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We investigate the electronic and structural changes at the nanoscale in vanadium dioxide (VO2) in the vicinity of its thermally driven phase transition. Both electronic and structural changes exhibit phase coexistence leading to…

The observation of electronic phase separation textures in vanadium dioxide (VO2), a prototypical electron-correlated oxide, has recently added new perspectives on the long standing debate about its metal-insulator transition and its…

Materials Science · Physics 2021-01-13 Felip Sandiumenge , Laura Rodriguez , Miguel Pruneda , Cesar Magen , Jose Santiso , Gustau Catalan

VO2 material is promising for developing energy-saving "smart window", owing to its thermochromic property induced by metal-insulator transition (MIT). However, its practical application is greatly limited by the relatively high critical…

Applied Physics · Physics 2019-05-10 Shi Chen , Zhaowu Wang , Hui Ren , Yuliang Chen , Wensheng Yan , Chengming Wang , Bowen Li , Jun Jiang , Chongwen Zou

In this paper we used Raman spectroscopy to investigate the optical properties of vanadium dioxide (VO2) thin films during the thermally induced insulating to metallic phase transition. We observed a significant difference in transition…

Materials Science · Physics 2013-01-14 E. Radue , E. Crisman , L. Wang , S. Kittiwatanakul , J. Lu , S. A. Wolf , R. Wincheski , R. A. Lukaszew , I. Novikova

A limiting optical diode is an asymmetric nonlinear device that is bidirectionally transparent at low power, but becomes opaque when illuminated by sufficiently intense light incident from a particular direction. We explore the use of a…

Photo-induced phase transitions (PIPTs) provide an ultrafast, energy-efficient way for precisely manipulating the topological properties of transition-metal ditellurides, and can be used to stabilize a topological phase in an otherwise…

Materials Science · Physics 2020-06-23 Bo Peng , Hao Zhang , Weiwen Chen , Zhi-Jun Qiu , Hezhu Shao , Heyuan Zhu , Bartomeu Monserrat , Desheng Fu , Hongming Weng

Characterizing and controlling the out-of-equilibrium state of nanostructured Mott insulators hold great promises for emerging quantum technologies while providing an exciting playground for investigating fundamental physics of…

Nitrogen vacancy (NV) centers, optically-active atomic defects in diamond, have attracted tremendous interest for quantum sensing, network, and computing applications due to their excellent quantum coherence and remarkable versatility in a…

Mesoscale and Nanoscale Physics · Physics 2021-04-06 Nathan J. McLaughlin , Yoav Kalcheim , Albert Suceava , Hailong Wang , Ivan K. Schuller , Chunhui Rita Du

We investigated the origin of collective electronic phase transitions induced at the heterointerface between monoclinic insulating VO2 and rutile metallic electron-doped VO2 layers using in situ soft x-ray photoemission spectroscopy (PES)…

Strongly Correlated Electrons · Physics 2025-10-23 D. Shiga , S. Inoue , T. Kanda , N. Hasegawa , M. Kitamura , K. Horiba , K. Yoshimatsu , A. F. Santander-Syro , H. Kumigashira

We report on local probe measurements of current-voltage and electrostatic force-voltage characteristics of electric-field-induced insulator to metal transition in VO2 thin film. In conducting AFM mode, switching from the insulating to…

Strongly Correlated Electrons · Physics 2012-01-09 B. Wu , A. Zimmers , H. Aubin , R. Ghosh , Y. Liu , R. Lopez

Textured VO2(011) microcrystals are grown in the monoclinic, M1 phase which undergo a reversible first order semiconductor to metal transition (SMT) accompanied by a structural phase transition to rutile tetragonal, R phase. Around the…

Materials Science · Physics 2017-10-26 Raktima Basu , P. Magudapathy , Manas Sardar , Ramanathaswamy Pandian , Sandip Dhara

The single crystal VO2, exihibiting a first-order metal-insulator transition (MIT) at 67.2 degrees C and an insulator-insulator transition (IIT) at ~49.7 degrees C, is grown. From synchrotron-based x-ray microdiffraction analysis, the IIT…

Impedance spectroscopy measurements were performed in high quality Vanadium dioxide (VO2) thin films. This technique allows us investigate the resistive and capacitive contribution to the dielectric response near the metal-insulator…

Materials Science · Physics 2011-05-24 J. -G. Ramírez , Edgar J. Patiño , Rainer Schmidt , Amos Sharoni , M. E. Gómez , Ivan K. Schuller

Many strongly correlated electronic materials, including high-temperature superconductors, colossal magnetoresistance and metal-insulator-transition (MIT) materials, are inhomogeneous on a microscopic scale as a result of domain structure…

Mesoscale and Nanoscale Physics · Physics 2012-09-05 Jiang Wei , Zenghui Wang , Wei Chen , David H. Cobden

Assembling transition metal dichalcogenides (TMDCs) at the two-dimensional (2D) limit is a promising approach for tailoring emerging states of matter such as superconductivity or charge density waves (CDWs). Single-layer (SL) VSe$_2$ stands…

RF radiation spectrum is central to wireless and radar systems among numerous high-frequency device technologies. Here, we demonstrate sensing of RF signals in the technologically relevant 2.4 GHz range utilizing vanadium dioxide (VO2), a…

Spinodal decomposition is a ubiquitous phenomenon leading to phase separation from a uniform solution. We show that a spinodal decomposition occurs in a unique combination of two rutile compounds of TiO2 and VO2, which are chemically and…

Strongly Correlated Electrons · Physics 2013-06-12 Zenji Hiroi , Hiroaki Hayamizu , Toru Yoshida , Yuji Muraoka , Yoshihiko Okamoto , Jun-ichi Yamaura , Yutaka Ueda

We present the first comprehensive broadband optical spectroscopy data on two insulating phases of vanadium dioxide (VO2): monoclinic M2 and triclinic. The main result of our work is that the energy gap and the electronic structure are…

Strongly Correlated Electrons · Physics 2017-02-22 T. J. Huffman , C. Hendriks , E. J. Walter , Joonseok Yoon , Honglyoul Ju , R. Smith , G. L. Carr , H. Krakauer , M. M. Qazilbash

Vanadium dioxide (VO$_{2}$) undergoes a first-order metal-insulator transition (MIT) upon cooling near room temperature, concomitant with structural change from rutile to monoclinic. Accurate characterization of lattice vibrations is vital…

Materials Science · Physics 2017-11-22 Yi Xia , Maria K. Y. Chan

VO2 is a strongly correlated material, which undergoes a reversible metal insulator transition (MIT) coupled to a structural phase transition upon heating (T= 67{\deg} C). Since its discovery the nature of the insulating state has long been…

Strongly Correlated Electrons · Physics 2020-01-14 A. D'Elia , S. J. Rezvani , A. Cossaro , M. Stredansky , C. Grazioli , B. W. Li , C. W. Zou , M. Coreno , A. Marcelli
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