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Traditional thermoelectric materials rely on low thermal conductivity to enhance their efficiency but suffer from inherently limited power factors. Novel pathways to optimize electronic transport are thus crucial. Here, we achieve ultrahigh…

Searching for high-performance thermoelectric (TE) materials in the paradigm of narrow-bandgap semiconductors has lasted for nearly 70 years and is obviously hampered by a bottleneck of research now. Here we report on the discovery of a few…

Strongly Correlated Electrons · Physics 2022-10-11 Zirui Dong , Yubo Zhang , Jun Luo , Ying Jiang , Zhiyang Yu , Nan Zhao , Liusuo Wu , Yurong Ruan , Fang Zhang , Kai Guo , Jiye Zhang , Wenqing Zhang

Metallic thermoelectric materials are promising candidates for active cooling applications, where high thermal conductivity and a high thermoelectric power factor are essential to maximize effective thermal conductivity. While metals…

Engineering new quantum phases requires fine tuning of the electronic, orbital, spin, and lattice degrees of freedom. To this end, the kagome lattice with flat bands has garnered great attention by hosting various topological and correlated…

We present the Stagome lattice, a variant of the Kagome lattice, where one can make any of the bands completely flat by tuning an externally controllable magnetic flux. This systematically allows the energy of the flat band to coincide with…

Strongly Correlated Electrons · Physics 2025-03-03 Biplab Pal , Georges Bouzerar

High Seebeck coefficient by creating large density of state (DOS) around the Fermi level through either electronic structure modification or manipulating nanostructures, is commonly considered as a route to advanced thermoelectrics.…

Materials Science · Physics 2011-11-24 Yanzhong Pei , Aaron D. LaLonde , Heng Wang , G. Jeffrey Snyder

The study of topological quantum materials for enhanced thermoelectric energy conversion has received significant attention recently. Topological materials (including topological insulators and Dirac/Weyl/nodal-line semi-metals) with unique…

We propose a simple theoretical model referred to as the {\it two-band model} to realize both a large Seebeck coefficient and high electrical conductivity, resulting in a high thermoelectric (TE) power factor ($PF$). Using the…

Materials Science · Physics 2023-09-18 Manaho Matsubara , Takahiro Yamamoto , Hidetoshi Fukuyama

Topological materials attract a considerable research interest because of their characteristic band structure giving rise to various new phenomena in quantum physics. Beside this, they are tempting from a functional materials point of view:…

Materials Science · Physics 2024-12-04 Markus Kriener , Takashi Koretsune , Ryotaro Arita , Yoshinori Tokura , Yasujiro Taguchi

We have theoretically investigated thermoelectric (TE) effects of narrow-gap single-walled carbon nanotubes (SWCNTs) with randomly substituted nitrogen (N) impurities, i.e., N-substituted (20,0) SWCNTs with a band gap of 0.497 eV. For such…

Mesoscale and Nanoscale Physics · Physics 2021-03-16 Manaho Matsubara , Kenji Sasaoka , Takahiro Yamamoto , Hidetoshi Fukuyama

Heavily doped semiconductors are by far the most studied class of materials for thermoelectric applications in the past several decades. They have Seebeck coefficient values which are 2-3 orders of magnitude higher than metals, making them…

Materials Science · Physics 2019-09-11 Maxime Markov , Emad Rezaei , Safoura Nayeb Sadeghi , Keivan Esfarjani , Mona Zebarjadi

Thermoelectric (TE) materials seamlessly convert thermal into electrical energy and vice versa, making them promising for applications such as power generation or cooling. Although historically the TE effect was first discovered in metals,…

A particularly promising pathway to enhance the efficiency of thermoelectric materials lies in the use of resonant states, as suggested by experimentalists and theorists alike. In this paper, we go over the mechanisms used in the literature…

Materials Science · Physics 2017-09-13 Simon Thébaud , Christophe Adessi , Stéphane Pailhès , Georges Bouzerar

Recent research on twisted bilayer graphene (TBG) uncovered that its twist-angle-dependent electronic structure leads to a host of unique properties, such as superconductivity, correlated insulating states, and magnetism. The flat bands…

Mesoscale and Nanoscale Physics · Physics 2021-03-29 Adithya Kommini , Zlatan Aksamija

Metals have high electronic conductivities, but very low Seebeck coefficients, which traditionally make them unsuitable for thermoelectric materials. Recent studies, however, showed that metals can deliver ultra-high thermoelectric power…

We report a transport, thermodynamic, and spectroscopic study of the recently identified topological semiconductor ZrTe$_5$ with a focus on elucidating the connections between its band structure and unusual thermoelectric properties. Using…

Materials Science · Physics 2023-03-22 Junbo Zhu , Changmin Lee , Fahad Mahmood , Takehito Suzuki , Shiang Fang , Nuh Gedik , Joseph G. Checkelsky

Nano-structuring is an extremely promising path to high performance thermoelectrics. Favorable improvements in thermal conductivity are attainable in many material systems, and theoretical work points to large improvements in electronic…

Flat bands, emergent in strongly correlated electron systems, stand at the frontier of condensed matter physics, providing fertile ground for unconventional quantum phases. Recent observations of dispersionless bands at the Fermi level in…

We theoretically unveil the unconventional possibility to achieve extremely high thermoelectric power factors in lightly doped narrow gap semiconductors with asymmetric conduction/valence bands operated in the bipolar transport regime.…

Materials Science · Physics 2020-08-05 Patrizio Graziosi , Neophytos Neophytou

Flat bands with small energy dispersion can give rise to strongly correlated electronic and topological phases, especially when located at the Fermi level. Whilst flat bands have been experimentally realized in two-dimensional (2D) twisted…

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