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Quantum-mechanical investigation is presented to study single attosecond pulse generation by gating high-order harmonic emission from H$_2^+$ molecule in intense laser pulses with time-dependent ellipticity. The high-order harmonic…

Atomic Physics · Physics 2018-01-17 Nehzat Safaei

Bright squeezed light from parametric down-conversion in the infrared (IR) frequency range has triggered the emergence of attosecond quantum optics -- a new research field at the interface of quantum optics, strong-field physics, and…

The shortest light pulses produced to date are of the order of a few tens of attoseconds, with central frequencies in the extreme ultraviolet range and bandwidths exceeding tens of eV. They are often produced as a train of pulses separated…

High-order harmonic generation (HHG), a robust tabletop source for producing attosecond pulses, has been extensively utilized in attosecond metrology. Traditionally, HHG driven by classical laser fields involves two typical quantum paths…

The ongoing development of intense high-harmonic generation (HHG) sources has recently enabled highly nonlinear ionization of atoms by the absorption of at least 10 extreme-ultraviolet (XUV) photons within a single atom [Senfftleben…

Recently, a spatiotemporal optical vortex (STOV) with a transverse orbital angular momentum (OAM) has been generated from coherent ultrafast pulses using mode-locked lasers. In contrast, we demonstrate theoretically and experimentally that…

Optics · Physics 2021-09-22 Amal Mirando , Yimin Zang , Qiwen Zhan , Andy Chong

The generation of attosecond X-ray pulses has garnered significant attention within the X-ray free-electron laser (FEL) community due to their potential for ultrafast time-resolved studies. Such pulses enable the investigation of electron…

Accelerator Physics · Physics 2025-12-01 Tu Lingjun , Sun Hao , Yi Huaiqian , Zeng Li , Liang Yifan , Yu Yong , Wang Xiaofan , Zhang Weiqing

Harmonic generation from solid surfaces is a promising tool for producing high energy attosecond pulses. We report shaping of the harmonic spectrum to achieve the bandwidth necessary for attosecond pulse generation. The shaping is…

Plasma Physics · Physics 2019-03-27 A. Seyen , R. Kohn , U. Bovensiepen , D. von der Linde , A. Tarasevitch

We generate high-order harmonics at high pulse repetition rates using a turnkey laser. High-order harmonics at 400 kHz are observed when argon is used as target gas. In neon we achieve generation of photons with energies exceeding 90 eV…

The mechanism underlying high harmonic generation (HHG) in gases has been well clarified, characterizing attosecond pulse trains (APT) in the time domain, significantly advances the synthesis of isolated attosecond pulse (IAP). However, the…

Optics · Physics 2025-07-25 Qing-Guo Fan , Kang Lai , Wen-hao Liu , Zhi Wang , Lin-Wang Wang , Jun-Wei Luo

We investigate the use of light beams carrying orbital angular momentum (OAM) in the context of high harmonic generation (HHG) within semiconductor crystals. Our contribution deals with the transfer and conservation of OAM in the…

Optics · Physics 2024-10-01 C. Granados , B. Kumar Das , M. F. Ciappina

We propose an effective scheme for the generation of intense coherent extreme ultraviolet light beams carrying orbital angular momentum (OAM). The light is produced by a high-gain harmonic-generation free-electron laser (FEL), seeded using…

Optics · Physics 2013-12-23 Primož Rebernik Ribič , David Gauthier , Giovanni De Ninno

The physics of high harmonics has led to the generation of attosecond pulses and to trains of attosecond pulses. Measurements that confirm the pulse duration are all performed in the far field. All pulse duration measurements tacitly assume…

Optics · Physics 2012-06-15 E. Frumker , G. G. Paulus , H. Niikura , A. Naumov , D. M. Villeneuve , P. B. Corkum

We present experimental results showing the appearance of a near-continuum in the high-order harmonic generation (HHG) spectra of atomic and molecular species as the driving laser intensity of an infrared pulse increases. Detailed…

We study high-order harmonic generation (HHG) resulting from the illumination of plasmonic nanostructures with a short laser pulse. We show that both the inhomogeneities of the local electric field and the confinement of the electron motion…

Atomic Physics · Physics 2012-04-27 M. F. Ciappina , Srdjan S. Acimovic , T. Shaaran , J. Biegert , R. Quidant , M. Lewenstein

We show that the divergence of extreme ultraviolet pulses from high harmonic generation, which is directly linked to the shape and size of the refocused beam, can be controlled by the relative delay between the fundamental and its intense…

High harmonic generation (HHG) from gas phase atoms (or molecules) has opened up a new frontier in ultrafast optics, where attosecond time resolution and Angstrom spatial resolution are accessible. The fundamental physical pictures of HHG…

Optics · Physics 2023-04-26 Liang Li , Pengfei Lan , Xiaosong Zhu , Peixiang Lu

Hermite-Gaussian (HG) beams are standard modes delivered by continuous or pulsed lasers systems, and pulse-front tilt is one of the most common, detrimental or beneficial, spatiotemporal couplings affecting ultrashort pulses. Combining…

Optics · Physics 2025-05-16 Miguel A. Porras , Spencer W. Jolly

Ultrafast extreme ultraviolet (XUV) sources with a controllable polarization state are powerful tools for investigating the structural and electronic as well as the magnetic properties of materials. However, such light sources are still…

Plasma Physics · Physics 2016-08-18 Zi-Yu Chen , Alexander Pukhov

The irradiation of atoms by a strong IR laser field of frequency $\omega$ results in the emission of odd-harmonics of $\omega$ ("IR harmonics") up to some maximal cut-off frequency. The addition of an XUV field of frequency…

Atomic Physics · Physics 2008-02-04 Avner Fleischer , Nimrod Moiseyev
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