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We have investigated the excitation spectra of $j_{eff}$=$\frac{1}{2}$ Mott insulator Na$_2$IrO$_3$. Taking into account a relativistic multiplet structure of Ir ions, we have calculated the optical conductivity $\sigma(\omega)$ and…

Strongly Correlated Electrons · Physics 2014-02-25 Beom Hyun Kim , G. Khaliullin , B. I. Min

We carried out temperature-dependent (20 - 550 K) measurements of resonant inelastic X-ray scattering on LaCoO$_3$ to investigate the evolution of its electronic structure across the spin-state crossover. In combination with charge-transfer…

The spin-orbit Mott insulator Sr3Ir2O7 provides a fascinating playground to explore insulator-metal transition driven by intertwined charge, spin, and lattice degrees of freedom. Here, we report high pressure electric resistance and…

We have investigated the electronic structure of CaCu3Ru4O12 and LaCu3Ru4O12 using soft x-ray photoelectron and absorption spectroscopy together with band structure and cluster configuration interaction calculations. We found the Cu to be…

Strongly Correlated Electrons · Physics 2015-06-12 N. Hollmann , Z. Hu , A. Maignan , A. Günther , L. -Y. Jang , A. Tanaka , H. -J. Lin , C. T. Chen , P. Thalmeier , L. H. Tjeng

We study theoretically resonant inelastic x-ray scattering (RIXS) at the Cu $L_3$-edge in a typical parent compound of high-$T_c$ cuprate superconductors La$_2$CuO$_4$ on the basis of a detailed electronic band structure. We construct a…

Strongly Correlated Electrons · Physics 2015-08-20 Takuji Nomura

V2O3 is an archetypal system for the study of correlation induced, Mott-Hubbard metal-insulator transitions. Despite decades of extensive investigations, the accurate description of its electronic properties remains an open problem in the…

We investigate the role of electron correlation in the electronic structure of honeycomb lattice Li$_2$RuO$_3$ using photoemission spectroscopy and band structure calculations. Monoclinic Li$_2$RuO$_3$ having Ru network as honeycomb lattice…

Strongly Correlated Electrons · Physics 2023-01-24 Sakshi Bansal , Asif Ali , B. H. Reddy , Ravi Shankar Singh

Motivated by the unveiled complexity of nonmagnetic insulating behavior in pentavalent post-perovskite NaIrO$_3$, we have studied its electronic structure and phase diagram in the plane of Coulomb repulsive interaction and spin-orbit…

Strongly Correlated Electrons · Physics 2014-01-13 Liang Du , Xianlei Sheng , Hongming Weng , Xi Dai

We present a temperature-dependent resonant elastic soft x-ray scattering (REXS) study of the metal-insulator transition in Sr3(Ru1-xMnx)2O7, performed at both Ru and Mn L-edges. Resonant magnetic superstructure reflections, which indicate…

The electronic structure of CuIr$_2$S$_4$ has been investigated using various bulk-sensitive x-ray spectroscopic methods near the Ir $L_3$-edge: resonant inelastic x-ray scattering (RIXS), x-ray absorption spectroscopy in the partial…

Strongly Correlated Electrons · Physics 2012-06-18 H. Gretarsson , Jungho Kim , D. Casa , T. Gog , K. R. Choi , S. W. Cheong , Young-June Kim

Ca$_{3}$Ru$_{2}$O$_{7}$ is a fascinating material that displays physical properties governed by spin-orbit interactions and structural distortions, showing a wide range of remarkable electronic phenomena. Here, we present a…

Materials Science · Physics 2023-10-23 A. M León , J. W. González , H. Rosner

Turning a pristine Mott insulator into a correlated metal by chemical doping is a common procedure in strongly correlated materials physics, e.g. underlying the phenomenology of high-$T_c$ cuprates. The ruthenate bilayer compound…

Strongly Correlated Electrons · Physics 2020-09-29 Frank Lechermann , Qiang Han , Andrew J. Millis

The electronic structures of the metallic and insulating phases of the alloy series Ca(2-x)Sr(x)RuO4 (0 <= x <= 2) are calculated using LDA, LDA+U and Dynamical Mean-Field Approximation methods. In the end members the groundstate…

Strongly Correlated Electrons · Physics 2009-09-25 V. I. Anisimov , I. A. Nekrasov , D. E. Kondakov , T. M. Rice , M. Sigrist

We investigate the evolution of the electronic structure in SrRu_(1-x)Ti_xO_3 as a function of x using high resolution photoemission spectroscopy, where SrRuO3 is a weakly correlated metal and SrTiO3 is a band insulator. The surface spectra…

Strongly Correlated Electrons · Physics 2009-11-13 Kalobaran Maiti , Ravi Shankar Singh , V. R. R. Medicherla

We report resonant inelastic x-ray measurements of insulating La$_2$CuO$_4$ and Sr$_2$CuO$_2$Cl$_2$ taken with the incident energy tuned near the Cu K absorption edge. We show that the spectra are well described in a shakeup picture in 3rd…

Strongly Correlated Electrons · Physics 2009-10-31 P. Abbamonte , C. A. Burns , E. D. Isaacs , P. M. Platzman , L. L. Miller , S. W. Cheong , M. V. Klein

The iso-electronic $d^{4}$ compounds of the $4d$ series show rich phase diagrams due to competing spin, charge and orbital degrees of freedom in presence of strong correlations and structural distortions. One such iso-electronic series,…

Strongly Correlated Electrons · Physics 2018-07-10 Swagata Acharya , Dibyendu Dey , T Maitra , A Taraphder

We present Ru $L_3$-edge resonant inelastic x-ray scattering (RIXS) measurements of spin-orbit and d-d excitations in exfoliated nanolayers of the Kitaev spin-liquid candidate RuCl$_3$. Whereas the spin-orbit excitations are independent of…

On the basis of density functional theory electronic band structure calculations using the augmented spherical wave method, the electronic and magnetic properties of the orthorhombic and tetragonal phases of Ca3Mn2O7 were investigated and…

Materials Science · Physics 2007-08-02 S. F. Matar , V. Eyert , A. Villesuzanne , M. -H. Whangbo

We used x-ray photoemission spectroscopy to investigate the electronic structure of the Mott insulator LaVO3 embedded in LaAlO3. By limiting the upper layer of LaAlO3 to 3 unit cells, the underlying LaVO3 could be probed. The V 2p…

Materials Science · Physics 2015-06-25 Y. Hotta , H. Wadati , A. Fujimori , T. Susaki , H. Y. Hwang

We report the structural, elastic and vibrational properties of five ionic-molecular solid oxidizers MNO$_3$ (M = Li, Na, K) and MClO$_3$ (M = Na, K). By treating long range electron-correlation effects, dispersion corrected method leads to…

Materials Science · Physics 2016-09-05 N. Yedukondalu , G. Vaitheeswaran