyrochlore magnet Tb2Ti2O7, which does not show any magnetic order down to 50 mK, have revealed that it shows condensation behavior below 0.4 K from a thermally…

Disordered Systems and Neural Networks · Physics 2011-12-13 Hiroshi Takatsu , Hiroaki Kadowaki , Taku J. Sato , Jeffrey W. Lynn , Yoshikazu Tabata , Teruo Yamazaki , Kazuyuki Matsuhira

We report the observation of a frequency ($\omega $) and temperature (T) -dependent loss peak in $\chi''$ and accompanying dispersion in $\chi'$ from microwave (2-18GHz) measurements of the complex susceptibility $\tilde{\chi}(\omega,…

Strongly Correlated Electrons · Physics 2007-05-23 Z. Zhai , P. V. Patanjali , N. Hakim , J. B. Sokoloff , S. Sridhar , U. Ammerahl , A. Vietkine , A. Revcolevschi

Quantum fluctuations are expected to lead to highly entangled spin-liquid states in certain two-dimensional spin-1/2 compounds. We have synthesized and measured thermodynamic properties and muon spin relaxation rates in the copper-based…

The intrinsic fluctuations of electron spins in semiconductors and atomic vapors generate a small, randomly-varying "spin noise" that can be detected by sensitive optical methods such as Faraday rotation. Recent studies have demonstrated…

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