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In the field of femtomagnetism magnetic matter is controlled by ultrafast laser pulses; here we show that coupling phonon excitations of the nuclei to spin and charge leads to femto-phono-magnetism, a powerful route to control magnetic…

Materials Science · Physics 2022-03-29 S. Sharma , S. Shallcross , P. Elliott , J. K. Dewhurst

We demonstrate optical control of magnons using femtosecond laser pulses by performing ab-initio real-time time-dependent density functional theory (TDDFT) simulations. We predict that the spin-wave dynamics in Fe$_{50}$Ni$_{50}$ can be…

Materials Science · Physics 2021-04-07 N. Singh , P. Elliott , J. K. Dewhurst , S. Sharma

The ultrafast switching of magnetization in multiferroic materials by a femtosecond laser could provide various advantages in photonics and magnonics. An efficient approach to control the light matter interaction is the modulation of…

One route to the control of quantum magnetism at ultrafast timescales is magnetophononics, the modulation of magnetic interactions by coherently driven lattice excitations. Theoretical studies of a gapped quantum magnet subject to…

Strongly Correlated Electrons · Physics 2026-02-04 B. Demazure , M. Krebs , G. S. Uhrig , B. Normand

Magnetophononics, the modulation of magnetic interactions by driving infrared-active lattice excitations, is emerging as a key mechanism for the ultrafast dynamical control of both semiclassical and quantum spin systems by coherent light.…

Strongly Correlated Electrons · Physics 2023-05-15 M. Yarmohammadi , M. Krebs , G. S. Uhrig , B. Normand

Magnetic order parameters in altermagnets can couple to quantized lattice vibration via both piezomagnetic and magnetoelastic effects, leading to the renormalization of phonon dispersion. Here, we demonstrate photo-induced dynamic frequency…

Time-dependent density functional theory is implemented in an all electron solid-state code for the case of fully non-collinear spins. We use this to study laser induced demagnetization in Fe, Co and Ni. It is shown that this…

Materials Science · Physics 2014-06-26 K. Krieger , J. K. Dewhurst , P. Elliott , S. Sharma , E. K. U. Gross

Understanding spin dynamics on femto- and picosecond timescales offers new opportunities for faster and more efficient spintronic devices. Here, we experimentally investigate the coherent spin dynamics after ultrashort laser excitation by…

Mesoscale and Nanoscale Physics · Physics 2024-01-26 Anulekha De , Akira Lentfert , Laura Scheuer , Benjamin Stadtmüller , Georg von Freymann , Martin Aeschlimann , Philipp Pirro

Laser induced ultrafast demagnetization is the process whereby the magnetic moment of a ferromagnetic material is seen to drop significantly on a timescale of $10-100$s of femtoseconds due to the application of a strong laser pulse. If this…

Materials Science · Physics 2016-01-20 P. Elliott , K. Krieger , J. K. Dewhurst , S. Sharma , E. K. U. Gross

Understanding spin-lattice interactions in antiferromagnets is one of the most fundamental issues at the core of the recently emerging and booming fields of antiferromagnetic spintronics and magnonics. Recently, coherent nonlinear…

A coherent THz optical lattice mode is triggered by femtosecond laser pulses in the antiferromagnetic van der Waals semiconductor FePS$_3$. The 380 nm thick exfoliated flake was placed on a substrate and laser-driven lattice and spin…

To gain control over magnetic order on ultrafast time scales, a fundamental understanding of the way electron spins interact with the surrounding crystal lattice is required. However, measurement and analysis even of basic collective…

A major question in the field of femtosecond laser-induced demagnetization is whereto the angular momentum lost by the electrons is transferred. Recent ultrafast electron diffraction measurements [Tauchert \textit{et al.}, Nature {\bf 602},…

Materials Science · Physics 2025-12-08 M. S. Mrudul , Markus Weißenhofer , Peter M. Oppeneer

The crystal lattice governs the emergent electronic, magnetic, and optical properties of quantum materials, making structural tuning through strain, pressure, or chemical substitution a key approach for discovering and controlling novel…

Using a combination of first-principles and magnetization-dynamics calculations, we study the effect of the intense optical excitation of phonons on the magnetic behavior in insulating magnetic materials. Taking the prototypical…

Strongly Correlated Electrons · Physics 2018-06-13 M. Fechner , A. Sukhov , L. Chotorlishvili , C. Kenel , J. Berakdar , N. A. Spaldin

We theoretically investigate the optically-induced demagnetization of ferromagnetic FePt using the time-dependent density functional theory (TDDFT). We compare the demagnetization mechanism in the perturbative and nonperturbative limits of…

Materials Science · Physics 2024-04-26 M. S. Mrudul , Peter M. Oppeneer

All-optical control dynamics of magnetization in sub-10 nm metallic thin films are investigated, as these films with quantum confinement undergo unique interactions with femtosecond laser pulses. Our theoretical derivations based on the…

Mesoscale and Nanoscale Physics · Physics 2021-08-11 Saeedeh Mokarian Zanjani , Muhammad Tahir Naseem , Özgür Müstecaplıoğlu , Mehmet Cengiz Onbaşlı

Terahertz (THz) lasers provide a new research perspective for spin electronics applications due to their sub-picosecond time resolution and non-thermal ultrafast demagnetization, but the interaction between spin, charge and lattice dynamics…

Materials Science · Physics 2025-06-06 Yiqi Huo , Shuo Li , Luo Yan , Ningbo Li , Sergei Tretiak , Liujiang Zhou

Despite intense experimental effort, theoretical proposals and modeling approaches, a lack of consensus exists about the intrinsic mechanisms driving ultrafast magnetization dynamics in 3$d$ ferromagnets. In this work, we find evidence of…

Materials Science · Physics 2023-03-29 Theodor Griepe , Unai Atxitia

Altermagnets have recently attracted considerable interest due to their unique symmetry-governed spintronic properties. Here, we investigate phonon-induced magnon spin currents in a two-dimensional altermagnet. Starting from a microscopic…

Mesoscale and Nanoscale Physics · Physics 2026-05-20 Sofie Helene Ursin , Mathias Kläui , Kjetil M. D. Hals
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