A coherent THz optical lattice mode is triggered by femtosecond laser pulses in the antiferromagnetic van der Waals semiconductor FePS3. The 380 nm thick exfoliated flake was placed on a substrate and laser-driven lattice and spin dynamics were investigated as a function of the excitation photon energy and sample temperature. The pump-probe spectroscopic measurements reveal that the photo-induced phonon is generated by a displacive mechanism. The amplitude of the phononic signal decreases as the sample is heated up to the N\'eel temperature and vanishes as the phase transition to the paramagnetic phase occurs. This evidence confirms that the excited lattice mode is intimately connected to the long-range magnetic order. Therefore our work discloses a pathway towards a femtosecond coherent manipulation of the magneto-crystalline anisotropy in a van der Waals antiferromagnet. In fact, it is reported that by applying a magnetic field the induced phonon mode hybridizes via the Kittel-mechanism with zone-centre magnons.
@article{arxiv.2111.01464,
title = {Ultrafast coherent THz lattice dynamics coupled to spins in a van der Waals antiferromagnetic flake},
author = {Fabian Mertens and David Mönkebüscher and Eugenio Coronado and Samuel Mañas-Valero and Carla Boix-Constant and Alberta Bonanni and Margherita Matzer and Rajdeep Adhikari and Alexandra M. Kalashnikova and Davide Bossini and Mirko Cinchetti},
journal= {arXiv preprint arXiv:2111.01464},
year = {2021}
}
Comments
The following article has been submitted to Applied Physics Letters. After it is published, it will be found at https://aip.scitation.org/journal/apl