Related papers: Attosecond vortex pulse trains
Structured light carrying orbital angular momentum enables new regimes of nonlinear light-matter interaction. Here we develop a molecular quantum electrodynamics description of third-harmonic generation (THG) driven by focused…
In any form of wave propagation, strong spatiotemporal coupling appears when non-elementary, three-dimensional wave-packets are composed by superimposing pure plane waves, or spontaneously generated by light-matter interaction and nonlinear…
Recently, the possibility of the generation and interaction of unipolar half-cycle electromagnetic pulses with quantum systems has been the subject of active research. Such pulses can have many different and interesting applications. They…
High-order harmonic generation stands as a unique nonlinear optical up-conversion process, mediated by a laser-driven electron recollision mechanism, which has been shown to conserve energy, momentum, and spin and orbital angular momentum.…
We present observations of the emission of XUV continua in the 20-37 eV region by high harmonic generation (HHG) with $4$-$7\ \mathrm{fs}$ pulses focused onto a Kr gas jet. The underlying mechanism relies on coherent control of the relative…
Attosecond electron pulses enable real-time probing of ultrafast matter dynamics, yet conventional modulation schemes suffer from drastically shortened longitudinal focal lengths when targeting sub-attosecond durations. To address this…
High harmonic spectra generated in condensed matter carry the fingerprints of sub-cycle electronic motion and the energy structure of the studied system. Here we show that tailoring the waveform of mid-infrared driving light by using a…
High harmonic generation (HHG) in solids could enable attosecond and ultraviolet light sources with high compactness, great controllability and rich functions. However, the HHG process is accompanied by a quite large wavevector mismatch…
We identify and explore a high orbital angular momentum (OAM) harmonics generation and amplification mechanism that manipulates the OAM independently of any other laser property, by preserving the initial laser wavelength, through…
High-harmonic generation (HHG) in two-dimensional materials offers a compelling route toward compact extreme ultraviolet sources and probing electron dynamics on the attosecond scale. However, achieving precise control over the emission and…
In this work the experimental realization of a tunable high photon flux extreme ultraviolet light source is presented. This is enabled by high harmonic generation of two temporally delayed driving pulses, resulting in a tuning range of 0.8…
High-order harmonic generation by the diffraction of an intense Laguerre-Gaussian (LG) laser beam through a small aperture is studied. It is found that the 2D peripheral electron dynamics on the rim can facilitate complex interplay between…
The generation of relativistic vortex electron beams via photoemission requires ultraviolet laser beams with well-controlled orbital angular momentum (OAM) and compatibility with radio-frequency (RF) photoinjector drive-laser systems.…
High-harmonic generation (HHG), an extreme nonlinear effect, introduces an unprecedented paradigm to detect emergent quantum phases and electron dynamics inconceivable in the framework of linear and low-order nonlinear processes. As an…
High-harmonic generation (HHG) in liquids is opening new opportunities for attosecond light sources and attosecond time-resolved studies of dynamics in the liquid phase. In gas-phase HHG, few-cycle pulses are routinely used to create…
Spatiotemporal optical vortex (STOV) with transverse orbital angular momentum (TOAM) can induce some novel properties in high energy density physics. However, the current STOV pulse energy is limited to the mJ level, which greatly hinders…
Energy coupling during relativistically intense laser-matter interactions is encoded in the attosecond motion of strongly driven electrons at the pre-formed plasma-vacuum boundary. Studying and controlling this motion can reveal details…
For decades, most research on high harmonic generation (HHG) considered matter as quantum but light as classical, leaving the quantum-optical nature of the harmonics an open question. Here we explore the quantum properties of high…
Accelerating and colliding particles has been a key strategy to explore the texture of matter. Strong lightwaves can control and recollide electronic wavepackets, generating high-harmonic (HH) radiation which encodes the structure and…
We study the high harmonic generation with vortex beams beyond the dipole approximation. To do so we employ the full minimal coupling approach to account for multipolar coupling without truncation and describe the full spatio-temporal…