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The solid-state diffusion coefficient of the electrode active material is one of the key parameters in lithium-ion battery modelling. Conventionally, this diffusion coefficient is estimated through the galvanostatic intermittent titration…

Chemical Physics · Physics 2021-10-18 Zeyang Geng , Yu-Chuan Chien , Matthew J. Lacey , Torbjörn Thiringer , Daniel Brandell

Galvanostatic Intermittent Titration Technique (GITT) is widely used to evaluate solid-state diffusion coefficients in electrochemical systems. However, the existing analysis methods for GITT data require numerous assumptions, and the…

In this article, a pioneering study is presented where the intermittent current interruption method is used to characterize the aging behavior of commercial lithium ion batteries. With a very resource-efficient implementation, this method…

Chemical Physics · Physics 2021-11-09 Zeyang Geng , Torbjörn Thiringer , Matthew J. Lacey

We introduce a simple and efficient model to describe the potential energy surface of lithium diffusing in a solid-state ionic conductor. First, we assume that the Li atoms are fully ionized and we neglect the weak dependence of the…

Materials Science · Physics 2019-02-07 Leonid Kahle , Aris Marcolongo , Nicola Marzari

The penetrations of lithium-ion batteries in transport, energy and communication systems are increasing rapidly. A meticulous model applicable for precise in-situ monitoring and convenient online controlling is in sought to bridge the gap…

Systems and Control · Electrical Eng. & Systems 2022-03-22 Yuxuan Gu , Jianxiao Wang , Yuanbo Chen , Zhongwei Deng , Hongye Guo , Kedi Zheng , Qixin Chen

Accurately predicting the lifespan of lithium-ion batteries is crucial for optimizing operational strategies and mitigating risks. While numerous studies have aimed at predicting battery lifespan, few have examined the interpretability of…

Machine Learning · Computer Science 2024-04-12 Jaewook Lee , Seongmin Heo , Jay H. Lee

Lithium-ion batteries are used to store energy in electric vehicles. Physical models based on electro-chemistry accurately predict the cell dynamics, in particular the state of charge. However, these models are nonlinear partial…

Analysis of PDEs · Mathematics 2017-09-13 Sepideh Afshar , Kirsten Morris , Amir Khajepour

The use of solid-state electrolytes to provide safer, next-generation rechargeable batteries is becoming more feasible as new materials with greater stability and higher ionic diffusion coefficients are designed. However, accurate…

Materials Science · Physics 2021-01-08 Ardeshir Baktash , James C. Reid , Tanglaw Roman , Debra J. Searles

Lithium ion batteries have been a central part of consumer electronics for decades. More recently, they have also become critical components in the quickly arising technological fields of electric mobility and intermittent renewable energy…

Computational Physics · Physics 2021-11-15 Chiara Panosetti , Simon B. Anniés , Cristina Grosu , Stefan Seidlmayer , Christoph Scheurer

We introduce Interleaved Gibbs Diffusion (IGD), a novel generative modeling framework for discrete-continuous data, focusing on problems with important, implicit and unspecified constraints in the data. Most prior works on discrete and…

Machine Learning · Computer Science 2025-07-04 Gautham Govind Anil , Sachin Yadav , Dheeraj Nagaraj , Karthikeyan Shanmugam , Prateek Jain

Battery degradation remains a critical challenge in the pursuit of green technologies and sustainable energy solutions. Despite significant research efforts, predicting battery capacity loss accurately remains a formidable task due to its…

This paper presents the development of machine learning-enabled data-driven models for effective capacity predictions for lithium-ion batteries under different cyclic conditions. To achieve this, a model structure is first proposed with the…

Machine Learning · Computer Science 2021-01-05 Kailong Liu , Xiaosong Hu , Zhongbao Wei , Yi Li , Yan Jiang

Impedance-based temperature detection (ITD) is a promising approach for rapid estimation of internal cell temperature based on the correlation between temperature and electrochemical impedance. Previously, ITD was used as part of an…

Systems and Control · Computer Science 2016-06-28 Robert R. Richardson , Shi Zhao , David A. Howey

Distributions of potential and lithium content inside lithium ion batteries highly affects their performance and durability. An increased heterogeneity of the lithium distribution is expected in thick electrodes with high energy densities…

We introduce the Composable Involution Delay Model (CIDM) for fast and accurate digital simulation. It is based on the Involution Delay Model (IDM) [F\"ugger et al., IEEE TCAD 2020], which has been shown to be the only existing candidate…

Other Computer Science · Computer Science 2021-04-23 Jürgen Maier , Daniel Öhlinger , Ulrich Schmid , Matthias Függer , Thomas Nowak

Future lithium-based batteries are expected to use solid electrolytes to achieve higher energy density and fast charge capabilities. The majority of solid electrolytes are thermodynamically unstable against layered oxide cathodes. Here, the…

Molecular dynamics simulations are a powerful tool to study diffusion processes in battery electrolyte and electrode materials. From a single molecular dynamics simulation many properties relevant to diffusion can be obtained, including the…

Chemical Physics · Physics 2018-07-09 Niek J. J. de Klerk , Eveline van der Maas , Marnix Wagemaker

Lithium-ion battery (Li-ion) is becoming the dominant energy storage solution in many applications such as hybrid electric and electric vehicles, due to its higher energy density and longer life cycle. For these applications, the battery…

Systems and Control · Electrical Eng. & Systems 2024-12-20 Jeongeun Son , Yuncheng Du

Lithium-graphite intercalation compounds (Li-GICs) are the most common anode material for modern Li-ion batteries. However, the dielectric response of this material in the electrostatic limit (and its variation with the state of charge…

Materials Science · Physics 2022-10-27 Simon Anniés , Christoph Scheurer , Chiara Panosetti

Accurate on-board capacity estimation is of critical importance in lithium-ion battery applications. Battery charging/discharging often occurs under a constant current load, and hence voltage vs. time measurements under this condition may…

Applications · Statistics 2018-01-17 Robert R. Richardson , Christoph R. Birkl , Michael A. Osborne , David A. Howey
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