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A highly conductive metallic gas that is quantum mechanically confined at a solid-state interface is an ideal platform to explore nontrivial electronic states that are otherwise inaccessible in bulk materials. Although two-dimensional…

Materials Science · Physics 2021-10-13 Naotaka Kasuya , Junto Tsurumi , Toshihiro Okamoto , Shun Watanabe , Jun Takeya

The ongoing demand for more energy-efficient, high-performance electronics is driving the exploration of innovative materials and device architectures, where interfaces play a crucial role due to the continuous downscaling of device…

Applied Physics · Physics 2024-12-06 Chang Niu , Linjia Long , Yizhi Zhang , Zehao Lin , Pukun Tan , Jian-Yu Lin , Wenzhuo Wu , Haiyan Wang , Peide D. Ye

Electrides, with excess anionic electrons confined in their empty space, are promising for uses in catalysis, nonlinear optics and spin-electronics. However, the application of electrides is limited by their high chemical reactivity with…

Materials Science · Physics 2023-01-03 Xuhui Yang , Kevin Parrish , Yan-Ling Li , Baisheng Sa , Hongbing Zhan , Qiang Zhu

The infinite-layer nickelates, proposed as analogs to superconducting cuprates, provide a promising platform for exploring the mechanisms of unconventional superconductivity. However, the superconductivity under atmospheric pressure has…

Superconductivity · Physics 2025-01-23 Yin Yuan , Wu Mei , Ding Xiang , He Peiyi , Li Qize , Zhang Xiaowen , Zhu Ruixue , Mao Ruilin , Gao Xiaoyue , Shi Ruochen , Qiao Liang , Gao Peng

Atomically thin transition metal dichalcogenides (TMDs) are promising candidates for next-generation transistor channels due to their superior scaling properties. However, the integration of ultra-thin gate dielectrics remains a challenge,…

Two-dimensional electron systems with fascinating properties exist in multilayers of standard semiconductors, on helium surfaces, and in oxides. Compared to the two-dimensional (2D) electron gases of semiconductors, the 2D electron systems…

Strongly Correlated Electrons · Physics 2016-06-22 J. Zabaleta , V. S. Borisov , R. Wanke , H. O. Jeschke , S. C. Parks , B. Baum , A. Teker , T. Harada , K. Syassen , T. Kopp , N. Pavlenko , R. Valentí , J. Mannhart

Future electronics require aggressive scaling of channel material thickness while maintaining device performance. Two-dimensional (2D) semiconductors are promising candidates, but despite over two decades of research, experimental…

In conventional electrides, excess electrons are localized in crystal voids to serve as anions. Most of these electrides are metallic and the metal cations are primarily from the s-block, d-block, or rare-earth elements. Here, we report a…

Materials Science · Physics 2025-03-05 Jiaqi Dai , Feng Yang , Cong Wang , Fei Pang , Zhihai Cheng , Wei Ji

We create a two-dimensional electron system (2DES) at the interface between EuO, a ferromagnetic insulator, and SrTiO3, a transparent non-magnetic insulator considered the bedrock of oxide-based electronics. This is achieved by a controlled…

Quantum ground states which arise at atomically controlled oxide interfaces provide an opportunity to address key questions in condensed matter physics, including the nature of two-dimensional (2D) metallic behaviour often observed adjacent…

Heterostructures of transition metal oxides (TMO) perovskites represent an ideal platform to explore exotic phenomena involving the complex interplay between the spin, charge, orbital and lattice degrees of freedom available in these…

Oxide heterostructures have repeatedly been shown to display apical properties at the interfaces, some of which favorable to the formation of two-dimensional electron systems, as well as high transition temperature superconductivity. In…

Superconductivity · Physics 2022-12-21 Wai Hei Terence Tse , Carla Lupo , Evan Sheridan , Evgeny Plekhanov , Cedric Weber

Two-dimensional electron gas (2DEG) formed at the interface between two insulating oxides offers an opportunity for fundamental research and device applications. Binary alkaline earth metal oxides possess compatible lattice constants with…

The discovery of a two-dimensional electron gas (2DEG) at the interface between insulating oxides has led to a well-deserved level of excitement due to possible applications as "in-plane" all-oxide nanoelectronics. Here we expand the range…

Materials Science · Physics 2009-09-16 J. D. Burton , J. P. Velev , E. Y. Tsymbal

Accurate electronic structures of the technologically important lanthanide/rare earth sesquioxides (Ln2O3, with Ln=La,...,Lu) and CeO2 have been calculated using hybrid density functionals HSE03, HSE06 and screened-exchange (sX-LDA). We…

Materials Science · Physics 2016-11-11 Roland Gillen , Stewart J. Clark , John Robertson

Modifications of the electronic bands of thin FeSe films due to oxygen vacancies in the supporting SrTiO 3 (001) substrate - and the interplay with spin-orbit coupling, magnetism, and epitaxy - are investigated by first-principles supercell…

Materials Science · Physics 2017-01-11 M. X. Chen , Zhuozhi Ge , Y. Y. Li , D. F. Agterberg , L. Li , M. Weinert

The epitaxial growth of crystalline oxides on semiconductors provides a pathway to introduce new functionalities to semiconductor devices. Key to electrically coupling crystalline oxides with semiconductors to realize functional behavior is…

Materials Science · Physics 2014-10-28 J. Moghadam , K. Ahmadi-Majlan , X. Shen , T. Droubay , M. Bowden , M. Chrysler , D. Su , S. A. Chambers , J. H. Ngai

Knowledge of atomic-level details of structure, chemistry, and electronic states is paramount for a comprehensive understanding of emergent properties at oxide interfaces. We utilise a novel methodology based on atomic-scale electron energy…

A 2D electron gas system in an oxide heterostructure serves as an important playground for novel phenomena. Here, we show that, by using fractional delta-doping to control the interface's composition in LaxSr1-xTiO3/SrTiO3 artificial oxide…

Strongly Correlated Electrons · Physics 2012-09-28 Woo Seok Choi , Suyoun Lee , Valentino R. Cooper , Ho Nyung Lee

We build a theoretical model for the electronic properties of the two-dimensional (2D) electron gas that forms at the interface between insulating SrTiO$_3$ and a number of polar cap layers, including LaTiO$_3$, LaAlO$_3$, and GdTiO$_3$.…

Strongly Correlated Electrons · Physics 2017-02-13 Amany Raslan , Patrick Lafleur , W. A. Atkinson