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We successfully synthesized ($p$-Py-V)[Cu(hfac)$_2$], a verdazyl-based complex. Molecular orbital calculations revealed five types of intermolecular interactions between the radical spins and two types of intramolecular interactions between…

We present a model compound with a spin-1/2 frustrated square lattice, in which three ferromagnetic (F) interactions and one antiferromagnetic (AF) compet. Considering the effective spin-1 formed by the dominant F dimer, this square lattice…

Strongly Correlated Electrons · Physics 2021-08-31 H. Yamaguchi , N. Uemoto , T. Okubo , Y. Kono , S. Kittaka , T. Sakakibara , T. Yajima , S. Shimono , Y. Iwasaki , Y. Hosokoshi

We consider a quantum many-body system made of $N$ interacting $S{=}1/2$ spins on a lattice, and develop a formalism which allows to extract, out of conventional magnetic observables, the quantum probabilities for any selected spin pair to…

Statistical Mechanics · Physics 2007-05-23 Andrea Fubini , Tommaso Roscilde , Valerio Tognetti , Matteo Tusa , Paola Verrucchi

We apply a random-plaquette $J_1$-$J_2$ model on the square lattice to capture the physics of a series of spin-$1/2$ Heisenberg antiferromagnet compounds Sr$_2$CuTe$_{1-x}$W$_x$O$_6$. With the input of experimentally relevant coupling…

Strongly Correlated Electrons · Physics 2024-07-09 Dian Wu , Fan Yang , Giuseppe Carleo

We discuss the ground state and the low-lying excitations of the spin-half Heisenberg antiferromagnet on the two-dimensional square-kagome lattice. This magnetic system belongs to the class of highly frustrated spin systems with an infinite…

Strongly Correlated Electrons · Physics 2007-05-23 J. Richter , J. Schulenburg , P. Tomczak , D. Schmalfuß

We consider quantum Hall states at even-denominator filling fractions, especially $\nu=5/2$, in the limit of small Zeeman energy. Assuming that a paired quantum Hall state forms, we study spin ordering and its interplay with pairing. We…

Mesoscale and Nanoscale Physics · Physics 2010-09-16 Ivailo Dimov , Bertrand I. Halperin , Chetan Nayak

Fractional magnetisation plateaus, in which the magnetisation is pinned at a fraction of its saturated value within a range of external magnetic field, are spectacular macroscopic manifestations of the collective quantum behaviours. One…

By means of the recently developed algorithm based on the tensor product states, the magnetization process of frustrated spin-1/2 spin-dimer models on a square lattice is investigated. Various field-induced quantum phases are discovered. In…

Strongly Correlated Electrons · Physics 2010-01-26 Pochung Chen , Chen-Yen Lai , Min-Fong Yang

Quantum spin rings represent fundamental model systems that exhibit distinctive quantum phenomena-such as quantum critical behavior and quasiparticle excitations-arising from their periodic boundary conditions and enhanced quantum…

We present a new model compound with the S = 1/2 frustrated square lattice composed of the charge-transfer salt (o-MePy-V)PF6. Ab initio calculations indicate the formation of an S = 1/2 square lattice, in which six types of…

Strongly Correlated Electrons · Physics 2018-09-26 H. Yamaguchi , Y. Sasaki , T. Okubo , M. Yoshida , T. Kida , M. Hagiwara , Y. Kono , S. Kittaka , T. Sakakibara , M. Takigawa , Y. Iwasaki , Y. Hosokoshi

We study the magnetization process in two-dimensional S=1/2 spin systems, to discuss the appearance of a plateau structure. The following three cases are considered: (1) the Heisenberg antiferromagnet and multiple-spin exchange model on the…

Strongly Correlated Electrons · Physics 2009-10-31 Tsutomu Momoi , Keisuke Totsuka

We study the quantum spin pumping of an antiferromagnetic spin-1/2 chain with competing exchange interactions. We show that spatially periodic potential modulated in space and time acts as a quantum spin pump. In our model system, an…

Strongly Correlated Electrons · Physics 2009-11-13 Sujit Sarkar , C. D. Hu

We explore the ground states and quantum phase transitions of two-dimensional, spin S=1/2, antiferromagnets by generalizing lattice models and duality transforms introduced by Sachdev and Jalabert (Mod. Phys. Lett. B 4, 1043 (1990),…

Strongly Correlated Electrons · Physics 2007-05-23 Subir Sachdev , Kwon Park

The spin-1/2 antiferromagnetic Heisenberg model on a Kagome lattice is geometrically frustrated, which is expected to promote the formation of many-body quantum entangled states. The most sought-after among these is the quantum spin liquid…

The J1-J2 square lattice Heisenberg model with spin S=1/2 has three phases with long-range magnetic order and two unconventionally ordered phases depending on the ratio of exchange constants. It describes a number of recently found layered…

Strongly Correlated Electrons · Physics 2009-11-13 P. Thalmeier , M. E. Zhitomirsky , B. Schmidt , N. Shannon

We study the spin wave in the S=1/2 multiple-spin exchange model on a triangular lattice in a magnetic field within the linear spin-wave theory. We take only two-, three- and four-spin exchange interactions into account and restrict…

Strongly Correlated Electrons · Physics 2009-11-11 Chitoshi Yasuda , Daisuke Kinouchi , Kenn Kubo

A three-dimensional system of interacting spins typically develops static long-range order when it is cooled. If the spins are quantum (S = 1/2), however, novel quantum paramagnetic states may appear. The most highly sought state among them…

Strongly Correlated Electrons · Physics 2015-05-13 S. -H. Lee , H. Kikuchi , Y. Qiu , B. Lake , Q. Huang , K. Habicht , K. Kiefer

Spin-orbital entanglement in the ground state of a one-dimensional SU(2)$\otimes$SU(2) spin-orbital model is analyzed using exact diagonalization of finite chains. For $S=1/2$ spins and $T=1/2$ pseudospins one finds that the quantum…

Strongly Correlated Electrons · Physics 2007-06-19 Andrzej M. Oles , Peter Horsch , Giniyat Khaliullin

We apply density functional theory band structure calculations, the coupled-cluster method, and exact diagonalization to investigate the microscopic magnetic model of the spin-1/2 compound Cu2GeO4. The model is quasi-two-dimensional, with…

Strongly Correlated Electrons · Physics 2011-03-24 Alexander A. Tsirlin , Ronald Zinke , Johannes Richter , Helge Rosner

Coherent states offer a promising path for near-term quantum computing due to their inherent protection against bit-flip noise. However, their large photon numbers can be challenging for numerical simulation. This paper introduces an…