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Strong coupling between a single quantum emitter and an electromagnetic mode is one of the key effects in quantum optics. In the cavity QED approach to plasmonics, strongly coupled systems are usually understood as single-transition…

The formation of hybrid light-molecule states (polaritons) offers a new strategy to manipulate the photochemistry of molecules. To fully exploit its potential, one needs to build a toolbox of polaritonic phenomenologies that supplement…

Mesoscale and Nanoscale Physics · Physics 2018-11-20 Jacopo Fregoni , Giovanni Granucci , Emanuele Coccia , Maurizio Persico , Stefano Corni

Strong light-matter coupling has shown great potential for modifying the electro-optical properties of semiconducting materials in recent years. In the strong coupling regime, excitons and cavity photons form new states named…

Applied Physics · Physics 2023-11-23 Yahui Tang , Alexandra Stuart , Timothy van der Laan , Girish Lakhwani

We observe vacuum Rabi splitting in a lossy nearly confocal cavity indicating the strong coupling regime, despite a weak single-atom single-mode coupling. Strong collective interaction manifests itself in the typical $\sqrt{N}$-dependence…

Quantum Gases · Physics 2011-11-30 A. Wickenbrock , P. Phoonthong , F. Renzoni

Strong light-matter coupling provides a versatile and novel means to manipulate chemical processes. Here we develop a theoretical framework to investigate the spectroscopy and dynamics of a molecular ensemble embedded in an optical cavity…

Quantum Physics · Physics 2023-06-16 Bing Gu

We propose a set of photonic crystals that realize a nonlinear quantum Rabi model equivalent to a two-level system driven by the phase of a quantized electromagnetic field. The crystals are exactly soluble in the weak-coupling regime and…

Enhancing the light-matter interactions in two-dimensional materials via optical metasurfaces has attracted much attention due to its potential to enable breakthrough in advanced compact photonic and quantum information devices. Here, we…

We extend the model of exciton-plasmon materials to include a ro-vibrational structure of molecules using wave-packet propagations on electronic potential energy surfaces. The new model replaces conventional two-level emitters with more…

Mesoscale and Nanoscale Physics · Physics 2017-08-18 Maxim Sukharev , Eric Charron

We simulate the near-field effects of strong coupling between molecular excitons and localized surface plasmons, supported by aluminum nanodisks. The simulations are done using a simple model of a two-level system, implemented in a…

Mesoscale and Nanoscale Physics · Physics 2020-01-29 Nadav Fain , Tal Ellenbogen , Tal Schwartz

We develop coupled-cluster theory for systems of electrons strongly coupled to photons, providing a promising theoretical tool in polaritonic chemistry with a perspective of application to all types of fermion-boson coupled systems. We show…

Circuit quantum electrodynamics allows one to probe, manipulate and couple superconducting quantum bits using cavity photons at an exquisite level. One of its cornerstones is the possibility to achieve the strong coupling which allows one…

Mesoscale and Nanoscale Physics · Physics 2018-10-24 L. E Bruhat , T. Cubaynes , J. J. Viennot , M. C. Dartiailh , M. M. Desjardins , A. Cottet , T. Kontos

Strong light-matter coupling has recently been demonstrated in sub-wavelength volumes by coupling engineered optical transitions in semiconductor heterostructures (e.g., quantum wells) to metasurface resonances via near fields. It has also…

The quantum Rabi model, involving a two-level system and a bosonic field mode, is arguably the simplest and most fundamental model describing quantum light-matter interactions. Historically, due to the restricted parameter regimes of…

Polariton chemistry exploits the strong interaction between quantized excitations in molecules and quantized photon states in optical cavities to affect chemical reactivity. Molecular polaritons have been experimentally realized by the…

Chemical Physics · Physics 2023-09-06 Jonathan J. Foley , Jonathan F. McTague , A. Eugene DePrince

In the regime of strong coupling between molecular excitons and confined optical modes, the intra-molecular degrees of freedom are profoundly affected, leading to a reduced vibrational dressing of polaritons compared to bare electronically…

Mesoscale and Nanoscale Physics · Physics 2018-10-17 Javier del Pino , Florian A. Y. N. Schröder , Alex W. Chin , Johannes Feist , Francisco J. Garcia-Vidal

Recently considerable effort is devoted to the realization of the strong coupling regime of the radiation matter interaction in the context of emitter at a meta surface. The strong interaction is well realized in cavity quantum…

Quantum Physics · Physics 2018-03-01 Svend-Age Biehs , Chenran Xu , Girish S. Agarwal

This review outlines several linear optical effects featured by molecular polaritons arising in the collective strong light-matter coupling regime. Under weak laser irradiation and when the single-molecule light-matter coupling can be…

Molecular polaritons are the optical excitations which emerge when molecular transitions interact strongly with confined electromagnetic fields. Increasing interest in the hybrid molecular-photonic materials that host these excitations…

Mesoscale and Nanoscale Physics · Physics 2018-02-26 Raphael F. Ribeiro , Luis A. Martínez-Martínez , Matthew Du , Jorge Campos-Gonzalez-Angulo , Joel Yuen-Zhou

Room-temperature strong coupling between plasmonic nanocavities and monolayer semiconductors is a prominent path towards efficient, integrated light-matter interactions. However, designing such systems is challenging due to the nontrivial…

When atoms come together and bond, we call these new states molecules, and their properties determine many aspects of our daily life. Strangely enough, it is conceivable for light and molecules to bond, creating new hybrid light-matter…

Materials Science · Physics 2018-02-19 Branko Kolaric , Bjorn Maes , Koen Clays , Thomas Durt , Yves Caudano