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We develop and implement a Gaussian approach to calculate partial cross-sections and asymmetry parameters for molecular photoionization. Optimal sets of complex Gaussian-type orbitals (cGTOs) are first obtained by non-linear optimization,…

Chemical Physics · Physics 2021-11-17 Abdallah Ammar , Lorenzo Ugo Ancarani , Arnaud Leclerc

The experimental binding energies of single-particle and single-hole neutron states belonging to neutron shells that extend from N = 126 to 184 and 82 to 126 respectively, have been reproduced by solving the Schr\"{o}dinger equation with a…

Nuclear Theory · Physics 2016-08-24 J. A. Liendo , E. Castro , R. Gómez , D. D. Caussyn

X-ray photoelectron spectra provide a wealth of information on the electronic structure. The extraction of molecular details requires adequate theoretical methods, which in case of transition metal complexes has to account for effects due…

We prove existence of spherically symmetric, static, self-gravitating photon shells as solutions to the massless Einstein-Vlasov system. The solutions are highly relativistic in the sense that the ratio $2m(r)/r$ is close to $8/9$, where…

General Relativity and Quantum Cosmology · Physics 2024-02-19 Håkan Andréasson , David Fajman , Maximilian Thaller

On the basis of first-principles GW calculations, we study the quasiparticle properties of the guanine, adenine, cytosine, thymine, and uracil DNA and RNA nucleobases. Beyond standard G0W0 calculations, starting from Kohn-Sham eigenstates…

Chemical Physics · Physics 2015-05-27 Carina Faber , Claudio Attaccalite , Valerio Olevano , Erich Runge , Xavier Blase

We apply a recently developed quasiparticle self-consistent $GW$ method (QSGW) to Gd, Er, EuN, GdN, ErAs, YbN and GdAs. We show that QSGW combines advantages separately found in conventional $GW$ and LDA+$U$ theory, in a simple and fully…

Materials Science · Physics 2007-11-10 Athanasios N. Chantis , Mark van Schilfgaarde , Takao Kotani

We implement the GW space-time method at finite temperatures, in which the Green's function G and the screened Coulomb interaction W are represented in the real space on a suitable mesh and in imaginary time in terms of Chebyshev…

Materials Science · Physics 2025-11-11 Sam Azadi , Arkadiy Davydov , Evgeny Kozik

We present the self-consistent Pauli equation, a semi-relativistic model for charged spin-$1/2$-particles with self-interaction with the electromagnetic field. The Pauli equation arises as the $O(1/c)$ approximation of the relativistic…

Mathematical Physics · Physics 2023-04-07 Jakob Möller , Norbert J. Mauser

This paper presents an auto-stabilized weak Galerkin (WG) finite element method for the Biot's consolidation model within the classical displacement-pressure two-field formulation. Unlike traditional WG approaches, the proposed scheme…

Numerical Analysis · Mathematics 2026-03-31 Chunmei Wang , Shangyou Zhang

Two state-of-the-art computational approaches: quantum Monte Carlo (QMC), based on accurate total energies, and GW with exciton effects (GW-BSE), based on perturbation theory are employed to calculate ionization potentials, electron…

Materials Science · Physics 2009-10-31 Jeffrey C. Grossman , Michael Rohlfing , Lubos Mitas , Steven G. Louie , Marvin L. Cohen

Accurate and efficient predictions of the quasiparticle properties of complex materials remain a major challenge due to the convergence issue and the unfavorable scaling of the computational cost with respect to the system size.…

Materials Science · Physics 2020-07-14 Weiyi Xia , Weiwei Gao , Gabriel Lopez-Candales , Yabei Wu , Wei Ren , Wenqing Zhang , Peihong Zhang

Green's function theory has emerged as a powerful many-body approach not only in condensed matter physics but also in quantum chemistry in recent years. We have developed a new all-electron implementation of the BSE@GW formalism using…

Chemical Physics · Physics 2024-10-15 Ruiyi Zhou , Yi Yao , Volker Blum , Xinguo Ren , Yosuke Kanai

Koopmans-compliant (KC) functionals have been shown to provide accurate spectral properties through a generalized condition of piece-wise linearity of the total energy as a function of the fractional addition/removal of an electron to/from…

Computational Physics · Physics 2019-07-09 Nicola Colonna , Ngoch Linh Nguyen , Andrea Ferretti , Nicola Marzari

In this paper we continue the development of a model for strong interactions at high energy, based on two ingredients: CGC/saturation approach and the BFKL Pomeron. In our approach, the unknown mechanism of confinement of quarks and gluons,…

High Energy Physics - Phenomenology · Physics 2015-05-20 E. Gotsman , E. Levin , U. Maor

For molecules and solids containing heavy elements, accurate electronic structure calculations require accounting not only for electronic correlations but also for relativistic effects. In molecules, relativity can lead to severe changes in…

Chemical Physics · Physics 2025-10-17 Gaurav Harsha , Vibin Abraham , Dominika Zgid

The Bethe-Salpeter equation (BSE) based on GW quasiparticle levels is a successful approach for calculating the optical gaps and spectra of solids and also for predicting the neutral excitations of small molecules. We here present an…

Materials Science · Physics 2020-02-19 Chi Liu , Jan Kloppenburg , Xinguo Ren , Heiko Appel , Yosuke Kanai , Volker Blum

A new kinetic self-consistent method is presented based on the proposed Gaussian Superposition Principle for computation of ensemble averaged observables of a macromolecule interacting via two-body forces. The latter leads to the derivation…

Statistical Mechanics · Physics 2025-05-15 Edward G. Timoshenko

This paper develops a weak Galerkin (WG) finite element method of arbitrary order for the steady incompressible Magnetohydrodynamics equations. The WG scheme uses piecewise polynomials of degrees $k(k\geq 1),k,k-1$, and $k-1$ respectively…

Numerical Analysis · Mathematics 2023-10-06 Min Zhang , Tong Zhang , Xiaoping Xie

The weak Galerkin (WG) finite element method is an effective and flexible general numerical technique for solving partial differential equations. It is a natural extension of the classic conforming finite element method for discontinuous…

Numerical Analysis · Mathematics 2020-04-29 Xiu Ye , Shangyou Zhang

We evaluate the performances of ab initio GW calculations for the ionization energies and HOMO-LUMO gaps of thirteen gas phase molecules of interest for organic electronic and photovoltaic applications, including the C60 fullerene,…

Materials Science · Physics 2011-04-01 Xavier Blase , Claudio Attaccalite , Valerio Olevano