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In continuous-variable quantum information processing, it is crucial to develop high-efficiency and broadband quantum memory of squeezed light, which enables the storage of full-bandwidth information. Here, we present a quantum memory of…

The range of stimulated Raman scattering (SRS) frequencies covers a domain which at the low end abuts half the laser frequency, omega_0 / 2, according to the simplest SRS theories, corresponding to scatter from electron densities near 1/4…

Plasma Physics · Physics 2015-05-20 Harvey A. Rose , Philippe Mounaix

Implementing stimulated Raman scattering in a low-loss microresonator could lead to Raman lasing. Here, we report the demonstration of an efficient Raman laser with $>50 \%$ power efficiency in an integrated silicon carbide platform for the…

Properties of quantum states have disclosed new technologies, ranging from quantum information to quantum metrology. Among them a recent research field is quantum imaging, addressed to overcome limits of classical imaging by exploiting…

Quantum Physics · Physics 2010-04-09 G. Brida , M. Genovese , I. Ruo Berchera

Rapid detection of bacterial growth is crucial in clinical, food safety, and environmental contexts, yet conventional optical methods are limited by noise and require hours of incubation. Here, we present the first experimental…

Coherent anti-Stokes Raman scattering (CARS) microscopy offers label-free chemical imaging capabilities, but its performance is constrained by small Raman scattering cross-section, strong non-resonant background (NRB), and limited…

Chemical imaging enabled by Raman processes is crucial to investigating biological and chemical samples in a label-free manner. Stimulated Raman spectroscopy (SRS) overcomes the key limitation associated with low signal levels in…

Optics · Physics 2026-03-25 Florian M. Schweizer , Hannah Terrasa , Manish Garg

Femtosecond, broadband stimulated Raman spectroscopy is a popular approach to measuring molecular dynamics with excellent signal-to-noise and spectral resolution. We present a new method for broadband stimulated Raman spectroscopy that…

Optics · Physics 2025-08-19 Nathan G. Drouillard , TJ Hammond

Raman sensing and Raman microscopy are amongst the most specific optical technologies to identify the chemical compounds of unknown samples, and to enable label-free biomedical imaging with molecular contrast. However, the high cost and…

Understanding and controlling decoherence in open quantum systems is of fundamental interest in science, while achieving long coherence times is critical for quantum information processing. Although great progress was made for individual,…

Mesoscale and Nanoscale Physics · Physics 2023-03-23 Lisanne Sellies , Raffael Spachtholz , Philipp Scheuerer , Jascha Repp

In Impulsive Stimulated Raman Scattering vibrational oscillations, coherently stimulated by a femtosecond Raman pulse, are real time monitored and read out as intensity modulations in the transmission of a temporally delayed probe pulse.…

Chemical Physics · Physics 2019-11-28 Giovanni Batignani , Carino Ferrante , Giuseppe Fumero , Tullio Scopigno

The principle and experimental realization of a novel Raman spectroscopic technique entitled stimulated Raman phase shift (SRPS) spectroscopy was demonstrated. This technique depends on the measurement of the stimulated Raman scattering…

Optics · Physics 2024-03-07 Meng Qi , Wenrong Wang , Yuan-ji Li , Jin-xia Feng , Kuan-shou Zhang

Single-beam spectrally controlled (SBSC) two-dimensional (2D) Raman spectroscopy is a unique 2D vibrational measurement technique utilizing trains of short pulses that are generated from a single broadband pulse by pulse shaping. This…

Chemical Physics · Physics 2021-03-30 Ju-Yeon Jo , Yoshitaka Tanimura

We propose and theoretically analyze a new vibrational spectroscopy, termed electron- and light-induced stimulated Raman (ELISR) scattering, that combines the high spatial resolution of electron microscopy with the molecular sensitivity of…

Optics · Physics 2020-08-12 Amr A. E. Saleh , Daniel K. Angell , Jennifer A. Dionne

Label-free nonlinear optical microscopy has become a powerful tool for biomedical research. However, the possible photodamage risk hinder further clinical applications. To reduce these adverse effects, we constructed a new platform of…

Optics · Physics 2022-10-26 Geng Wang , Stephen A. Boppart , Haohua Tu

Magnetic Resonance Spectroscopy (MRS) is a noninvasive tool to reveal metabolic information. One challenge of 1H-MRS is the low Signal-Noise Ratio (SNR). To improve the SNR, a typical approach is to perform Signal Averaging (SA) with M…

We propose a radical advance in Magnetic Resonance Imaging. MRI remains slow because it requires successive applications of magnetic field gradients to encode for spatial location. Parallel MRI accelerates imaging by permitting…

Medical Physics · Physics 2018-09-19 Michael Hutchinson , Ulrich Raff , Luis Osorio

We measured the spin noise spectroscopy (SNS) of rubidium atomic ensemble with two different atomic vapor cells (filled with the buffer gases or coated with paraffin film on the inner wall), and demonstrated the enhancement of signal to…

Quantum Physics · Physics 2022-01-19 Lele Bai , Lulu Zhang , Yongbiao Yang , Rui Chang , Yao Qin , Jun He , Xin Wen , Junmin Wang

We theoretically propose a new method in cavity- and surface-enhanced Raman spectroscopy (SERS) with improved temporal resolution in the measurement of stochastic Raman spectral fluctuations. Our approach combines Fourier spectroscopy and…

Optics · Physics 2025-07-02 Colburn Cobb-Bruno , Hendrik Utzat

The chaotic nature of x-ray free-electron-laser pulses is a major bottleneck that has limited the joint temporal and spectral resolution of spectroscopic measurements. We show how to use the stochastic x-ray field statistics to overcome…

Optics · Physics 2021-02-15 Stefano M. Cavaletto , Daniel Keefer , Shaul Mukamel
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