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A quantitative understanding of the processes that trigger light-induced demagnetization on ultrashort timescales is crucial for achieving an ultrafast, radiation-controlled magnetic response in materials. This milestone is essential for…

Electromagnetism and light-matter interaction in rotating systems is a rich area of ongoing research. We study the interaction of light with a gas of non-interacting two-level atoms confined to a rotating disk. We numerically solve the…

Optics · Physics 2019-06-11 Calum Maitland , Matteo Clerici , Fabio Biancalana

Since the first experimental observation of all-optical switching phenomena, intensive research has been focused on finding suitable magnetic systems that can be integrated as storage elements within spintronic devices and whose…

We identify that both the dynamic core polarization and dynamic orbital deformation are important in the orientation-dependent high-harmonic generation of CO molecules subjected to intense few cycle laser fields. These polarization dynamics…

Atomic Physics · Physics 2015-06-19 Bin Zhang , Jianmin Yuan , Zengxiu Zhao

Laser-induced ultrafast demagnetization is a phenomenon of utmost interest and attracts significant attention because it enables potential applications in ultrafast optoelectronics and spintronics. As a spin-orbit coupling assisted magnetic…

Irradiation with an ultrashort laser pulse can completely destroy the magnetic order of ferromagnetic thin films on the femtosecond timescale. This phenomenon holds great potential for ultrafast spintronics and information processing and is…

Optics · Physics 2022-06-16 Eva Prinz , Benjamin Stadtmüller , Martin Aeschlimann

We describe a mechanism by which both ferroelectric polarization and magnetization can be created in nonpolar, nonmagnetic materials. Using a combination of phenomenological modeling and first-principles calculations, we demonstrate that…

Materials Science · Physics 2024-04-26 Carolina Paiva , Michael Fechner , Dominik M. Juraschek

Stoner and Heisenberg excitations in magnetic materials are inherently different. The former involves an effective reduction of the exchange splitting, whereas the latter comprises excitation of spin-waves. In this work, we test the impact…

Materials Science · Physics 2022-03-14 Mohamed F. Elhanoty , Olle Eriksson , Ronny Knut , Olof Karis , Oscar Grånäs

The parallel or antiparallel arrangement of electron spins plays a pivotal role in determining the properties of a physical system. To meet the demands for innovative technological solutions, extensive efforts have been dedicated to…

The manipulation of the magnetic direction by using the ultrafast laser pulse is attractive for its great advantages in terms of speed and energy efficiency for information storage applications. However, the heating and helicity effects…

Materials Science · Physics 2020-09-29 Guanqi Li , Xiangyu Zheng , Junlin Wang , Xianyang Lu , Jing Wu , Jianwang Cai , Thomas Ostler , Yongbing Xu

The practical difficulty in distinguishing the impact of magnetic circular dichroism and the inverse Faraday effect fuels intense debates over which mechanism predominantly drives the process of helicity dependent all-optical switching of…

Ultrafast non-thermal manipulation of magnetization by light relies on either indirect coupling of the electric field component of the light with spins via spin-orbit interaction or direct coupling between the magnetic field component and…

Low-index transparent conducting oxides have attracted significant attention because ultrafast optical excitation in these materials can induce exceptionally large temporal index gradients. Due to this remarkable nonlinear optical…

Strong laser-induced magnetization of oxygen gas at room temperature and atmospheric pressure is achieved experimentally on the sub-nanosecond time scale. The method is based on controlling the electronic spin of paramagnetic molecules by…

Quantum Physics · Physics 2017-06-21 A. A. Milner , A. Korobenko , V. Milner

Simultaneous detection of THz emission and transient magneto-optical response is employed to study ultrafast laser-induced magnetization dynamics in multisublattice magnets NdFeCo and GdFeCo amorphous alloys with in-plane magnetic…

Materials Science · Physics 2015-09-18 T. J. Huisman , R. V. Mikhaylovskiy , A. Tsukamoto , Th. Rasing , A. V. Kimel

Using a three-dimensional quasiclassical technique we explore molecular double ionization by a linearly polarized, infrared (800 nm) and ultrashort (6 fs) laser pulse. We first focus on intensities corresponding to the tunneling regime and…

Atomic Physics · Physics 2015-05-14 A. Emmanouilidou , A. Staudte

The ultrafast non-thermal control of magnetization has recently become feasible in canted antiferromagnets through photomagnetic instantaneous pulses [A.V. Kimel {\it et al.}, Nature {\bf 435}, 655 (2005)]. In this experiment circularly…

Other Condensed Matter · Physics 2009-11-11 C. A. Perroni , A. Liebsch

We present a theoretical formulation of the coherent ultrafast nonlinear optical response of a strongly correlated system and discuss an example where the Coulomb correlations dominate. We separate out the correlated contributions to the…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 A. T. Karathanos , I. E. Perakis , N. A. Fromer , D. S. Chemla

Time-dependent density functional theory is implemented in an all electron solid-state code for the case of fully non-collinear spins. We use this to study laser induced demagnetization in Fe, Co and Ni. It is shown that this…

Materials Science · Physics 2014-06-26 K. Krieger , J. K. Dewhurst , P. Elliott , S. Sharma , E. K. U. Gross

Nonlinear optical signals in optically driven quantum systems can reveal coherences and thereby open up the possibility for manipulation of quantum states. While the limiting cases of ultrafast and continuous-wave excitation have been…