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We utilize ultrafast photoexcitation to drive coherent lattice oscillations in the layered ferrimagnetic crystal Mn3Si2Te6, which significantly stiffen below the magnetic ordering temperature. We suggest that this is due to an…

CoPS3 stands out in the family of the van der Waals antiferromagnets XPS3 (X=Mn, Ni, Fe, Co) due to the unquenched orbital momentum of the magnetic Co2+ ions which is known to facilitate the coupling of spins to both electromagnetic waves…

The control of antiferromagnets with ultrashort optical pulses has emerged as a prominent field of research. Tailored laser excitation can launch coherent spin waves at terahertz frequencies, yet a comprehensive description of their…

The crystal lattice governs the emergent electronic, magnetic, and optical properties of quantum materials, making structural tuning through strain, pressure, or chemical substitution a key approach for discovering and controlling novel…

We combine polarized infrared magneto-transmission and Faraday angle rotation measurements to map the collective excitations of the van der Waals antiferromagnet FePS$_3$. Below the N\'{e}el temperature ($T_\mathrm{N} \approx 118$ K), the…

Strongly Correlated Electrons · Physics 2025-08-21 Kartik Panda , Itzik Kapon , Dumitru Dumcenco , Dirk van der Marel , Alexey Kuzmenko , Nimrod Bachar

Strong-field terahertz (THz) excitations enable dynamic control over electronic, lattice and symmetry degrees of freedom in quantum materials. Here, we uncover pronounced terahertz-induced symmetry modulations and coherent phonon dynamics…

The impulsive generation of two-magnon modes in antiferromagnets by femtosecond optical pulses, so-called femto-nanomagnons, leads to coherent longitudinal oscillations of the antiferromagnetic order parameter that cannot be described by a…

Mesoscale and Nanoscale Physics · Physics 2019-07-31 D. Bossini , S. Dal Conte , O. Gomonay , R. V. Pisarev , M. Borovsak , D. Mihailovic , J. Sinova , G. Cerullo , J. H. Mentink , Th. Rasing , A. V. Kimel

We investigate the out-of-equilibrium lattice dynamics in the spin-ladder system $\alpha'$-NaV$_2$O$_5$ using intense terahertz (THz) pump and near-infrared (NIR) probe spectroscopy. When quasi-single-cycle THz pulses interact with…

Spintronics is postulated on the possibility to employ the magnetic degree of freedom of electrons for computation and couple it to charges. In this view, the combination of the high-frequency of spin manipulations offered by…

Magnetic order parameters in altermagnets can couple to quantized lattice vibration via both piezomagnetic and magnetoelastic effects, leading to the renormalization of phonon dispersion. Here, we demonstrate photo-induced dynamic frequency…

Fe$_3$GeTe$_2$ is a prototypical metallic van der Waals ferromagnet with itinerant magnetism and a highly tunable Curie temperature, yet how electronic excitations couple to spin and lattice degrees of freedom across its magnetic transition…

Understanding spin-lattice coupling represents a key challenge in modern condensed matter physics, with crucial importance and implications for ultrafast and 2D-magnetism. The efficiency of angular momentum and energy transfer between spins…

Terahertz (THz) lasers provide a new research perspective for spin electronics applications due to their sub-picosecond time resolution and non-thermal ultrafast demagnetization, but the interaction between spin, charge and lattice dynamics…

Materials Science · Physics 2025-06-06 Yiqi Huo , Shuo Li , Luo Yan , Ningbo Li , Sergei Tretiak , Liujiang Zhou

We use ultrafast optical spectroscopy to investigate the electronic and lattice dynamics of the charge-density wave (CDW) material 1$T$-TiSe$_2$ across various temperatures and pump fluences. We reveal a close relationship between the…

Strongly Correlated Electrons · Physics 2026-04-28 Xue-Qing Ye , Hao Liu , Qi-Yi Wu , Chen Zhang , Xiao-Fang Tang , Bo Chen , Chuan-Cun Shu , Hai-Yun Liu , Yu-Xia Duan , Peter M. Oppeneer , Jian-Qiao Meng

Understanding spin-lattice interactions in antiferromagnets is one of the most fundamental issues at the core of the recently emerging and booming fields of antiferromagnetic spintronics and magnonics. Recently, coherent nonlinear…

We report on the dynamics of coherent phonons in semimetal 1T'-MoTe2 using femtosecond pump-probe spectroscopy. On an ultrafast sub-picosecond time scale at room temperature, a low frequency and long-lifetime shear phonon mode was observed…

Materials Science · Physics 2020-03-09 T. Fukuda , K. Makino , Y. Saito , P. Fons , A. V. Kolobov , K. Ueno , M. Hase

We investigate the excitation of phonons in photoexcited antimony and demonstrate that the entire electron-lattice interactions, in particular coherent and incoherent electron-phonon coupling, can be probed simultaneously. Using femtosecond…

Magnetic order in van der Waals magnets can strongly influence their lattice dynamics, yet how this interaction manifests across different phonon length scales remains unclear. Optical phonons probe bond-scale exchange modulation and…

Femtosecond dynamics of coherent optical phonons in GeTe/Sb$_{2}$Te$_{3}$ superlattices (SLs), a new class of semiconductor SLs with three different states, have been investigated by using a reflection-type pump-probe technique at various…

Materials Science · Physics 2015-03-23 Muneaki Hase , Yoshinobu Miyamoto , Junji Tominaga

Emergent cooperative motions of individual degrees of freedom, i.e. collective excitations, govern the low-energy response of system ground states under external stimulations and play essential roles for understanding many-body phenomena in…

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