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Structured light enables the characterization of chirality of optically small nanoparticles by taking advantage of the helicity maximization concept recently introduced in[1]. By referring to fields with nonzero helicity density as chiral…

Applied Physics · Physics 2020-11-04 Mina Hanifeh , Mohammad Albooyeh , Filippo Capolino

For over three decades, the study of optical vortex beams carrying orbital angular momentum (OAM) has been at the forefront of optics, driven by fundamental questions about optical momentum as well as diverse applications in quantum…

Optics · Physics 2025-08-15 Kayn A Forbes

Chirality is a fundamental asymmetry phenomenon, with chiral optical elements exhibiting asymmetric response in reflection or absorption of circularly polarized light. Recent realizations of such elements include nanoplasmonic systems with…

It has been observed that achiral nano-particles, such as flat helices, may be subjected to an optical torque even when illuminated by normally incident linearly polarized light. However, the origin of this fascinating phenomenon has so far…

Optics · Physics 2023-05-29 Karim Achouri , Mintae Chung , Andrei Kiselev , Olivier J. F. Martin

Light interaction with rotating nanostructures gives rise to phenemona as varied as optical torques and quantum friction. Here we reveal that circular dichroism of rotating optically-isotropic particles has an unexpectedly strong dependence…

Mesoscale and Nanoscale Physics · Physics 2019-08-14 Deng Pan , Hongxing Xu , F. Javier García de Abajo

We report observation of electron helical dichroism on a material with chiral structure. In analogy with circular dichroism, a common technique for molecular structural fingerprinting, we use a nanofabricated forked diffraction grating to…

Materials Science · Physics 2015-07-08 Tyler R. Harvey , Jordan S. Pierce , Jordan J. Chess , Benjamin J. McMorran

Chiral light-matter interactions have traditionally been understood in terms of electric-magnetic dipolar interference driven by light with spin angular momentum. Here, we show that optical chirality can also originate from the orbital…

Optics · Physics 2025-08-13 Shun Hashiyada , An'an Wu , Yoshito Y. Tanaka

Nonlinear chiral photonics explores nonlinear response of chiral structures, and it offers a pathway to novel optical functionalities not accessible through linear or achiral systems. Here we present the first application of nanostructured…

Whether or not chiral interaction exists between the optical orbital angular momentum (OAM) and a chiral molecule remains unanswered. So far, such an interaction has not been observed experimentally. Here we present a T-matrix method to…

Optics · Physics 2018-01-01 Tong Wu , Rongyao Wang , Xiangdong Zhang

We present a system consisting of two stacked chiral plasmonic nanoelements, so-called triskelia, that exhibits a high degree of circular dichroism. The optical modes arising from the interactions between the two elements are the main…

Artificial nanostructures enable fine control of electromagnetic fields at the nanoscale, a possibility that has recently been extended to the interaction between polarised light and chiral matter. The theoretical description of such…

We investigate the polarization dependence of optical nonlinearity enhancement for a uniaxial anisotropic composite of metal nanocrystals in a dielectric host. Three cases are distinguished depending on whether the polarization is parallel,…

Soft Condensed Matter · Physics 2007-05-23 K. P. Yuen , M. F. Law , K. W. Yu , Ping Sheng

We explore experimentally if the light's orbital angular momentum (OAM) interacts with chiral nematic polymer films. Specifically, we measure the circular dichroism of such a material using light beams with different OAM. We investigate the…

Optics · Physics 2011-06-20 W. Löffler , D. J. Broer , J. P. Woerdman

Azimuthal orientation and handedness dependence of the optical responses, accompanied by asymmetric transmission and asymmetric dichroism, were demonstrated on multilayers constructed with subwavelength periodic arrays of Babinet…

Optics · Physics 2024-04-29 Emese Tóth , Olivér A. Fekete , Balázs Bánhelyi , Mária Csete

Optically active achiral metasurfaces offer a promising way to detect chiral molecules based on chiroptic methods. The combination of plasmonic enhanced circular dichroism and reversible optical activity would boost the sensitivity and…

Structured x-rays carrying an orbital angular momentum break spatial inversion symmetry and have been proposed as a means to probe chirality. We theoretically investigate twisted non-resonant x-ray diffraction from chiral molecules and…

Optics · Physics 2026-03-02 Akilesh Venkatesh , Phay J. Ho , Jérémy R. Rouxel

As characteristic lengths in plasmonics rapidly approach the sub-nm regime, quantum-informed models that can capture those aspects of the quantum nature of the electron gas that are not accessible by the standard approximations of classical…

Mesoscale and Nanoscale Physics · Physics 2018-12-20 Christos Tserkezis , A. T. Mina Yeşilyurt , Jer-Shing Huang , N. Asger Mortensen

We investigate the nonlinear optical response of a four-level double-V-type quantum system interacting with a pair of weak probe fields while located near a two-dimensional array of metal-coated dielectric nanospheres. Such a quantum system…

Quantum Physics · Physics 2020-04-27 Hamid Reza Hamedi , Vassilios Yannopapas , Emmanuel Paspalakis

Resonant dielectric planar structures can interact selectively with light of particular helicity thus providing an attractive platform for chiral flat optics. The absence of mirror-symmetry planes defines geometric chirality, and it remains…

We introduce meta-diastereomers, hybrid systems where molecular chirality ($\leq 10$\,nm) and nanoscale chirality ($>100$\,nm) combine to create a new hierarchical chiral state with emergent optical properties. By coupling chiral…