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We introduce a refined tight-binding (TB) model for Pt-based jacutingaite materials Pt$_{2}N$X$_{3}$, ($N$ = Zn, Cd, Hg; X = S, Se, Te), offering a detailed representation of the low-energy physics of its monolayers. This model incorporates…

Materials Science · Physics 2024-10-11 G. Santos-Castro , L. K. Teles , I. Guilhon Mitoso , J. M. Pereira

The quantum mechanical motion of the atomic nuclei is considered over a single- or a multi-dimensional subspace of electronic states which is separated by a gap from the rest of the electronic spectrum over the relevant range of nuclear…

Chemical Physics · Physics 2019-07-24 Edit Matyus , Stefan Teufel

An approximate relativistic two-component Hamiltonian for use in molecular electronic structure calculations is derived in the form of a sum of fixed atom-centered kinetic and spin-orbit operators added to the non-relativistic Hamiltonian.…

Chemical Physics · Physics 2019-02-13 Dimitri N. Laikov

Multiple gaps in the tight-binding band of a pentagonal lattice are found. Unlike the Cairo pentagonal lattice this lattice is made of irregular pentagons with arms of different lengths. The tight-binding Hamiltonian is exactly solved to…

Mesoscale and Nanoscale Physics · Physics 2017-02-28 Susobhan Paul , Asim Kumar Ghosh

Magnetic properties of metals are investigated through electronic structure calculations based on the recently-proposed magnetic-field-containing relativistic tight-binding approximation (MFRTB) method [Phys. Rev. B \textbf{91}, 075122…

Strongly Correlated Electrons · Physics 2017-05-31 Masahiko Higuchi , Katsuhiko Higuchi

Electronic structure simulation is an anticipated application for quantum computers. Due to high-dimensional quantum entanglement in strongly correlated systems, the quantum resources required to perform such simulations are far beyond the…

Quantum Physics · Physics 2022-01-25 Jie Liu , Zhenyu Li , Jinlong Yang

Entanglement is one of the most fascinating concepts of modern physics. In striking contrast to its abstract, mathematical foundation, its practical side is, however, remarkably underdeveloped. Even for systems of just two orbitals or sites…

Quantum Physics · Physics 2022-07-08 Lexin Ding , Zoltan Zimboras , Christian Schilling

Based on the metastable electron-pair energy band in a two-dimensional (2D) periodic potential obtained previously by Hai and Castelano [J. Phys.: Condens. Matter 26, 115502 (2014)], we present in this work a Hamiltonian of many electrons…

Superconductivity · Physics 2015-01-21 G. -Q. Hai , F. M. Peeters

Parameterized tight-binding models fit to first principles calculations can provide an efficient and accurate quantum mechanical method for predicting properties of molecules and solids. However, well-tested parameter sets are generally…

Materials Science · Physics 2023-04-28 Kevin F. Garrity , Kamal Choudhary

The extended Hubbard Hamiltonian is a widely accepted model for uncovering the effects of strong correlations on the phase diagram of low-dimensional systems, and a variety of theoretical techniques have been applied to it. In this paper…

Strongly Correlated Electrons · Physics 2007-09-07 H. A. Craig , C. N. Varney , W. E. Pickett , R. T. Scalettar

We describe a semi-empirical atomic basis Extended H\"uckel Theoretical (EHT) technique that can be used to calculate bulk bandstructure, surface density of states, electronic transmission and interfacial chemistry of various materials…

Materials Science · Physics 2009-11-11 Diego Kienle , Jorge I. Cerda , Avik W. Ghosh

We present a tight-binding calculation that, for the first time, accurately describes the structural, vibrational and elastic properties of amorphous silicon. We compute the interatomic force constants and find an unphysical feature of the…

Materials Science · Physics 2009-11-10 J. L. Feldman , N. Bernstein , D. A. Papaconstantopoulos , M. J. Mehl

Quantum simulation of the electronic structure problem is one of the most researched applications of quantum computing. The majority of quantum algorithms for this problem encode the wavefunction using $N$ Gaussian orbitals, leading to…

We present a tight-binding potential based on the moment expansion of the density of states, which includes up to the fifth moment. The potential is fitted to bcc and hcp Zr and it is applied to the computation of vibrational properties of…

Materials Science · Physics 2009-10-31 Marcel Porta , Teresa Castan

The chemical bond is an important local concept to understand chemical compounds and processes. Unfortunately, like most local concepts, the chemical bond and the bond order do not correspond to any physical observable and thus cannot be…

Strongly Correlated Electrons · Physics 2017-09-13 Matthieu Mottet , Pawel Tecmer , Katharina Boguslawski , Ors Legeza , Markus Reiher

We analyze and present applications of a recently proposed empirical tight-binding scheme for investigating the effects of alloy disorder on various electronic and optical properties of semiconductor alloys, such as the band gap variation,…

Materials Science · Physics 2024-01-31 Anh-Luan Phan , Alessandro Pecchia , Alessia Di Vito , Matthias Auf der Maur

We analyze the scattering dynamics and spectrum of a quantum particle on a tight-binding lattice subject to a non-Hermitian (purely imaginary) local potential. The reflection, transmission and absorption coefficients are studied as a…

Quantum Physics · Physics 2020-07-20 Phillip C. Burke , Jan Wiersig , Masudul Haque

We show how lattice Quantum Monte Carlo can be applied to the electronic properties of carbon nanotubes in the presence of strong electron-electron correlations. We employ the path-integral formalism and use methods developed within the…

Strongly Correlated Electrons · Physics 2016-06-10 Thomas Luu , Timo A. Lähde

We describe the screened Korringa-Kohn-Rostoker (KKR) method and the third-generation linear muffin-tin orbital (LMTO) method for solving the single-particle Schroedinger equation for a MT potential. The simple and popular formalism which…

Condensed Matter · Physics 2007-05-23 O. K. Andersen , C. Arcangeli , R. W. Tank , T. Saha-Dasgupta , G. Krier , O. Jepsen , I. Dasgupta

We provide a comprehensive analysis of the prominent tight-binding (TB) models for transition metal dichalcogenides (TMDs) available in the literature. We inspect the construction of these TB models, discuss their parameterization used and…

Materials Science · Physics 2024-06-25 Bert Jorissen , Lucian Covaci , Bart Partoens