English
Related papers

Related papers: A novel non-adiabatic spin relaxation mechanism in…

200 papers

The connection between molecular vibrations and spin polarization in charge transport through molecular junctions is currently a topic of high interest, with important consequences for a variety of phenomena, such as chirality-induced spin…

Mesoscale and Nanoscale Physics · Physics 2025-03-13 Samuel L. Rudge , Christoph Kaspar , Rudolf Smorka , Riley J. Preston , Joseph Subotnik , Michael Thoss

An experiment demonstrating the quantum simulation of a spin-lattice Hamiltonian is proposed. Dipolar interactions between nuclear spins in a solid state lattice can be modulated by rapid radio-frequency pulses. In this way, the effective…

Quantum Physics · Physics 2007-05-23 Georgios Roumpos , Cyrus P. Master , Yoshihisa Yamamoto

We demonstrate electrical control of the spin relaxation time T_1 between Zeeman split spin states of a single electron in a lateral quantum dot. We find that relaxation is mediated by the spin-orbit interaction, and by manipulating the…

Mesoscale and Nanoscale Physics · Physics 2010-09-28 S. Amasha , K. MacLean , Iuliana P. Radu , D. M. Zumbuhl , M. A. Kastner , M. P. Hanson , A. C. Gossard

We present a flexible scheme to realize non-artificial non-Markovian dynamics of an electronic spin qubit, using a nitrogen-vacancy center in diamond where the inherent nitrogen spin serves as a regulator of the dynamics. By changing the…

Electronic spin superposition states enable nanoscale sensing through their sensitivity to the local environment, yet their sensitivity to vibrational motion also limits their coherence times. In molecular spin systems, chemical tunability…

Quantum Physics · Physics 2026-02-04 Stefan H. Lohaus , Kay T. Xia , Yongqiang Cheng , Ryan G. Hadt

We study the spin-phonon relaxation rate of both Kramers and non-Kramers molecular magnets in strongly diluted samples at low temperature. Using the "rotational" contribution to the spin-phonon Hamiltonian, universal formulae for the…

Strongly Correlated Electrons · Physics 2018-01-31 Le Tuan Anh Ho , Liviu F. Chibotaru

We explore how to encode more than a qubit in vanadyl porphyrin molecules hosting a electronic spin 1/2 coupled to a nuclear spin 7/2. The spin Hamiltonian and its parameters, as well as the spin dynamics, have been determined via a…

Quantum Physics · Physics 2021-01-29 I. Gimeno , A. Urtizberea , J. Román-Roche , D. Zueco , A. Camón , P. J. Alonso , O. Roubeau , F. Luis

Non-Hermiticity and chirality are two fundamental properties known to give rise to various intriguing phenomena. However, the interplay between these properties has been rarely explored. In this work, we bridge this gap by introducing an…

Quantum Physics · Physics 2024-11-26 Haowei Xu , Guoqing Wang , Changhao Li , Hao Tang , Paola Cappellaro , Ju Li

We study the behavior of the Rabi oscillations of a driven central spin (qubit) coupled to an antiferromagnetic spin bath (environment). It is found that the decoherence behavior of the central spin depends on the detuning, driving…

Quantum Physics · Physics 2011-02-11 Xiao-Zhong Yuan , Hsi-Sheng Goan , Ka-Di Zhu

We demonstrate that the combination of an external magnetic field and the intrinsic spin-orbit interaction results in nonadiabatic precession of the electron spin after transmission through a quantum point contact (QPC). We suggest that…

Mesoscale and Nanoscale Physics · Physics 2015-06-12 T. Li , O. P. Sushkov

NMR spin-spin relaxation in solids in strong magnetic fields is normally described only with the help of the secular part of the full spin-spin interaction Hamiltonian. This approximation is associated with the averaging of the spin-spin…

Statistical Mechanics · Physics 2012-09-11 Chahan M. Kropf , Boris V. Fine

We calculate the spin relaxation rates in a parabolic InSb quantum dots due to the spin interaction with acoustical phonons. We considered the deformation potential mechanism as the dominant electron-phonon coupling in the Pavlov-Firsov…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 C. L. Romano , G. E. Marques , L. Sanz , A. M. Alcalde

The implementation of a spin qubit in a quantum ring occupied by one or a few electrons is proposed. Quantum bit involves the Zeeman sublevels of the highest occupied orbital. Such a qubit can be initialized, addressed, manipulated, read…

Mesoscale and Nanoscale Physics · Physics 2011-03-07 Elzbieta Zipper , Marcin Kurpas , Janusz Sadowski , Maciej M. Maska

Recently experiments have shown very significant spin activity in biological molecules such as DNA, proteins, oligopeptides and aminoacids. Such molecules have in common their chiral structure, time reversal symmetry and the absence of…

Mesoscale and Nanoscale Physics · Physics 2020-07-29 Juan Daniel Torres , Raul Hidalgo , Solmar Varela , Ernesto Medina

We propose a quantum algorithm for inferring the molecular nuclear spin Hamiltonian from time-resolved measurements of spin-spin correlators, which can be obtained via nuclear magnetic resonance (NMR). We focus on learning the anisotropic…

The interaction between a central qubit spin and a surrounding bath of spins is critical to spin-based solid state quantum sensing and quantum information processing. Spin-bath interactions are typically strongly anisotropic, and rapid…

A clear separation of the time scales governing the dynamics of "slow" and "fast" degrees of freedom often serves as a prerequisite for the emergence of an independent low-energy theory. Here, we consider (slow) classical spins exchange…

Mesoscale and Nanoscale Physics · Physics 2022-09-30 Nicolas Lenzing , Alexander I. Lichtenstein , Michael Potthoff

Molecular spins are promising candidates for quantum information science, leveraging coherent electronic spin states for quantum sensing and computation. However, the practical application of these systems is hindered by electronic spin…

Quantum Physics · Physics 2026-03-03 Timothy J. Krogmeier , Anthony W. Schlimgen , Kade Head-Marsden

Twisted transition metal dichalcogenide (TMD) homobilayers have recently emerged as a powerful platform for studying correlated insulating states. In the strongly correlated limit, we construct an effective spin Hamiltonian on a honeycomb…

Strongly Correlated Electrons · Physics 2021-10-04 Mohammad-Hossein Zare , Hamid Mosadeq

Optically addressable spins are a promising platform for quantum information science due to their combination of a long-lived qubit with a spin-optical interface for external qubit control and read out. The ability to chemically synthesize…

Quantum Physics · Physics 2022-04-04 S. L. Bayliss , P. Deb , D. W. Laorenza , M. Onizhuk , G. Galli , D. E. Freedman , D. D. Awschalom