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We report on {\it ab-initio} simulations of the quantum dynamics of electronic charge and spin when subjected to intense laser pulses. By performing separate calculations for a Ni thin film and bulk Ni, we conclude that surface effects have…

Materials Science · Physics 2017-05-24 K. Krieger , P. Elliott , T. Müller , N. Singh , J. K. Dewhurst , E. K. U. Gross , S. Sharma

Since the beginning of femtomagnetism, it has been hotly debated how an ultrafast laser pulse can demagnetize a sample and switch its spins within a few hundred femtoseconds, but no consensus has been reached. In this paper, we propose that…

Materials Science · Physics 2015-06-22 G. P. Zhang , Mingqiang Gu , X. S. Wu

We present time-resolved scanning x-ray microscopy measurements with picosecond photo-excitation via a tailored infrared pump laser at a scanning transmission x-ray microscope. Specifically, we image the laser-induced demagnetization and…

Pulsed laser excitation causes the luminescence of Nitrogen Vacancy centers in diamond to unexpectedly decrease with increasing pulse energy. This decrease is observed in both the negatively charged and neutral centers and is caused by…

Mesoscale and Nanoscale Physics · Physics 2017-12-22 Robert Chapman , Taras Plakhotnik

Nonstationary pump-probe interaction between short laser pulses propagating in a resonant optically dense coherent medium is considered. A special attention is paid to the case, where the density of two-level particles is high enough that a…

Quantum Physics · Physics 2007-05-23 V. S. Egorov , V. N. Lebedev , I. B. Mekhov , P. V. Moroshkin , I. A. Chekhonin , S. N. Bagayev

We demonstrate the coherent optical control of magnetization precession in a thin Ni film by a second excitation pulse which amplifies or attenuates the precession induced by a first pulse depending on the fluences of the pump-pulses and…

Materials Science · Physics 2023-11-09 M. Mattern , F. -C. Weber , D. Engel , C. Korff-Schmising , M. Bargheer

The mechanism underlying femtosecond laser pulse induced ultrafast magnetization dynamics remains elusive despite two decades of intense research on this phenomenon. Most experiments focused so far on characterizing magnetization and charge…

Photo-excited precession of magnetization in (Ga,Mn)As is investigated by measuring time-resolved magneto-optical response and transient differential reflectivity with pump-and-probe technique. In the time region less than 1 ps, rapidly…

Materials Science · Physics 2014-09-09 T. Matsuda , K. Nishibayashi , H. Munekata

Ultrafast irradiation of correlated electronic systems triggers complex dynamics involving quasi-particle excitations, doublons, charge carriers, and spin fluctuations. To describe these effects, we develop an efficient non-equilibrium…

Strongly Correlated Electrons · Physics 2026-01-22 Nagamalleswararao Dasari , Hugo U. R. Strand , Martin Eckstein , Alexander I. Lichtenstein , Evgeny A. Stepanov

We study the impact of dephasing on the excitation dynamics of a cloud of ultracold two-level Rydberg atoms for both resonant and off-resonant laser excitation, using the wave function Monte Carlo (MCWF) technique. We find that while for…

Atomic Physics · Physics 2015-06-18 David W. Schönleber , Martin Gärttner , Jörg Evers

Laser-induced femtosecond demagnetization has attracted a broad attention as a possible candidate for information storage technology. However, whether or not lattice vibration directly participates in demagnetization has been highly…

Materials Science · Physics 2022-09-14 G. P. Zhang , Y. H. Bai

The ultrafast dynamics of ions in solids following intense femtosecond laser excitation is governed by two fundamentally distinct yet interplaying effects. On one hand, the significant generation of hot electron-hole pairs by the light…

Computational Physics · Physics 2024-01-22 Bernd Bauerhenne , Martin E. Garcia

The numerical simulations of an ultrashort pulse propagation in a one-dimensional nonlinear photonic crystal are carried out. It is known that the relaxation of cubic nonlinearity is the reason for the effect of pulse self-trapping in such…

Optics · Physics 2013-03-05 Denis Novitsky

A brief review is given of topics relating to dynamical processes arising in nonlinear interactions between light and resonant systems (atoms or molecules) in the presence of a magnetic field.

Atomic Physics · Physics 2009-11-10 E. B. Alexandrov , M. Auzinsh , D. Budker , D. F. Kimball , S. M. Rochester , V. V. Yashchuk

Strongly magnetizing a plasma adds a range of waves that do not exist in unmagnetized plasmas and enlarges the laser-plasma interaction (LPI) landscape. In this paper, we use particle-in-cell (PIC) simulations to investigate strongly…

Plasma Physics · Physics 2022-11-23 Lili Manzo , Matthew R. Edwards , Yuan Shi

We study the photoluminescence dynamics of ultra-cold indirect excitons optically created in a double quantum well heterostructure. Above a threshold laser excitation, our experiments reveal the apparition of the so-called inner…

Mesoscale and Nanoscale Physics · Physics 2012-02-10 M. Alloing , A. Lemaitre , E. Galopin , F. Dubin

Sub-picosecond magnetisation manipulation via femtosecond optical pumping has attracted wide attention ever since its original discovery in 1996. However, the spatial evolution of the magnetisation is not yet well understood, in part due to…

We calculated third order non-linear polarization to estimate the two-photon absorption of non-interacting two-level molecules in the transmission-type degenerate pump-probe geometry. The spectral intensity and the phase changes of the…

Optics · Physics 2019-05-01 Tsogvoo Khos-Ochir , Kim Myung-Whun , Purevdorj Munkhbaatar

We report dynamic control of magnetization precession by light alone. A ferromagnetic (Ga,Mn)As epilayer was used for experiments. Amplitude of precession was modulated to a large extent by tuning the time interval between two successive…

Materials Science · Physics 2009-11-13 Y. Hashimoto , H. Munekata

Understanding and controlling the electronic as well as ro-vibrational motion and, thus, the entire chemical dynamics in molecules is the ultimate goal of ultrafast laser and imaging science. In photochemistry, laser-induced dissociation…