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Motivated by the recent observation of superconductivity in the pressurized trilayer La$_4$Ni$_3$O$_{10}$ Ruddlesden-Popper (RP) nickelate, we explore its structural, electronic, and magnetic properties as a function of hydrostatic pressure…

Superconductivity · Physics 2024-07-19 Harrison LaBollita , Jesse Kapeghian , Michael R. Norman , Antia S. Botana

The newly discovered Ruddlesden-Popper bilayer La$_3$Ni$_2$O$_7$ reaches an remarkable superconducting transition temperature $T_c$ = 80 K under a pressure of above 14 GPa. Here we propose a minimal bilayer two-orbital model of the…

Superconductivity · Physics 2023-09-26 Zhihui Luo , Xunwu Hu , Meng Wang , Wéi Wú , Dao-Xin Yao

The recent discovery of superconductivity in bilayer La$_3$Ni$_2$O$_7$ (327-LNO) under pressure stimulated much interest in layered nickelates. However, superconductivity was not found in another bilayer nickelate system, La$_3$Ni$_2$O$_6$…

Superconductivity · Physics 2024-02-09 Yang Zhang , Ling-Fang Lin , Adriana Moreo , Thomas A. Maier , Elbio Dagotto

Motivated by the recently reported high-temperature superconductivity in the bilayer La$_3$Ni$_2$O$_7$ (LNO) under pressure, here we comprehensively study this system using {\it ab initio} techniques. The Ni $3d$ orbitals have a large…

Superconductivity · Physics 2023-11-29 Yang Zhang , Ling-Fang Lin , Adriana Moreo , Elbio Dagotto

It has been recently shown that under pressure trilayer Ruddlesden-Popper nickelate La$_4$Ni$_3$O$_{10}$ (LNO) becomes superconducting below a critical temperature $\sim$20 K, in addition to the infinite-layer and bilayer systems. Motivated…

Strongly Correlated Electrons · Physics 2024-06-12 I. V. Leonov

Atomic structure and electronic band structure are fundamental properties for understanding the mechanism of superconductivity. Motivated by the discovery of pressure-induced high-temperature superconductivity at 80 K in the bilayer…

Signatures of superconductivity under pressure have recently been reported in the bilayer La$_3$Ni$_2$O$_7$ and trilayer La$_4$Ni$_3$O$_{10}$ Ruddlesden-Popper (RP) nickelates with general chemical formula La$_{n+1}$Ni$_n$O$_{3n+1}$ ($n=$…

Superconductivity · Physics 2025-07-14 Yi-Feng Zhao , Antia S. Botana

Recently, signatures of superconductivity with critical temperature from 20 to 30 K have been reported in pressured trilayer nickelate La$_4$Ni$_3$O$_{10}$ through a pressure-induced structure transition. Here we explore the evolution of…

Strongly Correlated Electrons · Physics 2024-06-18 Peng-Fei Tian , Hao-Tian Ma , Xing Ming , Xiao-Jun Zheng , Huan Li

Motivated by the recently reported signatures of superconductivity in trilayer La$_4$Ni$_3$O$_{10}$ under pressure, we comprehensively study this system using {\it ab initio} and random-phase approximation techniques. Without electronic…

Superconductivity · Physics 2024-09-24 Yang Zhang , Ling-Fang Lin , Adriana Moreo , Thomas A. Maier , Elbio Dagotto

The discovery of superconductivity in Ruddlesden-Popper nickelates has established a new frontier in the study of high-temperature superconductors. However, the underlying pairing mechanism and its relationship to the material's electronic…

The recent experiment shows the superconducting transition temperature in the Ruddlesden-Popper bilayer La$_3$Ni$_2$O$_{7}$ decreases monotonically with increasing pressure above 14 GPa. In order to unravel the underlying mechanism for this…

Superconductivity · Physics 2025-02-25 Kai-Yue Jiang , Yu-Han Cao , Qing-Geng Yang , Hong-Yan Lu , Qiang-Hua Wang

Motivated by the recently proposed alternating single-layer trilayer stacking structure for the nickelate La$_3$Ni$_2$O$_7$, we comprehensively study this system using {\it ab initio} and random-phase approximation techniques. Our analysis…

Superconductivity · Physics 2024-08-15 Yang Zhang , Ling-Fang Lin , Adriana Moreo , Thomas A. Maier , Elbio Dagotto

We employ correlated density-functional theory methods (DFT + Hubbard $U$) to investigate the spin-density wave state of the bilayer Ruddlesden-Popper (RP) nickelate La$_{3}$Ni$_{2}$O$_{7}$ which becomes superconducting under pressure. We…

Strongly Correlated Electrons · Physics 2024-12-17 Harrison LaBollita , Victor Pardo , Michael R. Norman , Antia S. Botana

We study the possibility of superconductivity in a trilayer Ruddlesden-Popper nickelate La$_4$Ni$_3$O$_{10}$ under pressure both theoretically and experimentally, making comparison with the recently discovered high $T_c$ superconductor…

The recent discovery of bulk superconductivity in trilayer nickelate La$_4$Ni$_3$O$_{10}$ with the critical temperature $T_c$ near $30$K under high pressure is attracting a new wave of research interest, after the breakthrough of bilayer…

Superconductivity · Physics 2024-07-03 Qing-Geng Yang , Kai-Yue Jiang , Da Wang , Hong-Yan Lu , Qiang-Hua Wang

We report a comprehensive theoretical analysis of the Ruddlesden-Popper layered nickelates La$_{m+1}$Ni$_m$O$_{3m+1}$ ($m = 1$ to 6) under pressure. Our results suggest that, while these Ruddlesden-Popper layered nickelates display many…

Superconductivity · Physics 2025-11-07 Yang Zhang , Ling-Fang Lin , Adriana Moreo , Satoshi Okamoto , Thomas A. Maier , Elbio Dagotto

Motivated by the recent discovery of superconductivity in La$_3$Ni$_2$O$_7$ under pressure, we discuss the basic ingredients of a model that captures its microscopic physics under pressure tuning. We anchor our description in terms of the…

Superconductivity · Physics 2024-08-01 Zhiguang Liao , Lei Chen , Guijing Duan , Yiming Wang , Changle Liu , Rong Yu , Qimiao Si

The recent discovery of Ruddlesden--Popper (RP) nickelate thin-film superconductors has opened a new frontier in unconventional superconductivity. Its realization requires both compressive epitaxial strain and highly oxidative growth…

Trilayer Ruddlesden-Popper phase La4Ni3O10 has been observed with Tc of about 30 K at high pressure in recent experiment, which further expanded the family of nickelate superconductors. In this study, we explored the effects of electronic…

Strongly Correlated Electrons · Physics 2024-08-02 Zihao Huo , Peng Zhang , Zihan Zhang , Defang Duan , Tian Cui

The discovery of pressurized superconductivity at 80 K in La3Ni2O7 officially brings nickelates into the family of high-temperature superconductors, which gives rise to not only new insights but also mysteries in the strongly correlated…

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