Subcycle phase matching effects in short attosecond pulse trains
Abstract
Attosecond pulses produced by High-order Harmonic Generation (HHG) in gases driven by intense laser fields have become a cornerstone technique for probing ultrafast electronic motion in matter. These applications require a good knowledge of the temporal and spectral properties of the emitted radiation. In this work, we generate a train of two to three attosecond pulses that we characterize using two-color laser-assisted photoionization. \textcolor{black}{An unexpected spectral behavior, with more pulses at high energies than at low energies, is observed when the carrier-to-envelope phase of the laser field is changed by 90.} HHG simulations indicate that the time-dependent phase matching of the harmonics contributes in a non-trivial way to the structure of the pulse train. Two-color laser-assisted photoionization enables us to unravel the dynamical influence of subcycle phase matching on the spectral properties of the attosecond pulse train, going beyond the predictions of the response of a single atom to a strong laser field.
Cite
@article{arxiv.2507.06386,
title = {Subcycle phase matching effects in short attosecond pulse trains},
author = {N. Ouahioune and R. Martín-Hernández and D. Hoff and P. K. Maroju and C. Guo and R. Weissenbilder and S. Mikaelsson and A. L'Huillier and M Lucchini and C. L. Arnold and M. Gisselbrecht},
journal= {arXiv preprint arXiv:2507.06386},
year = {2026}
}
Comments
16 pages, 10 figures