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Second-order nonlinearity in solids gives rise to a plethora of unique physical phenomena ranging from piezoelectricity and optical rectification to optical parametric amplification, spontaneous parametric down-conversion, and the…

High-harmonic generation (HHG) in solids has rapidly emerged as a promising platform for creating compact attosecond sources and probing ultrafast electron dynamics. Resonant metasurfaces are essential for enhancement of the otherwise small…

Optical second-harmonic generation (SHG) is a nonlinear parametric process that doubles the frequency of incoming light. Only allowed in non-centrosymmetric materials, it has been widely used in frequency modulation of lasers, surface…

Materials Science · Physics 2021-01-05 Wontaek Kim , Je Yhoung Ahn , Juseung Oh , Ji Hoon Shim , Sunmin Ryu

High-harmonic generation (HHG) in solids has typically been explored in transparent dielectrics and semiconductors. Metals have long been dismissed due to their strong reflectivity at infrared wavelengths. Here, we demonstrate HHG from…

We generate high-order harmonics of a mid-infrared laser from a silicon single crystal and find their origin in the recollision of coherently accelerated electrons with their holes, analogously to the atomic and molecular case, and to ZnO…

We present a theoretical study of high-order harmonic generation (HHG) driven by ultrashort optical pulses with different kind of chirps. The goal of the present work is perform a detailed study to clarify the relevant parameters in the…

Atomic Physics · Physics 2016-12-21 E Neyra , F Videla , J A Pérez-Hernández , M F Ciappina , L Roso , G A Torchia

We employ the two-band density-matrix equations and time-dependent density functional theory to calculate high-order harmonic generation (HOHG) in graphene under a femtosecond laser irradiation. Our investigation uncovers a striking…

Atomic Physics · Physics 2023-07-25 Fulong Dong , Qinzhi Xia , Jie Liu

Here, we study the possibility of selective high-harmonic generation (HHG) based on the concept of charge transfer plasmons (CTP) in bridged nanoparticle assemblies. By choosing plasmonic dimer nanoantenna, as a fundamental member of…

Optics · Physics 2018-01-16 Burak Gerislioglu , Arash Ahmadivand , Nezih Pala

The recent observation of high-harmonic generation from solids creates a new possibility for engineering fundamental strong-field processes by patterning the solid target with subwavelength nanostructures. All-dielectric metasurfaces…

The generation of high-order harmonics in bulk solids subjected to intense ultrashort laser pulses has opened up new avenues for research in extreme nonlinear optics and light-matter interaction on sub-cycle timescales. Despite significant…

We study high order harmonics generation (HHG) in crystalline silicon and diamond subjected to near and mid-infrared laser pulses. We employ time-dependent density functional theory and solve the time-dependent Kohn-Sham equation in the…

Materials Science · Physics 2022-08-31 David Freeman , Shunsuke Yamada , Atsushi Yamada , Kazuhiro Yabana , Anatoli Kheifets

We report on experimental investigation of nonperturbative high harmonic generation (HHG) in monolayer MoS2 in the ultraviolet spectral region driven by mid-infrared light. We study how the HHG is influenced by pre-excitation of the…

Solids in an intense laser field show high-harmonic generation (HHG), which can provide information on carrier dynamics and band structures in weakly correlated systems. In strongly correlated systems, a laser field can induce a transition…

Strongly Correlated Electrons · Physics 2025-08-04 Ryohei Ikeda , Yuta Murakami , Daiki Sakai , Tatsuya Miyamoto , Toshimitsu Ito , Hiroshi Okamoto

High-order harmonic generation (HHG) with relativistically strong laser pulses is considered employing electron ionization-recollisions from multiply charged ions in counterpropagating, linearly polarized attosecond pulse trains. The…

Atomic Physics · Physics 2015-05-19 Markus C. Kohler , Michael Klaiber , Karen Z. Hatsagortsyan , Christoph H. Keitel

We present Floquet calculations of high harmonic generation (HHG) for the lowest two electronic states of the $\mbox{H}_2^+$ ion by strong continuous-wave laser fields. We solve the non-Hermitian matrix problem to get accurate solutions to…

Atomic Physics · Physics 2015-06-18 Ts Tsogbayar , M Horbatsch

High-order harmonic generation (HHG) is investigated for H$_2^+$ and its isotopomers under seven- and ten-cycle trapezoidal laser pulses at 800 nm wavelength and $I$=4$\times 10^{14}$ W$/$cm$^2$ intensity. We solved numerically…

Atomic Physics · Physics 2016-03-03 H. Ahmadi , M. Vafaee , A. Maghari

Layered NbOX$_2$ ($X=\mathrm{Cl,\,Br,\,I}$), a member of the van der Waals ferroelectric family, exhibits intrinsic ferroelectricity and pronounced nonlinear optical responses, making it a promising candidate for integrated nanophotonics…

We investigate high-order harmonic generation (HHG) in graphene with a quantum master equation approach. The simulations reproduce the observed enhancement in HHG in graphene under elliptically polarized light [N. Yoshikawa et al, Science…

Materials Science · Physics 2021-02-03 Shunsuke A. Sato , Hideki Hirori , Yasuyuki Sanari , Yoshihiko Kanemitsu , Angel Rubio

In this work the extreme nonlinear optical response of a giant fullerene molecule C$_{240}$ in strong laser field is studied. The investigation of high-order harmonic generation in such quantum nanostructure is presented modeling the…

Optics · Physics 2023-09-15 H. K. Avetissian , S. Sukiasyan , T. M. Markosyan , G. F. Mkrtchian

Second-harmonic emission at a frequency that is twice the laser frequency is an important diagnostic for nonlinear laser-plasma interaction. It is forbidden for centrosymmetric materials such as the bulk of sapphire. The symmetry, however,…