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Transient absorption is a very powerful observable in attosecond experiments on atoms, molecules and solids and is frequently used in experiments employing phase-locked few-cycle infrared and XUV laser pulses derived from high harmonic…

Atomic Physics · Physics 2020-08-26 Lorenz Drescher , Marc J. J. Vrakking , Jochen Mikosch

An intuitive physical mechanism for single attosecond pulse generation in multi-cycle pulse regime is proposed. We suggest that the continuum spectra of HHG can be controlled through the modulation of carrier wave, while keeping the…

Optics · Physics 2011-11-01 Xiang Yang , Yueping Niu , Shangqing Gong

Raman amplification in plasma has been promoted as a means of compressing picosecond optical laser pulses to femtosecond duration to explore the intensity frontier. Here we show for the first time that it can be used, with equal success, to…

Plasma Physics · Physics 2015-05-27 R. Trines , F. Fiuza , R. Bingham , R. A. Fonseca , L. O. Silva , R. A. Cairns , P. A. Norreys

In this work, we demonstrate post-compression of 1.2 picosecond laser pulses to 13 fs via gas-based multi-pass spectral broadening. Our results yield a single-stage compression factor of about 40 at 200 W in-burst average power and a total…

Ultrashort electron pulses with a high average current provide a powerful means of enhancing time-resolved imaging and photon generation. In this study, we report the attosecond shaping of sub-relativistic electron beams using membranes in…

We propose a novel scheme to generate single-cycle terahertz (THz) pulses via reflection of an optical femtosecond pulse train from a thin layer of nonlinear resonant medium. Our method is based on a coherent control of low-frequency…

The availability of electromagnetic pulses with controllable field waveform and extremely short duration, even below a single optical cycle, is imperative to fully harness strong-field processes and to gain insight into ultrafast…

The use of laser pulse sequences to drive the cascaded difference frequency generation of high energy, high peak-power and multi-cycle terahertz pulses in cryogenically cooled periodically poled lithium niobate is proposed. Detailed…

Optics · Physics 2016-10-27 Koustuban Ravi , Damian N. Schimpf , Franz X. Kärtner

The generation of the shortest isolated attosecond pulses requires both broad spectral bandwidth and control of the spectral phase. Rapid progress has been made in both aspects, leading to the generation of the world-record-shortest 67 as…

Optics · Physics 2013-12-06 Michael Chini , Kun Zhao , Zenghu Chang

We demonstrate compression and shaping of few cycle pulses from a high average power Ytterbium laser system. The pulses from a commercial 20 W, 100 kHz Yb laser system are spectrally broadened in two-stages using gas-filled, stretched…

This article demonstrates a new compression scheme that has the potential to compress a high energy pulse as high as a few hundred Joules in a pulse as short as one optical cycle at 0.8{\mu}m making a true ultra-relativistic {\lambda}^3…

Optics · Physics 2015-06-18 G. Mourou , S. Mironov , E. Khazanov , A. Sergeev

We present an interferometric pump-probe technique for the characterization of attosecond electron wave packets (WPs) that uses a free WP as a reference to measure a bound WP. We demonstrate our method by exciting helium atoms using an…

Attosecond electron pulses enable real-time probing of ultrafast matter dynamics, yet conventional modulation schemes suffer from drastically shortened longitudinal focal lengths when targeting sub-attosecond durations. To address this…

Plasma Physics · Physics 2026-05-15 Qi Huang , Qing Jia , Zhongxuan Wang , Jian Zheng

In multi-dimensional time-resolved spectroscopic experiments, multiple (more than two) short laser pulses with variable pulse delay times are employed for the time-resolved exploration of the photoinduced dynamics of molecular chromophores.…

Chemical Physics · Physics 2026-03-25 Sebastian V. Pios , Maxim F. Gelin , Wolfgang Domcke , Lipeng Chen

The short wavelength and high peak power of the present generation of free-electron lasers (FELs) opens the possibility of ultra-short pulses even surpassing the present (tens to hundreds of attoseconds) capabilities of other light sources…

Accelerator Physics · Physics 2013-09-03 D. J. Dunning , B. W. J. McNeil , N. R. Thompson

We present a detailed numerical study of ultrashort pulse compression using a three-stage hybrid all-bulk multipass cell scheme. By operating in the enhanced frequency chirp regime, we achieve the compression of pulses from around 180 fs to…

Optics · Physics 2025-06-24 V. W. Segundo Staels , E. Conejero Jarque , J. San Roman

Attosecond transient absorption spectroscopy (ATAS) has emerged as a powerful technique within the field of attosecond science, combining extremely high temporal and excellent spectral resolution. So far, ATAS has been implemented in…

Laser-plasma accelerators (LPAs), producing high-quality electron beams, provide an opportunity to reduce the size of free-electron lasers (FELs) to only a few meters. A complete system is proposed here, which is based on FEL technology and…

Accelerator Physics · Physics 2018-07-04 Z. Tibai , Gy. Tóth , A. Nagyváradi , A. Sharma , M. I. Mechler , J. A. Fülöp , G. Almási , J. Hebling

Attosecond pulses produced by High-order Harmonic Generation (HHG) in gases driven by intense laser fields have become a cornerstone technique for probing ultrafast electronic motion in matter. These applications require a good knowledge of…